ENTRY 10864 20200907 14731086400000001 SUBENT 10864001 20200907 14731086400100001 BIB 11 18 1086400100002 TITLE Cumulative yields of stable and long-lived isotopes 1086400100003 of ruthenium and palladium in neutron-induced fission 1086400100004 AUTHOR (M.Shima,H.G.Thode,R.H.Tomlinson) 1086400100005 INSTITUTE (1CANMCM) 1086400100006 REFERENCE (J,CJP,56,1340,1978) 1086400100007 #NSR:1978SH15 1086400100008 FACILITY (REAC,1CANMCM) 1086400100009 SAMPLE Sample sealed in small quartz capsule, wrapped in 1086400100010 aluminum foil, and placed in aluminum capsules. 1086400100011 DETECTOR 15-inch radius tandem mass spectrometer with cold trap 1086400100012 on source head to reduce hydrocarbon peaks. 1086400100013 METHOD (ASEP) Isotope dilution mass spectrometry. 1086400100014 ANALYSIS Data values averaged over several samples 1086400100015 CORRECTION Corrected for contamination by natural Ru,Pd,Cd, and Ag1086400100016 HISTORY (19791218C) 1086400100017 (19900529A) BIB update, Spectrum corrected 1086400100018 (20200907U) OG. Converted to lower case and 4-digit 1086400100019 year. #NSR added. STATUS updated. 1086400100020 ENDBIB 18 0 1086400100021 NOCOMMON 0 0 1086400100022 ENDSUBENT 21 0 1086400199999 SUBENT 10864002 20200907 14731086400200001 BIB 6 14 1086400200002 REACTION ((92-U-233(N,F)ELEM/MASS,CUM,FY,,SPA)/ 1086400200003 (92-U-233(N,F)44-RU-101,CUM,FY,,SPA)) 1086400200004 INC-SPECT Reactor neutrons 1086400200005 CORRECTION Ratios corrected for instrument mass discrimination 1086400200006 and for decay of Ru-103,106 during and after 1086400200007 irradiation. 1086400200008 Instrument calibration data obtained for the palladium 1086400200009 isotopes was extended to the ruthenium isotopes. 1086400200010 ERR-ANALYS (DATA-ERR) Data errors for isotopes 103 and 106 include1086400200011 half-life uncertainty 1086400200012 STATUS (TABLE) Tab.2 on p.1344 in Can.J.Chem.,56,1340,1978 1086400200013 HISTORY (19800812A) Data units corrected. 1086400200014 (19801029A) REACTION coded as ratio 1086400200015 (20200907U) OG. STATUS added. 1086400200016 ENDBIB 14 0 1086400200017 COMMON 2 3 1086400200018 EN-DUMMY ELEMENT 1086400200019 EV NO-DIM 1086400200020 0.0253 44. 1086400200021 ENDCOMMON 3 0 1086400200022 DATA 3 4 1086400200023 MASS DATA DATA-ERR 1086400200024 NO-DIM NO-DIM NO-DIM 1086400200025 102. 0.7461 0.0025 1086400200026 103. 0.556 0.014 1086400200027 104. 0.3021 0.0011 1086400200028 106. 0.0749 0.0004 1086400200029 ENDDATA 6 0 1086400200030 ENDSUBENT 29 0 1086400299999 SUBENT 10864003 20200907 14731086400300001 BIB 6 14 1086400300002 REACTION ((92-U-235(N,F)ELEM/MASS,CUM,FY,,SPA)/ 1086400300003 (92-U-235(N,F)44-RU-101,CUM,FY,,SPA)) 1086400300004 INC-SPECT Reactor neutrons 1086400300005 CORRECTION Ratios corrected for instrument mass discrimination 1086400300006 and for decay of Ru-103,106 during and after 1086400300007 irradiation. 