ENTRY 23098 20220212 23102309800000001 SUBENT 23098001 20220212 23102309800100001 BIB 14 49 2309800100002 TITLE Measurement and spectroscopy of radioactive isotopes 2309800100003 by LOHENGRIN and ISOLDE 2309800100004 AUTHOR (U.Koester) 2309800100005 REFERENCE (T,KOESTER,2000) PhD Thesis of Ulli Koester, 2309800100006 Physik-Department der Technischen Universitaet Munchen.2309800100007 Data tables and exp. details. In German. 2309800100008 (J,NP/A,734,213,2004) Author F.Goennenwein. 2309800100009 Graph for U-235 chain yield (DEP, Subent 005). 2309800100010 (J,NP/A,652,371,1999) - prelim.data 2309800100011 INSTITUTE (2FR ILL) 2309800100012 FACILITY (REAC,2FR ILL) High-flux reactor of ILL. 2309800100013 58 MW thermal power, 1.5E+15 cm**2/s maximum 2309800100014 unperturbed flux. 2309800100015 Recoil separator LOHENGRIN: 2309800100016 -main magnet for p/q separation, 2309800100017 -condenser for E/q separation, 2309800100018 -RED magnet, 2309800100019 DETECTOR (IOCH) - ionization chamber in focal plane. 2309800100020 Flight time of fragments from target to detector below2309800100021 2 micros. 2309800100022 Energy and nuclear charge calibration of IOCH was done2309800100023 with reference spectra using separator settings A/q=3.2309800100024 One channel approximately corresponds to 75 keV. 2309800100025 INC-SOURCE (REAC) 2309800100026 INC-SPECT At target position, about 50 cm from reactor core, 2309800100027 the thermal neutron flux about 5.3E+14 /cm**2/s . 2309800100028 Epithermal flux was more than two orders of magnitude 2309800100029 smaller; fast flux was more than three orders of 2309800100030 magnitude smaller. Both contribution can be neglected.2309800100031 SAMPLE Targets of high isotopic purity were produced by 2309800100032 deposition of actinide material as oxide on 2309800100033 platinum-coated titanium backing. 2309800100034 METHOD (EDE) 2309800100035 Absolute energy calibration of separator by: 2309800100036 Li-6(n,a)t Et=2.73 MeV, Ea=2.05 MeV; 2309800100037 Ni-59(n,a) Ea=4.78 MeV; 2309800100038 Cm-242 decay alphas with up to 6.11 MeV. 2309800100039 CORRECTION For : backgrounds, separator acceptance, target burnup2309800100040 energy loss. 2309800100041 First experiment indicated evidence for possible 2309800100042 additional contribution of light charge particles from2309800100043 extremely asymmetric binary fission, but more 2309800100044 systematic studies need to be performed for proof. 2309800100045 ANALYSIS Total yield of an isotope was determined by 2309800100046 integration over different kinetic energies. 2309800100047 ADD-RES (COMP) Comparison with model predictions. 2309800100048 HISTORY (20100112C) M.M. 2309800100049 (20130203U) SD: Small correction in SAMPLE in Subent 5.2309800100050 (20220212U) SD: Ref. NP/A,652,371 added. 2309800100051 ENDBIB 49 0 2309800100052 COMMON 1 3 2309800100053 EN-DUMMY 2309800100054 EV 2309800100055 0.025 2309800100056 ENDCOMMON 3 0 2309800100057 ENDSUBENT 56 0 2309800199999 SUBENT 23098002 20100112 22212309800200001 BIB 6 42 2309800200002 REACTION 1((94-PU-241(N,F)ELEM/MASS,TER,FY,,MXW)/ 2309800200003 (94-PU-241(N,F)2-HE-4,TER,FY,,MXW)) 2309800200004 2(94-PU-241(N,F)ELEM/MASS,TER,KE,,MXW) Emean . 2309800200005 SAMPLE Four Pu-241 targets prepared by IRMM: 2309800200006 Total mass Area Cover Thickness 2309800200007 microg cm**2 Angstrom microg Pu/cm**2 2309800200008 636 7x0.5 2500 Ni 208 2309800200009 1157 7x0.5 2500 Ni 362 2309800200010 1268 7x0.5 2500 Ni 379 2309800200011 350 7x0.5 2500 Ni. 100 2309800200012 1-st was used at measurement of binary fission; 2309800200013 4-th was used to exactly measure the energy 2309800200014 distribution of helium isotopes down to 3 MeV; 2309800200015 2-nd and 3-rd served for measurement of ternary fission2309800200016 yields relative to Be-10. 