ENTRY 23141 20170825 22652314100000001 SUBENT 23141001 20170825 22652314100100001 BIB 15 113 2314100100002 TITLE Neutron-capture cross-sections of 244Cm and 246Cm 2314100100003 measured with an array of large germanium detectors in 2314100100004 the ANNRI at J-PARC/MLF. 2314100100005 AUTHOR (A.Kimura,S.Goko,H.Harada,M.Oshima,M.Ohta,K.Furutaka, 2314100100006 T.Kin,F.Kitatani,M.Koizumi,S.Nakamura,Y.Toh,M.Igashira,2314100100007 T.Katabuchi,M.Mizumoto,Y.Kiyanagi,K.Kino,M.Furusaka, 2314100100008 F.Hiraga,T.Kamiyama,J.Hori,T.Fujii,S.Fukutani, 2314100100009 K.Takamiya,Y.Hara,K.Hirose,M.Oshima) 2314100100010 INSTITUTE (2JPNJAE) S.Goko,A.Kimura,H.Harada,M.Oshima,M.Ohta, 2314100100011 K.Furutaka,T.Kin,F.Kitatani,M.Koizumi,S.Nakamura,Y.Toh.2314100100012 (2JPNTIT) M.Igashira,T.Katabuchi,M.Mizumoto,Y.Hara, 2314100100013 K.Hirose,M.Oshima. 2314100100014 (2JPNHOK) Hokkaido University, Kita 13, Nishi 8, 2314100100015 Kita-ku, Sapporo, 060-8628, Japan. 2314100100016 Y.Kiyanagi,K.Kino,M.Furusaka,F.Hiraga,T.Kamiyama, 2314100100017 S.Goko. 2314100100018 (2JPNKTO) J.Hori,T.Fujii,S.Fukutani,K.Takamiya,M.Ohta. 2314100100019 (2JPNKEK) K.Kino. 2314100100020 REFERENCE (J,NST,49,(7),708,2012) First author A.Kimura. 2314100100021 #doi:10.1080/00223131.2012.693887 2314100100022 (W,KIMURA,20121023) e-mails from Atsushi Kimura. 2314100100023 (J,NST,47,(12),1097,2010) First author S.Goko 2314100100024 #doi:10.3327/jnst.47.1097 2314100100025 (J,KPS,59,(2),1828,2011) First author A.Kimura. 2314100100026 #doi:10.3938/jkps.59.1828 2314100100027 ND2010 Conf. Proc. 2314100100028 REL-REF (I,,K.Kino+,J,NIM/A,626-627,58,2011) 2314100100029 Measurement of energy spectra and spatial distributions2314100100030 of neutron beams provided by the ANNRI beam-line for 2314100100031 capture cross-section measurements at the J-PARC/MLF, 2314100100032 FACILITY (SYNCH,2JPNJAE) The neutron-nucleus reaction instrument2314100100033 (NNRI) at the J-PARC MLF Beam Line No. 4 (BL04). 2314100100034 Accelerator was operated in double-bunch mode at a 2314100100035 beam power of 120 kW and a repetition rate of 25 Hz. 2314100100036 Disk chopper with a semicircular shape was used to 2314100100037 prevent the intrusion of the low-energy tail of neutron2314100100038 pulse into the next pulse duration. 2314100100039 METHOD (TOF) Flight length 21.502+-0.005 m. 2314100100040 Disk chopper with semicircular shape was installed at 2314100100041 flight length of 14 m to exclude the effect from 2314100100042 overlapping neutrons. 2314100100043 Data were measured with event-by-event mode storing the2314100100044 information of gamma-ray pulse height (PHA), TOF and 2314100100045 time-interval between coincidence signals. 2314100100046 Time resolution of DAQ system is 10 ns. 2314100100047 INC-SOURCE (SPALL) Pulsed neutron beam was collimated to diameter 2314100100048 of 7 mm at the sample position. Proton energy 3 GeV, 2314100100049 average beam power 120 kW, repetition rate 25 Hz. 2314100100050 Proton intensity of shots was stable within 1% in FWHM.2314100100051 Primary neutron production target - mercury. 2314100100052 Time resolution of proton beam 600ns (The proton beams 2314100100053 were supplied in the "double-bunch mode," each bunch 2314100100054 with a width of 100 ns, at intervals of 600 ns). 2314100100055 Para H as moderator of 1400 mm diameter, 120 mm height.2314100100056 DETECTOR (D4PI,GE,BGO) 4PI Ge spectrometer: two cluster-Ge 2314100100057 detectors and eight coaxial Ge detectors surrounded by 2314100100058 BGO anti-Compton shields. Set at a position 21.5m from 2314100100059 the neutron source. To detect the prompt gamma-rays. 2314100100060 In the present measurement only two cluster Ge 2314100100061 detectors (each of 7 Ge crystals) were used. 2314100100062 To suppress the gamma-flash effect to the detector, 2314100100063 Pb filter of 37.5 mm thickness was inserted into the 2314100100064 flight path. 2314100100065 The sample was set in Al beam duct. To decrease 2314100100066 background scattering from N-14 and O-16, the duct was 2314100100067 filled with He gas. Lithium hydride powder in Al 2314100100068 containers, sheets of boron and rubber mixture, lead 2314100100069 plates of 3 mm thickness were set between the beam duct2314100100070 and the cluster Ge detectors to protect scattered 2314100100071 neutrons and decay gamma-rays from the high-activity 2314100100072 Cm-244 sample. The detectors were covered with 2314100100073 radiation shield of lead, iron, and boron resin. 