1086400300008 Instrument calibration data obtained for the palladium 1086400300009 isotopes was extended to the ruthenium isotopes. 1086400300010 ERR-ANALYS (DATA-ERR) Data errors for isotopes 103 and 106 include1086400300011 half-life uncertainty 1086400300012 STATUS (TABLE) Tab.2 on p.1344 in Can.J.Chem.,56,1340,1978 1086400300013 HISTORY (19800812A) Data units corrected. 1086400300014 (19801029A) REACTION coded as ratio 1086400300015 (20200907U) OG. STATUS added. 1086400300016 ENDBIB 14 0 1086400300017 COMMON 2 3 1086400300018 EN-DUMMY ELEMENT 1086400300019 EV NO-DIM 1086400300020 0.0253 44. 1086400300021 ENDCOMMON 3 0 1086400300022 DATA 3 4 1086400300023 MASS DATA DATA-ERR 1086400300024 NO-DIM NO-DIM NO-DIM 1086400300025 102. 0.838 0.014 1086400300026 103. 0.611 0.04 1086400300027 104. 0.396 0.005 1086400300028 106. 0.0748 0.0005 1086400300029 ENDDATA 6 0 1086400300030 ENDSUBENT 29 0 1086400399999 SUBENT 10864004 20200907 14731086400400001 BIB 7 18 1086400400002 REACTION ((92-U-233(N,F)ELEM/MASS,CUM,FY,,SPA)/ 1086400400003 (92-U-233(N,F)46-PD-105,CUM,FY,,SPA)) 1086400400004 INC-SPECT Reactor neutrons 1086400400005 MONITOR Known concentrations of Pd and Ru isotopes used to 1086400400006 calibrate spectrometer. 1086400400007 CORRECTION Ratios corrected for 1086400400008 -instrument mass discrimination 1086400400009 -decay of Ru-106 to Pd-106 1086400400010 -neutron capture by Rh-105 which enhances Pd-106 yield1086400400011 at expense of Pd-105. 1086400400012 Instrument calibration data obtained for the palladium 1086400400013 isotopes was extended to the ruthenium isotopes. 1086400400014 ERR-ANALYS (DATA-ERR) Quoted errors include 1086400400015 contamination-correction uncertainty. 1086400400016 STATUS (TABLE) Tab.3 on p.1345 in Can.J.Chem.,56,1340,1978 1086400400017 HISTORY (19800812A) Data units corrected. 1086400400018 (19801029A) REACTION coded as ratio 1086400400019 (20200907U) OG. STATUS added. 1086400400020 ENDBIB 18 0 1086400400021 COMMON 2 3 1086400400022 EN-DUMMY ELEMENT 1086400400023 EV NO-DIM 1086400400024 0.0253 44. 1086400400025 ENDCOMMON 3 0 1086400400026 DATA 3 4 1086400400027 MASS DATA DATA-ERR 1086400400028 NO-DIM NO-DIM NO-DIM 1086400400029 106. 0.479 0.023 1086400400030 107. 0.2212 0.0014 1086400400031 108. 0.1482 0.0008 1086400400032 110. 0.0766 0.0007 1086400400033 ENDDATA 6 0 1086400400034 ENDSUBENT 33 0 1086400499999 SUBENT 10864005 20200907 14731086400500001 BIB 8 21 1086400500002 REACTION ((92-U-235(N,F)ELEM/MASS,CUM,FY,,SPA)/ 1086400500003 (92-U-235(N,F)46-PD-105,CUM,FY,,SPA)) 1086400500004 INC-SPECT Reactor neutrons 1086400500005 MONITOR Known concentrations of Pd and Ru isotopes used to 1086400500006 calibrate spectrometer. 