2309800200017 At the time of the measurements for three targets about2309800200018 20%, 31%, 28% respectively of the Pu-241 had decayed to2309800200019 Am-241, but during two weeks of measurement the 2309800200020 contribution of other fissile isotopes (e.g. from 2309800200021 bred Am-242(n,f)) will stay below 6%. The last target 2309800200022 was used 9 months after plutonium separation, thus 2309800200023 limiting contributions from other fissile systems 2309800200024 below 2 %. 2309800200025 ANALYSIS Emean (DATA 2) and Efwhm (MISC2) were obtained by 2309800200026 fitting a Gaussian distribution to data points. 2309800200027 Yields were normalized to a standard of 10000 for He-4.2309800200028 Yield of He-4 can be determined from small energy range2309800200029 (10 to 13 MeV). 2309800200030 ERR-ANALYS (DATA-ERR) Individual errors for each isotope, 2309800200031 do not include the error of the reference point and 2309800200032 systematic error due to non-Gaussian behavior in the 2309800200033 fit range. 2309800200034 MISC-COL (MISC1) Emean, taken from systematics, fixed. 2309800200035 (MISC2) Efwhm obtained by fitting. 2309800200036 (MISC3) Efwhm from systematics, fixed. 2309800200037 (MISC4) Maximum kinetic energy Ebin which the light 2309800200038 charged particle could attain if it was produced in a 2309800200039 binary reaction, e.g. Pu-241(n,alpha)U-238 . 2309800200040 For lighter isotopes it's evident from the high 2309800200041 energies (>Ebin) that they are indeed produced in 2309800200042 ternary fission. 2309800200043 STATUS (TABLE) Tables 1.5.1, 1.5.2, A.5.7 of T,KOESTER. 2309800200044 ENDBIB 42 0 2309800200045 NOCOMMON 0 0 2309800200046 DATA 12 59 2309800200047 ELEMENT MASS DATA 1DATA-ERR 1DATA-MAX 1DATA 22309800200048 DATA-ERR 2MISC1 MISC2 MISC2-ERR MISC3 MISC4 2309800200049 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM MEV 2309800200050 MEV MEV MEV MEV MEV MEV 2309800200051 1. 2. 42. E-04 4. E-04 2309800200052 8.4 7.4 0.4 2309800200053 1. 3. 786. E-04 42. E-04 2309800200054 8.4 7.2 0.4 2309800200055 2. 4. 1. 700. E-04 2309800200056 15.9 10.7 0.5 11.1 2309800200057 2. 6. 260. E-04 30. E-04 11.3 2309800200058 0.2 10.3 0.5 1. 2309800200059 2. 8. 15. E-04 1. E-04 8.7 2309800200060 0.2 9.6 0.5 2309800200061 3. 7. 6.7 E-04 0.6 E-04 14.7 2309800200062 0.5 11.6 1.2 3.7 2309800200063 3. 8. 4.2 E-04 0.6 E-04 15.7 2309800200064 1.1 13.9 2.2 2309800200065 3. 9. 8.3 E-04 0.8 E-04 12.6 2309800200066 0.6 14.6 1.0 2309800200067 3. 11. 0.0045E-04 0.0015E-04 2309800200068 11. 12.9 2309800200069 4. 7. 0.2 E-04 2309800200070 20. 15.3 1. 2309800200071 4. 9. 4.4 E-04 0.5 E-04 17.9 2309800200072 0.6 15.2 1.6 10.5 2309800200073 4. 10. 46. E-04 6. E-04 18. 2309800200074 0.7 18.8 2.9 12.4 2309800200075 4. 11. 5.9 E-04 1.7 E-04 17.5 2309800200076 0.7 14.1 2.4 6.7 2309800200077 4. 12. 2.8 E-04 0.3 E-04 14.3 2309800200078 0.8 15.7 2.2 4.8 2309800200079 4. 14. 0.0027E-04 0.0010E-04 2309800200080 13. 15.3 2309800200081 5. 10. 0.03 E-04 2309800200082 22. 21.2 9.4 2309800200083 5. 11. 1.6 E-04 1.0 E-04 2309800200084 21. 20. 15.7 2309800200085 5. 12. 1.0 E-04 0.4 E-04 2309800200086 20. 18.8 13.4 2309800200087 5. 14. 0.13 E-04 0.04 E-04 2309800200088 19. 17.6 8. 2309800200089 5. 15. 0.046E-04 0.010E-04 17.7 2309800200090 0.6 15.2 1.2 5.8 2309800200091 5. 17. 0.001E-04 2309800200092 16. 15.3 2309800200093 6. 14. 12.6 E-04 0.8 E-04 20.8 2309800200094 0.6 25.4 2.2 27.4 2309800200095 6. 15. 4.3 E-04 0.4 E-04 18.6 2309800200096 1.3 27.1 3.1 22.5 2309800200097 6. 16. 5.0 E-04 0.9 E-04 16.6 2309800200098 2.7 30. 7. 22.1 2309800200099 6. 17. 0.64 E-04 0.15 E-04 2309800200100 18. 23.5 16.7 2309800200101 6. 18. 0.28 E-04 0.05 E-04 17.7 2309800200102 1.7 17.9 2.2 16. 2309800200103 6. 19. 0.0025E-04 0.0014E-04 2309800200104 17. 20. 10.1 2309800200105 6. 20. 0.0036E-04 0.0028E-04 2309800200106 16. 18.8 8.4 2309800200107 15. 7. 0.044E-04 2309800200108 22. 21.2 3.5 29.3 2309800200109 15. 8. 0.12E-04 2309800200110 24. 23.5 23.6 2309800200111 16. 7. 0.079E-04 0.032E-04 2309800200112 21. 23.5 26.2 2309800200113 17. 7. 0.34 E-04 0.10 E-04 2309800200114 20. 23.5 27.3 2309800200115 18. 7. 0.16 E-04 0.04 E-04 2309800200116 19. 21.9 2.3 24.3 2309800200117 19. 7. 0.26 E-04 0.08 E-04 2309800200118 18. 21.2 24.7 2309800200119 19. 8. 0.26 E-04 0.12 E-04 2309800200120 23. 23.5 34.5 2309800200121 19. 9. 0.020E-04 0.016E-04 2309800200122 26. 25.9 35.9 2309800200123 20. 7. 0.0029E-04 0.0016E-04 2309800200124 17.5 20.6 21. 2309800200125 20. 8. 1.10 E-04 0.12 E-04 22.1 2309800200126 0.9 21.7 2.4 37.5 2309800200127 20. 9. 0.002E-04 2309800200128 25. 27. 36.9 2309800200129 21. 7. 0.0025E-04 0.0014E-04 2309800200130 17. 20. 20.6 2309800200131 21. 8. 0.23 E-04 0.06 E-04 2309800200132 21. 19.9 4.1 35.1 2309800200133 21. 9. 0.021E-04 0.006E-04 2309800200134 23. 22.6 8.8 40.3 2309800200135 22. 8. 0.12 E-04 0.04 E-04 2309800200136 20. 18.8 37.4 2309800200137 22. 9. 0.30 E-04 0.21 E-04 2309800200138 23. 27. 40. 2309800200139 24. 8. 0.08E-04 2309800200140 18. 21.2 33.2 2309800200141 24. 9. 0.030E-04 0.016E-04 2309800200142 21. 26.2 3.8 40.9 2309800200143 24. 10. 0.040E-04 0.012E-04 2309800200144 25. 23.5 3.2 52.8 2309800200145 24. 11. 0.001E-04 2309800200146 28. 28.2 2309800200147 27. 10. 0.008E-04 2309800200148 24. 25.9 48.4 2309800200149 27. 11. 0.005E-04 2309800200150 26. 28.2 57.7 2309800200151 27. 12. 0.0012E-04 2309800200152 30. 30.6 2309800200153 28. 11. 0.006E-04 0.004E-04 2309800200154 26. 28.2 55.9 2309800200155 28. 12. 0.018E-04 2309800200156 30. 30.6 67.4 2309800200157 30. 11. 0.0008E-04 2309800200158 24. 28.2 53.1 2309800200159 30. 12. 0.009E-04 0.006E-04 2309800200160 28. 30.6 67.9 2309800200161 30. 13. 0.002E-04 2309800200162 32. 33. 2309800200163 34. 14. 0.001E-04 2309800200164 36. 35.3 58.3 2309800200165 35. 14. 0.003E-04 2309800200166 35. 35.3 78.4 2309800200167 36. 14. 0.004E-04 2309800200168 33. 35.3 80.4 2309800200169 ENDDATA 122 0 2309800200170 ENDSUBENT 169 0 2309800299999 SUBENT 23098003 20100112 22212309800300001 BIB 6 28 2309800300002 REACTION (94-PU-241(N,F)ELEM/MASS,TER,FY,,MXW) 2309800300003 Absolute yields per fission. 2309800300004 SAMPLE Four Pu-241 targets prepared by IRMM: 2309800300005 Total mass Area Cover Thickness 2309800300006 microg cm**2 Angstrom microg Pu/cm**2 2309800300007 636 7x0.5 2500 Ni 208 2309800300008 1157 7x0.5 2500 Ni 362 2309800300009 1268 7x0.5 2500 Ni 379 2309800300010 350 7x0.5 2500 Ni. 100 2309800300011 1-st was used at measurement of binary fission; 2309800300012 4-th was used to exactly measure the energy 2309800300013 distribution of helium isotopes down to 3 MeV; 2309800300014 2-nd and 3-rd served for measurement of ternary fission2309800300015 yields relative to Be-10. 2309800300016 At the time of the measurements for three targets about2309800300017 20%, 31%, 28% respectively of the Pu-241 had decayed to2309800300018 Am-241, but during two weeks of measurement the 2309800300019 contribution of other fissile isotopes (e.g. from 2309800300020 bred Am-242(n,f)) will stay below 6%. The last target 2309800300021 was used 9 months after plutonium separation, thus 2309800300022 limiting contributions from other fissile systems 2309800300023 below 2 %. 2309800300024 ANALYSIS Absolute yields could be identified in the 2309800300025 deltaE-E-scatter plot. 2309800300026 ERR-ANALYS (DATA-ERR) Not specified. 2309800300027 STATUS (TABLE) Text of T,KOESTER, page 26 . 2309800300028 HISTORY (20100112C) 2309800300029 PRT/FIS -> PRD/FIS according to comment N.Otsuka,NDS.2309800300030 ENDBIB 28 0 2309800300031 NOCOMMON 0 0 2309800300032 DATA 4 3 2309800300033 ELEMENT MASS DATA DATA-ERR 2309800300034 NO-DIM NO-DIM PRD/FIS PRD/FIS 2309800300035 3. 