1086400500007 CORRECTION Ratios corrected for 1086400500008 -instrument mass discrimination 1086400500009 -decay of Ru-106 to Pd-106 1086400500010 -neutron capture by Rh-105 which enhances Pd-106 yield1086400500011 at expense of Pd-105. 1086400500012 ERR-ANALYS (DATA-ERR) Quoted errors include 1086400500013 contamination-correction uncertainty. 1086400500014 Errors caused by interfering peaks and poor 1086400500015 spectrograph precision due to small sample size making 1086400500016 weighted mean for Pd-108 and Pd-110 poor. 1086400500017 FLAG (1.) Calculated by fitting individual runs to a 1086400500018 straight line and extrapolating. 1086400500019 STATUS (TABLE) Tab.4 on p.1345 in Can.J.Chem.,56,1340,1978 1086400500020 HISTORY (19800812A) Data units corrected. 1086400500021 (19801029A) REACTION coded as ratio 1086400500022 (20200907U) OG. STATUS added. 1086400500023 ENDBIB 21 0 1086400500024 COMMON 2 3 1086400500025 EN-DUMMY ELEMENT 1086400500026 EV NO-DIM 1086400500027 0.0253 46. 1086400500028 ENDCOMMON 3 0 1086400500029 DATA 4 4 1086400500030 MASS DATA DATA-ERR FLAG 1086400500031 NO-DIM NO-DIM NO-DIM NO-DIM 1086400500032 106. 0.406 0.006 1086400500033 107. 0.1540 0.0002 1086400500034 108. 0.0555 0.0005 1. 1086400500035 110. 0.0258 0.0004 1. 1086400500036 ENDDATA 6 0 1086400500037 ENDSUBENT 36 0 1086400599999 SUBENT 10864006 20200907 14731086400600001 BIB 8 17 1086400600002 REACTION ((94-PU-239(N,F)ELEM/MASS,CUM,FY,,SPA)/ 1086400600003 (94-PU-239(N,F)46-PD-105,CUM,FY,,SPA)) 1086400600004 INC-SPECT Reactor neutrons 1086400600005 MONITOR Known concentrations of Pd and Ru isotopes used to 1086400600006 calibrate spectrometer. 1086400600007 CORRECTION Ratios corrected for 1086400600008 -instrument mass discrimination 1086400600009 -decay of Ru-106 to Pd-106 1086400600010 -neutron capture by Rh-105 which enhances Pd-106 yield1086400600011 at expense of Pd-105. 1086400600012 ERR-ANALYS (DATA-ERR) Quoted errors include 1086400600013 contamination-correction uncertainty 1086400600014 FLAG (1.) Average value rather than weighted mean 1086400600015 STATUS (TABLE) Tab.5 on p.1345 in Can.J.Chem.,56,1340,1978 1086400600016 HISTORY (19800812A) Data units corrected. 1086400600017 (19801029A) REACTION coded as ratio 1086400600018 (20200907U) OG. STATUS added. 1086400600019 ENDBIB 17 0 1086400600020 COMMON 2 3 1086400600021 EN-DUMMY ELEMENT 1086400600022 EV NO-DIM 1086400600023 0.0253 46. 1086400600024 ENDCOMMON 3 0 1086400600025 DATA 4 4 1086400600026 MASS DATA DATA-ERR FLAG 1086400600027 NO-DIM NO-DIM NO-DIM NO-DIM 1086400600028 106. 0.747 0.021 1. 1086400600029 107. 0.5665 0.0011 1086400600030 108. 0.3701 0.0007 1086400600031 110. 0.1101 0.0003 1086400600032 ENDDATA 6 0 1086400600033 ENDSUBENT 32 0 1086400699999 SUBENT 10864007 20200907 14731086400700001 BIB 8 14 1086400700002 REACTION (92-U-233(N,F)MASS,CHN,FY,,SPA) 1086400700003 INC-SPECT Reactor neutrons 1086400700004 MONITOR (92-U-233(N,F)44-RU-101,CUM,FY,,SPA) Used to derive 1086400700005 absolute normalization. 