11. 8.4E-10 2.8E-10 2309800300036 4. 14. 5.0E-10 1.9E-10 2309800300037 5. 19. 4.7E-10 2.6E-10 2309800300038 ENDDATA 5 0 2309800300039 ENDSUBENT 38 0 2309800399999 SUBENT 23098004 20100112 22212309800400001 BIB 8 43 2309800400002 REACTION 1((96-CM-245(N,F)ELEM/MASS,TER,FY,,MXW)/ 2309800400003 (96-CM-245(N,F)2-HE-4,TER,FY,,MXW)) 2309800400004 2(96-CM-245(N,F)ELEM/MASS,TER,KE,,MXW) Emean . 2309800400005 SAMPLE Three Cm-245 targets: 2309800400006 first two prepared by 4RUSEPA as Cm oxide,beside Cm-2452309800400007 (98.8% of Cm fraction) mainly the non-fissile isotopes2309800400008 Cm-244 and Cm-246 and small traces of radioactive decay2309800400009 daughters Pu-241 and Am-241 are present; 2309800400010 third of 3mm diameter spot- by Mainz University 2309800400011 Chemistry Department from Cm-245 separated at 1USAORL. 2309800400012 Contribution of impurities was neglected. 2309800400013 Total mass Area Cover Thickness 2309800400014 microg cm**2 Angstrom microg/cm**2 2309800400015 13.3 1x0.4 2500 Ni 33. 2309800400016 10.4 1x0.4 2500 Ni 26. 2309800400017 4. 0.07 2500 Ni - 2309800400018 ANALYSIS Emean (DATA 2) and Efwhm (MISC2) were obtained by 2309800400019 fitting a Gaussian distribution to data points. 2309800400020 To calculate the elemental yield of hydrogen and the 2309800400021 total ternary yield, the sum of proton and deuteron 2309800400022 yield was estimated to (2.0+-0.5) % of LRA yield. 2309800400023 Yields were normalized to a standard of 10000 for He-4.2309800400024 Yield of He-4 can be determined from small energy range2309800400025 (10 to 13 MeV). 2309800400026 ERR-ANALYS (DATA-ERR) Individual errors for each isotope, 2309800400027 do not include the error of the reference point and 2309800400028 systematic error due to non-Gaussian behavior in the 2309800400029 fit range. 2309800400030 MISC-COL (MISC1) Emean, taken from systematics, fixed. 2309800400031 (MISC2) Efwhm obtained by fitting. 2309800400032 (MISC3) Efwhm from systematics, fixed. 2309800400033 FLAG (1.) Yield was evaluated under two different 2309800400034 assumptions for the mean energy: 2309800400035 - once with the average value of all fissile 2309800400036 systems reported in B,WAGEMANS 2309800400037 (2.) and once with the value reported in T,KOZCON 2309800400038 (see REL-REF) . 2309800400039 REL-REF (R,,C.Wagemans,B,WAGEMANS,,199,1991) 2309800400040 Charged-particle-induced fission,1991, pp.199-226. 2309800400041 (R,,P.Kozcon,T,KOZCON,1988) 2309800400042 Mass and energy distributions of the products from 2309800400043 the 245Cm(nth,f) reaction, Ph.D. thesis, TH Darmstadt.2309800400044 STATUS (TABLE) Tables 1.5.3, 1.5.4, A.5.10 of T,KESTREL. 2309800400045 ENDBIB 43 0 2309800400046 NOCOMMON 0 0 2309800400047 DATA 12 46 2309800400048 ELEMENT MASS DATA 1DATA-ERR 1DATA-MAX 1DATA 22309800400049 DATA-ERR 2MISC1 MISC2 MISC2-ERR MISC3 FLAG 2309800400050 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM MEV 2309800400051 MEV MEV MEV MEV MEV NO-DIM 2309800400052 1. 3. 679. E-4 44. E-4 2309800400053 8.4 7.4 0.3 2309800400054 2. 3. 0.6 E-4 2309800400055 20. 10. 2309800400056 2. 4. 1. 600. 2309800400057 15.9 11.6 0.5 1. 2309800400058 2. 4. 11900.E-4 600. E-4 2309800400059 16.8 12.7 0.5 2. 2309800400060 2. 6. 286. E-4 16. E-4 11.3 2309800400061 0.4 11.2 0.7 2309800400062 2. 8. 19. E-4 4. E-4 10.4 2309800400063 0.9 12.8 2.5 2309800400064 3. 6. 0.3 E-4 2309800400065 20. 10. 2309800400066 3. 7. 13.6 E-4 1.3 E-4 15.1 2309800400067 0.7 14.3 1.3 2309800400068 3. 8. 5.6 E-4 0.8 E-4 15.8 2309800400069 1.1 14.1 2.7 2309800400070 3. 9. 13.6 E-4 1.7 E-4 13.4 2309800400071 0.7 15.2 2.4 2309800400072 3. 11. 0.010 E-4 0.006E-4 2309800400073 12. 12. 2309800400074 4. 9. 9.1 E-4 1.1 E-4 18.3 2309800400075 1.1 19.6 2.7 2309800400076 4. 10. 66. E-4 5. E-4 19.2 2309800400077 0.6 17.5 1.6 2309800400078 4. 11. 8.1 E-4 1.0 E-4 15.6 2309800400079 0.8 17.5 2.3 2309800400080 4. 12. 5.5 E-4 0.7 E-4 14.2 2309800400081 0.9 18.0 2.0 2309800400082 4. 14. 0.018 E-4 0.012E-4 2309800400083 14. 14. 2309800400084 5. 10. 0.3 E-4 2309800400085 25. 20. 2309800400086 5. 11. 2.4 E-4 1.3 E-4 2309800400087 22. 18. 2309800400088 5. 12. 2.3 E-4 0.4 E-4 20.6 2309800400089 1.5 18.1 2.2 2309800400090 5. 13. 2.2 E-4 0.6 E-4 20.3 2309800400091 1.3 16.7 5.8 2309800400092 5. 14. 0.21 E-4 0.06 E-4 2309800400093 19. 17. 2309800400094 5. 15. 0.09 E-4 0.05 E-4 2309800400095 18. 16. 2309800400096 6. 12. 4.8 E-4 2309800400097 25. 27. 2309800400098 6. 13. 1.1 E-4 0.5 E-4 2309800400099 24. 26. 2309800400100 6. 14. 23.3 E-4 1.6 E-4 23.3 2309800400101 0.7 27.7 2.2 2309800400102 6. 15. 7.7 E-4 1.1 E-4 22.4 2309800400103 1.0 24.6 3.0 2309800400104 6. 16. 9.5 E-4 3.3 E-4 22.8 2309800400105 2.7 26. 9.5 2309800400106 6. 17. 0.65 E-4 0.21 E-4 2309800400107 22. 24. 2309800400108 6. 18. 0.32 E-4 0.11 E-4 2309800400109 21.5 22.9 2309800400110 6. 19. 0.030E-4 2309800400111 20. 21. 2309800400112 6. 20. 0.053E-4 2309800400113 19. 20. 2309800400114 7. 14. 4.1 E-4 2309800400115 26. 27. 2309800400116 7. 15. 0.17 E-4 0.07 E-4 2309800400117 25. 26. 2309800400118 7. 17. 0.77 E-4 0.31 E-4 2309800400119 22. 24. 2309800400120 7. 18. 0.47 E-4 0.21 E-4 2309800400121 22. 24.6 6.5 2309800400122 7. 19. 0.53 E-4 0.19 E-4 2309800400123 21. 22. 2309800400124 7. 20. 0.061E-4 2309800400125 20. 21. 2309800400126 7. 21. 0.024E-4 2309800400127 19. 20. 2309800400128 8. 16. 47. E-4 2309800400129 28. 28. 2309800400130 8. 17. 0.2 E-4 2309800400131 27. 27. 2309800400132 8. 18. 1.0 E-4 0.4 E-4 2309800400133 26. 26. 2309800400134 8. 19. 0.77 E-4 0.47 E-4 21.3 2309800400135 4.9 24. 14.3 2309800400136 8. 20. 2.7 E-4 0.4 E-4 23.5 2309800400137 1.3 22.1 3.8 2309800400138 8. 21. 0.71 E-4 0.24 E-4 20.6 2309800400139 4.3 24.8 5.6 2309800400140 8. 22. 0.39 E-4 0.18 E-4 2309800400141 22. 23. 2309800400142 9. 20. 0.08 E-4 2309800400143 32. 28. 2309800400144 ENDDATA 96 0 2309800400145 ENDSUBENT 144 0 2309800499999 SUBENT 23098005 20130203 22342309800500001 BIB 6 28 2309800500002 REACTION 1((96-CM-245(N,F)MASS,CHN,FY,,MXW)/ 2309800500003 (96-CM-245(N,F)2-HE-4,TER,FY,,MXW)) 2309800500004 2(96-CM-245(N,F)MASS,,KE,,MXW) Emean . 2309800500005 SAMPLE Three Cm-245 targets: 2309800500006 first two prepared by 4RUSEPA as Cm oxide,beside Cm-2452309800500007 (98.8% of Cm fraction) mainly the non-fissile isotopes2309800500008 Cm-244 and Cm-246 and small traces of radioactive decay2309800500009 daughters Pu-241 and Am-241 are present; 2309800500010 third of 3mm diameter spot- by Mainz University 2309800500011 Chemistry Department from Cm-245 separated at 1USAORL. 2309800500012 Contribution of impurities was neglected. 2309800500013 Total mass Area Cover Thickness 2309800500014 microg cm**2 Angstrom microg/cm**2 2309800500015 13.3 1x0.4 2500 Ni 33. 2309800500016 10.4 1x0.4 2500 Ni 26. 2309800500017 4. 0.07 2500 Ni - 2309800500018 METHOD After having finished the measurement of ternary 2309800500019 particle yields with the second curium target, RED 2309800500020 magnet was removed and measurement was continued to 2309800500021 measure a binary reference mass at the straight beam 2309800500022 position. For mass 90 an integrated mass yield of 2309800500023 normalization used in tables 1.5.3 and 1.5.4 (i.e. per 2309800500024 10**4 He-4) was obtained. The mean ionic charge 2309800500025 at E = 104.6 MeV was q = 20.8+-0.1 and the width of the2309800500026 charge distribution qFWHM = 5.0+-0.2. 2309800500027 ERR-ANALYS (DATA-ERR) Not specified. 2309800500028 MISC-COL (MISC) Efwhm obtained by fitting. 2309800500029 STATUS (TABLE) Table 1.5.4 of T,KOESTER . 