1086400700006 MONIT-REF (,M.E.Meek+,P,NEDO-12154-1,1974) 1086400700007 METHOD Pd normalized relative to Ru using known concentrations1086400700008 of Ru-100 and Pd-104 1086400700009 ERR-ANALYS (DATA-ERR) No information on sources of uncertainties 1086400700010 STATUS (DEP,10864002) 1086400700011 (DEP,10864004) 1086400700012 (TABLE) Tab.7 on p.1347 in Can.J.Chem.,56,1340,1978 1086400700013 HISTORY (19810309A) Isotope corrected. 1086400700014 (19820514A) Data table correction. 1086400700015 (20200907U) OG. STATUS updated, MONIT-REF added. 1086400700016 ENDBIB 14 0 1086400700017 COMMON 3 3 1086400700018 EN-DUMMY MONIT MONIT-ERR 1086400700019 EV PC/FIS PC/FIS 1086400700020 0.0253 3.22 0.03 1086400700021 ENDCOMMON 3 0 1086400700022 DATA 3 8 1086400700023 MASS DATA DATA-ERR 1086400700024 NO-DIM PC/FIS PC/FIS 1086400700025 102. 2.40 0.03 1086400700026 103. 1.79 0.05 1086400700027 104. 0.97 0.01 1086400700028 105. 0.521 0.016 1086400700029 106. 0.241 0.002 1086400700030 107. 0.116 0.004 1086400700031 108. 0.078 0.003 1086400700032 110. 0.0399 0.0013 1086400700033 ENDDATA 10 0 1086400700034 ENDSUBENT 33 0 1086400799999 SUBENT 10864008 20200907 14731086400800001 BIB 8 14 1086400800002 REACTION (92-U-235(N,F)MASS,CHN,FY,,SPA) 1086400800003 INC-SPECT Reactor neutrons 1086400800004 MONITOR (92-U-235(N,F)44-RU-101,CUM,FY,,MXW) Used to derive 1086400800005 absolute normalization. 1086400800006 MONIT-REF (,M.E.Meek+,P,NEDO-12154-1,1974) 1086400800007 METHOD Relative yields of Pd isotopes normalized to Ru using 1086400800008 ratio of Pd to Ru obtained from isotope dilution 1086400800009 measurements. 1086400800010 ERR-ANALYS (DATA-ERR) No information on sources of uncertainties 1086400800011 STATUS (DEP,10864003) 1086400800012 (DEP,10864005) 1086400800013 (TABLE) Tab.8 on p.1347 in Can.J.Chem.,56,1340,1978 1086400800014 HISTORY (19810309A) Monitor value corrected. 1086400800015 (20200907U) OG. STATUS updated, MONIT-REF added. 1086400800016 ENDBIB 14 0 1086400800017 COMMON 3 3 1086400800018 EN-DUMMY MONIT MONIT-ERR 1086400800019 EV PC/FIS PC/FIS 1086400800020 0.0253 5.04 0.05 1086400800021 ENDCOMMON 3 0 1086400800022 DATA 3 8 1086400800023 MASS DATA DATA-ERR 1086400800024 NO-DIM PC/FIS PC/FIS 1086400800025 102. 4.22 0.08 1086400800026 103. 3.08 0.21 1086400800027 104. 2.00 0.03 1086400800028 105. 0.941 0.017 1086400800029 106. 0.376 0.003 1086400800030 107. 0.145 0.003 1086400800031 108. 0.0523 0.0013 1086400800032 110. 0.0243 0.0005 1086400800033 ENDDATA 10 0 1086400800034 ENDSUBENT 33 0 1086400899999 SUBENT 10864009 20200907 14731086400900001 BIB 7 9 1086400900002 REACTION (94-PU-239(N,F)MASS,CHN,FY,,SPA) 1086400900003 INC-SPECT Reactor neutrons 1086400900004 MONITOR (94-PU-239(N,F)44-RU-106,CUM,FY,,SPA) Used to derive 1086400900005 absolute normalization. 