2309800500030 ENDBIB 28 0 2309800500031 NOCOMMON 0 0 2309800500032 DATA 7 1 2309800500033 MASS DATA 1DATA-ERR 1DATA 2DATA-ERR 2MISC 2309800500034 MISC-ERR 2309800500035 NO-DIM NO-DIM NO-DIM MEV MEV MEV 2309800500036 MEV 2309800500037 90. 45000. 5000. 103.6 0.6 20.4 2309800500038 1.8 2309800500039 ENDDATA 6 0 2309800500040 ENDSUBENT 39 0 2309800599999 SUBENT 23098006 20100112 22212309800600001 BIB 9 25 2309800600002 REACTION 1((92-U-233(N,F)ELEM/MASS,TER,FY,,MXW)/ 2309800600003 (92-U-233(N,F)2-HE-4,TER,FY,,MXW)) 2309800600004 2(92-U-233(N,F)ELEM/MASS,TER,KE,,MXW) 2309800600005 SAMPLE U-233 sample of total mass 1329 microg, thickness 2309800600006 380 microg/cm**2, covered by 2500 Angstrom nickel foil.2309800600007 Provided by IRMM, Geel. 2309800600008 METHOD He-4 could only be measured up to max.energy 11.6 MeV.2309800600009 ANALYSIS All yields were normalized to Be-10 yield of 43 per 2309800600010 10000 LRA (REL-REF of A.Vorobiev et al.) 2309800600011 REL-REF (R,,A.Vorobiev+,J,PL/B,30,332,1969) 2309800600012 (D,,A.Vorobiev+,J,PL/B,30,332,1969) 2309800600013 Energy distributions of this measurement are shifted 2309800600014 towards to lower energies by about 0.5 to 1. MeV. 2309800600015 (A,,M.Woestheinrich+,S,AIP-447,330,1998) 2309800600016 Are consistent excluding mean kinetic energy of 17.2 2309800600017 MeV for Be-10, thus confirming the result of 2309800600018 A.Vorobiev+ - 17.0 MeV. 2309800600019 MISC-COL (MISC1) Emean, taken from systematics, fixed. 2309800600020 (MISC2) Efwhm obtained by fitting. 2309800600021 (MISC3) Efwhm from systematics, fixed. 2309800600022 FLAG (1.) DATA 1 , DATA 2, MISC2 are questionable. 2309800600023 (2.) MISC2 is questionable. 2309800600024 (3.) DATA 1 are questionable. 2309800600025 ERR-ANALYS (DATA-ERR) Not specified. 2309800600026 STATUS (TABLE) Tables 1.5.6, A.5.2 of T,KOESTER. 2309800600027 ENDBIB 25 0 2309800600028 NOCOMMON 0 0 2309800600029 DATA 12 15 2309800600030 ELEMENT MASS DATA 1DATA-ERR 1DATA-MAX 1DATA 22309800600031 DATA-ERR 2MISC1 MISC2 MISC2-ERR MISC3 FLAG 2309800600032 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM MEV 2309800600033 MEV MEV MEV MEV MEV NO-DIM 2309800600034 2. 3. 0.018 E-4 2309800600035 20. 10. 2309800600036 2. 4. 1. 2309800600037 2309800600038 2. 6. 179. E-4 15. E-4 10.3 2309800600039 0.3 10.3 0.6 3. 2309800600040 3. 9. 4.3 E-4 0.6 E-4 11.2 2309800600041 0.7 13.2 2.0 2309800600042 3. 11. 0.00037E-4 0.00027E-4 2309800600043 11. 11. 2309800600044 4. 10. 43. E-4 3. E-4 16.5 2309800600045 0.5 14.9 0.8 1. 2309800600046 4. 11. 1.9 E-4 1.0 E-4 2309800600047 15. 15. 2309800600048 4. 14. 0.0011 E-4 2309800600049 12. 12. 2309800600050 5. 14. 0.021 E-4 0.007 E-4 2309800600051 18.2 18.7 2309800600052 6. 15. 2.2 E-4 0.3 E-4 21.6 2309800600053 0.8 16.7 1.3 2. 2309800600054 8. 15. 0.013 E-4 2309800600055 30. 18. 2309800600056 8. 20. 0.73 E-4 0.09 E-4 22.8 2309800600057 1.5 21.6 2.1 2. 2309800600058 8. 21. 0.031 E-4 0.008 E-4 2309800600059 22. 21. 2309800600060 8. 22. 0.0052 E-4 0.0024 E-4 2309800600061 21. 20. 2309800600062 9. 21. 0.0077 E-4 0.0034 E-4 26.1 2309800600063 2.2 12.5 4.4 2309800600064 ENDDATA 34 0 2309800600065 ENDSUBENT 64 0 2309800699999 SUBENT 23098007 20100112 22212309800700001 BIB 7 21 2309800700002 REACTION 1((92-U-235(N,F)ELEM/MASS,TER,FY,,MXW)/ 2309800700003 (92-U-235(N,F)2-HE-4,TER,FY,,MXW)) 2309800700004 2(92-U-235(N,F)ELEM/MASS,TER,KE,,MXW) 2309800700005 SAMPLE Two U-235 targets : 2309800700006 Total mass Area Cover Thickness 2309800700007 microg cm**2 Angstrom microg/cm**2 2309800700008 1614 7x0.5 100 Ta 461. 2309800700009 1130 7x0.5 2500 Ni 323. 2309800700010 Contaminations with other fissile isotopes are 2309800700011 negligible, <0.1% . 2309800700012 Provided by IRMM, Geel. 2309800700013 METHOD Due to instabilities of the condenser high voltage 2309800700014 only few reliable points could be taken at high 2309800700015 voltages. This affects mainly the He isotopes, causing 2309800700016 large uncertainties in yields and energy distributions.2309800700017 ANALYSIS He isotopes were not evaluated and 2309800700018 yields were normalized to Be-10 yield of W.Baum (see 2309800700019 REL-REF) of 27.6 per 10000 LRA. 2309800700020 REL-REF (R,,W.Baum,T,BAUM,1992) Ph.D. thesis, TH Darmstadt. 2309800700021 ERR-ANALYS (DATA-ERR) Not specified. 2309800700022 STATUS (TABLE) Tables 1.5.7, A.5.4, A.5.5 of T,KOESTER. 2309800700023 ENDBIB 21 0 2309800700024 NOCOMMON 0 0 2309800700025 DATA 11 15 2309800700026 ELEMENT MASS DATA 1DATA-ERR 1DATA-MAX 1DATA 22309800700027 DATA-ERR 2MISC1 MISC2 MISC2-ERR MISC3 2309800700028 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM MEV 2309800700029 MEV MEV MEV MEV MEV 2309800700030 2. 3. 0.008 E-4 2309800700031 20. 10. 2309800700032 2. 4. 1. 2309800700033 2309800700034 3. 6. 0.015 E-4 2309800700035 20. 10. 2309800700036 3. 9. 2.9 E-4 0.3 E-4 11.8 2309800700037 0.5 13.2 1.5 2309800700038 3. 11. 0.00090E-4 0.00022E-4 9.6 2309800700039 1.1 7.9 2.1 2309800700040 4. 7. 0.009 E-4 2309800700041 28. 14. 2309800700042 4. 10. 27.6 E-4 2.0 16.8 2309800700043 0.5 16.5 0.8 2309800700044 4. 14. 0.00034E-4 0.00020E-4 2309800700045 13. 13. 2309800700046 5. 10. 0.008 E-4 2309800700047 25. 20. 2309800700048 5. 17. 0.0004 E-4 2309800700049 15. 15. 2309800700050 6. 15. 1.5 E-4 0.5 E-4 22.3 2309800700051 2.5 22.0 7.7 2309800700052 8. 15. 0.016 E-4 2309800700053 30. 18. 2309800700054 8. 20. 0.45 E-4 0.08 E-4 22.5 2309800700055 2.4 22.2 2.9 2309800700056 8. 21. 0.053 E-4 0.015 E-4 2309800700057 21. 21. 2309800700058 8. 22. 0.017 E-4 0.006 E-4 2309800700059 20. 20. 2309800700060 ENDDATA 34 0 2309800700061 ENDSUBENT 60 0 2309800799999 SUBENT 23098008 20100112 22212309800800001 BIB 3 6 2309800800002 REACTION ((92-U-233(N,F)ELEM/MASS,TER,FY,,MXW)// 2309800800003 (92-U-233(N,F)ELEM/MASS,TER,FY,,MXW)) 2309800800004 Yield ratios of halo nuclei and well-bound isotopes. 2309800800005 ERR-ANALYS (DATA-ERR) Not specified. 2309800800006 STATUS (TABLE) Tables 1.6.4, 1.6.5 of T,KOESTER. 2309800800007 (DEP,23098006) 2309800800008 ENDBIB 6 0 2309800800009 NOCOMMON 0 0 2309800800010 DATA 7 10 2309800800011 ELEM-NM MASS-NM ELEM-DN MASS-DN DATA DATA-ERR 2309800800012 DATA-MIN 2309800800013 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 2309800800014 NO-DIM 2309800800015 2. 4. 2. 6. 73. 4. 2309800800016 2309800800017 2. 6. 2. 8. 38. 5. 2309800800018 2309800800019 3. 7. 3. 9. 1.0 0.2 2309800800020 2309800800021 3. 9. 3. 11. 11500. 9000. 2309800800022 2309800800023 4. 9. 4. 11. 1.9 1.1 2309800800024 2309800800025 4. 10. 4. 12. 39. 8. 2309800800026 2309800800027 4. 12. 4. 14. 2309800800028 840. 2309800800029 6. 14. 6. 16. 6.0 1.0 2309800800030 2309800800031 6. 16. 6. 18. 40. 11. 2309800800032 2309800800033 8. 20. 8. 22. 140. 70. 2309800800034 2309800800035 ENDDATA 24 0 2309800800036 ENDSUBENT 35 0 2309800899999 SUBENT 23098009 20100112 22212309800900001 BIB 3 6 2309800900002 REACTION ((92-U-235(N,F)ELEM/MASS,TER,FY,,MXW)// 2309800900003 (92-U-235(N,F)ELEM/MASS,TER,FY,,MXW)) 2309800900004 Yield ratios of halo nuclei and well-bound isotopes. 2309800900005 ERR-ANALYS (DATA-ERR) Not specified. 2309800900006 STATUS (TABLE) Tables 1.6.4, 1.6.5 of T,KOESTER. 2309800900007 (DEP,23098007) 2309800900008 ENDBIB 6 0 2309800900009 NOCOMMON 0 0 2309800900010 DATA 6 12 2309800900011 ELEM-NM MASS-NM ELEM-DN MASS-DN DATA DATA-ERR 2309800900012 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 2309800900013 2. 4. 2. 6. 52. 3. 2309800900014 2. 6. 2. 8. 23. 3. 2309800900015 3. 7. 3. 9. 1.1 0.1 2309800900016 3. 9. 3. 11. 3300. 900. 2309800900017 4. 9. 4. 11. 1.2 0.3 2309800900018 4. 10. 4. 12. 23. 2. 2309800900019 4. 12. 4. 14. 3600. 2200. 2309800900020 6. 14. 6. 16. 6.1 0.9 2309800900021 6. 