1086400900006 MONIT-REF (,M.E.Meek+,P,NEDO-12154-1,1974) 1086400900007 ERR-ANALYS (DATA-ERR) No information on sources of uncertainties 1086400900008 STATUS (DEP,10864006) 1086400900009 (TABLE) Tab.9 on p.1348 in Can.J.Chem.,56,1340,1978 1086400900010 HISTORY (20200907U) OG. STATUS updated, MONIT-REF added. 1086400900011 ENDBIB 9 0 1086400900012 COMMON 3 3 1086400900013 EN-DUMMY MONIT MONIT-ERR 1086400900014 EV PC/FIS PC/FIS 1086400900015 0.0253 4.28 0.12 1086400900016 ENDCOMMON 3 0 1086400900017 DATA 3 4 1086400900018 MASS DATA DATA-ERR 1086400900019 NO-DIM PC/FIS PC/FIS 1086400900020 105. 5.73 0.23 1086400900021 107. 3.24 0.13 1086400900022 108. 2.12 0.08 1086400900023 110. 0.63 0.03 1086400900024 ENDDATA 6 0 1086400900025 ENDSUBENT 24 0 1086400999999 SUBENT 10864010 20200907 14731086401000001 BIB 5 7 1086401000002 REACTION ((92-U-235(N,F)ELEM/MASS,CUM,FY,,EPI)/ 1086401000003 (92-U-235(N,F)44-RU-101,CUM,FY,,EPI)) 1086401000004 INC-SPECT Epicadmium spectrum 1086401000005 ERR-ANALYS (DATA-ERR) No information on sources of uncertainties 1086401000006 STATUS (TABLE) Tab.10 on p.1348 in Can.J.Chem.,56,1340,1978 1086401000007 HISTORY (19900529C) 1086401000008 (20200907U) OG. STATUS added. 1086401000009 ENDBIB 7 0 1086401000010 COMMON 1 3 1086401000011 EN-MIN 1086401000012 EV 1086401000013 0.5 1086401000014 ENDCOMMON 3 0 1086401000015 DATA 4 7 1086401000016 ELEMENT MASS DATA DATA-ERR 1086401000017 NO-DIM NO-DIM NO-DIM NO-DIM 1086401000018 44. 102. 0.920 0.018 1086401000019 44. 104. 0.628 0.016 1086401000020 44. 106. 0.158 0.007 1086401000021 46. 105. 0.235 0.006 1086401000022 46. 107. 0.055 0.004 1086401000023 46. 108. 0.040 0.002 1086401000024 46. 110. 0.0135 0.0010 1086401000025 ENDDATA 9 0 1086401000026 ENDSUBENT 25 0 1086401099999 SUBENT 10864011 20200907 14731086401100001 BIB 5 7 1086401100002 REACTION ((94-PU-239(N,F)ELEM/MASS,CUM,FY,,EPI)/ 1086401100003 (94-PU-239(N,F)44-RU-101,CUM,FY,,EPI)) 1086401100004 INC-SPECT Epicadmium spectrum 1086401100005 ERR-ANALYS (DATA-ERR) No information on sources of uncertainties 1086401100006 STATUS (TABLE) Tab.11 on p.1349 in Can.J.Chem.,56,1340,1978 1086401100007 HISTORY (19900529C) 1086401100008 (20200907U) OG. STATUS added. 1086401100009 ENDBIB 7 0 1086401100010 COMMON 1 3 1086401100011 EN-MIN 1086401100012 EV 1086401100013 0.5 1086401100014 ENDCOMMON 3 0 1086401100015 DATA 4 7 1086401100016 ELEMENT MASS DATA DATA-ERR 1086401100017 NO-DIM NO-DIM NO-DIM NO-DIM 1086401100018 44. 102. 1.064 0.008 1086401100019 44. 104. 1.010 0.005 1086401100020 44. 106. 0.641 0.010 1086401100021 46. 105. 0.90 0.05 1086401100022 46. 107. 0.42 0.10 1086401100023 46. 108. 0.23 0.09 1086401100024 46. 110. 0.08 0.04 1086401100025 ENDDATA 9 0 1086401100026 ENDSUBENT 25 0 1086401199999 ENDENTRY 11 0 1086499999999