15. 6. 17. 8.3 1.2 2309800900022 6. 16. 6. 18. 25. 7. 2309800900023 6. 18. 6. 20. 9. 4. 2309800900024 8. 20. 8. 22. 26. 11. 2309800900025 ENDDATA 14 0 2309800900026 ENDSUBENT 25 0 2309800999999 SUBENT 23098010 20100112 22212309801000001 BIB 4 9 2309801000002 REACTION ((94-PU-239(N,F)ELEM/MASS,TER,FY,,MXW)// 2309801000003 (94-PU-239(N,F)ELEM/MASS,TER,FY,,MXW)) 2309801000004 Yield ratios of halo nuclei and well-bound isotopes. 2309801000005 COMMENT Of compiler. In text of thesis, it is mentioned that 2309801000006 data of ratios are from this experiment, but yields are2309801000007 not given. Probably, these ratios were estimated using 2309801000008 data of other experiments. 2309801000009 ERR-ANALYS (DATA-ERR) Not specified. 2309801000010 STATUS (TABLE) Tables 1.6.4, 1.6.5 of T,KOESTER. 2309801000011 ENDBIB 9 0 2309801000012 NOCOMMON 0 0 2309801000013 DATA 6 7 2309801000014 ELEM-NM MASS-NM ELEM-DN MASS-DN DATA DATA-ERR 2309801000015 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 2309801000016 2. 4. 2. 6. 52. 3. 2309801000017 2. 6. 2. 8. 22. 2. 2309801000018 3. 7. 3. 9. 1.2 0.1 2309801000019 3. 9. 3. 11. 3100. 1200. 2309801000020 4. 9. 4. 11. 1.5 0.3 2309801000021 4. 10. 4. 12. 22. 6. 2309801000022 4. 12. 4. 14. 5600. 3700. 2309801000023 ENDDATA 9 0 2309801000024 ENDSUBENT 23 0 2309801099999 SUBENT 23098011 20100112 22212309801100001 BIB 3 6 2309801100002 REACTION ((94-PU-241(N,F)ELEM/MASS,TER,FY,,MXW)// 2309801100003 (94-PU-241(N,F)ELEM/MASS,TER,FY,,MXW)) 2309801100004 Yield ratios of halo nuclei and well-bound isotopes. 2309801100005 ERR-ANALYS (DATA-ERR) Not specified. 2309801100006 STATUS (TABLE) Tables 1.6.4, 1.6.5 of T,KOESTER. 2309801100007 (DEP,23098002) 2309801100008 ENDBIB 6 0 2309801100009 NOCOMMON 0 0 2309801100010 DATA 6 13 2309801100011 ELEM-NM MASS-NM ELEM-DN MASS-DN DATA DATA-ERR 2309801100012 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 2309801100013 2. 4. 2. 6. 38. 4. 2309801100014 2. 6. 2. 8. 17. 3. 2309801100015 3. 7. 3. 9. 0.81 0.11 2309801100016 3. 9. 3. 11. 1800. 700. 2309801100017 4. 9. 4. 11. 0.75 0.23 2309801100018 4. 10. 4. 12. 16. 3. 2309801100019 4. 12. 4. 14. 1000. 400. 2309801100020 6. 14. 6. 16. 2.5 0.5 2309801100021 6. 15. 6. 17. 6.7 1.7 2309801100022 6. 16. 6. 18. 18. 5. 2309801100023 6. 17. 6. 19. 260. 160. 2309801100024 6. 18. 6. 20. 78. 63. 2309801100025 8. 20. 8. 22. 9.2 3.2 2309801100026 ENDDATA 15 0 2309801100027 ENDSUBENT 26 0 2309801199999 SUBENT 23098012 20100112 22212309801200001 BIB 3 6 2309801200002 REACTION ((96-CM-245(N,F)ELEM/MASS,TER,FY,,MXW)// 2309801200003 (96-CM-245(N,F)ELEM/MASS,TER,FY,,MXW)) 2309801200004 Yield ratios of halo nuclei and well-bound isotopes. 2309801200005 ERR-ANALYS (DATA-ERR) Not specified. 2309801200006 STATUS (TABLE) Tables 1.6.4, 1.6.5 of T,KOESTER. 2309801200007 (DEP,23098004) 2309801200008 ENDBIB 6 0 2309801200009 NOCOMMON 0 0 2309801200010 DATA 7 13 2309801200011 ELEM-NM MASS-NM ELEM-DN MASS-DN DATA DATA-ERR 2309801200012 DATA-MIN 2309801200013 NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM NO-DIM 2309801200014 NO-DIM 2309801200015 2. 4. 2. 6. 35. 3. 2309801200016 2309801200017 2. 6. 2. 8. 15. 3. 2309801200018 2309801200019 3. 7. 3. 9. 1.0 0.2 2309801200020 2309801200021 3. 9. 3. 11. 1400. 900. 2309801200022 2309801200023 4. 9. 4. 11. 1.1 0.2 2309801200024 2309801200025 4. 10. 4. 12. 12. 2. 2309801200026 2309801200027 4. 12. 4. 14. 310. 210. 2309801200028 2309801200029 6. 14. 6. 16. 2.5 0.9 2309801200030 2309801200031 6. 15. 6. 17. 12. 5. 2309801200032 2309801200033 6. 16. 6. 18. 30. 15. 2309801200034 2309801200035 6. 17. 6. 19. 2309801200036 15. 2309801200037 6. 18. 6. 20. 2309801200038 4. 2309801200039 8. 20. 8. 22. 7.0 3.5 2309801200040 2309801200041 ENDDATA 30 0 2309801200042 ENDSUBENT 41 0 2309801299999 ENDENTRY 12 0 2309899999999