2314100100074 Gamma-ray signals from the 14 Ge crystals in the 2314100100075 cluster Ge detectors were acquired using an original 2314100100076 data acquisition (DAQ) system based on a digital data 2314100100077 processing technique. 2314100100078 Random pulse generator (Berkeley Nucleonics, DB-2) was 2314100100079 used to estimate the dead time of detectors. 2314100100080 The total efficiency of the 4PI Ge spectrometer for the2314100100081 entire energy region was less than 12%, as calculated 2314100100082 using standard gamma-ray sources (Cs-137, Co-60) and 2314100100083 the EGS5 Monte Carlo simulation code. 2314100100084 PART-DET (G) Prompt gamma-rays. 2314100100085 ANALYSIS The neutron energy was calibrated by measuring a Au 2314100100086 sample with well-known neutron resonances. 2314100100087 Detection efficiency of capture gamma-rays for each 2314100100088 resonance was assumed to be constant. 2314100100089 The relative yields were normalized at the first 2314100100090 resonance of 240Pu to the weighted evaluated values in 2314100100091 JENDL-4.0 by the abundance of 240Pu 2314100100092 CORRECTION For dead time - correction factor was obtained by using2314100100093 the random pulse generator. Dead time typically 5musec.2314100100094 For background due to overlapping neutron and decay 2314100100095 gamma rays and for neutron energy dependent background.2314100100096 For self-shielding and multiple-scattering effects by 2314100100097 the Monte Carlo simulation code MCNP. 2314100100098 For influence of fission events. 2314100100099 MONITOR (5-B-10(N,A)3-LI-7,PAR,SIG,G) 2314100100100 Energy dependence of neutron flux was estimated from 2314100100101 the TOF spectrum gated at the 478 keV gamma-ray peak 2314100100102 emitted from the 10B(n,alpha gamma)7Li reaction. 2314100100103 MONIT-REF (,,3,JENDL-4.0,,2012) 2314100100104 HISTORY (20110805C) M.M. 2314100100105 (20120823A) M.M. Reference J,NST,49,708,2012 was added.2314100100106 BIB information was updated. 2314100100107 Subents 005-017 were added. 2314100100108 Request for the data of neutron capture cross sections2314100100109 for Cm-244, Cm246 was sent to Atsushi Kimura 11.10.20122314100100110 kimura.atsushi04@jaea.go.jp . 2314100100111 (20121023R) Data for Subents 003,004 were received from2314100100112 author Atsushi Kimura. 2314100100113 Authors' data were added in Subents 003,004. 2314100100114 (20170825U) SD: Small correction in Subent 002. 2314100100115 ENDBIB 113 0 2314100100116 COMMON 1 3 2314100100117 E-NRM 2314100100118 KEV 2314100100119 478. 2314100100120 ENDCOMMON 3 0 2314100100121 ENDSUBENT 120 0 2314100199999 SUBENT 23141002 20170825 22652314100200001 BIB 8 50 2314100200002 REACTION ((96-CM-244(N,G)96-CM-245,,SIG,,RES)// 2314100200003 (96-CM-244(N,G)96-CM-245,,SIG,,RES)) 2314100200004 SAMPLE Cm-244 sample was composed of curium oxide powder 2314100200005 CmO2; weight 0.6 mg; activity 1.8 GBq and Al powder 2314100200006 (weight 25 mg) for dilution. The isotopic ratio of the2314100200007 Cm sample measured by the Kyoto University Research 2314100200008 Reactor Institute (KURRI): 2314100200009 Isotope Spec. sheet KURRI 2314100200010 Cm-243 0.02 - 2314100200011 Cm-244 82.42 89.57 +- 1.68 2314100200012 Cm-245 2.19 2.66 +- 0.34 2314100200013 Cm-246 5.86 7.08 +- 0.33 2314100200014 Cm-247 0.15 - 2314100200015 Cm-248 0.11 - 2314100200016 Sample was contained in Al case with an inner diameter 2314100200017 of 5mm and inner depth of 0.5 mm. The outer diameter of2314100200018 the Al case is 9mm and the thickness is 1.2 mm. 2314100200019 Cm sample was irradiated with neutron pulses of 2.6E+6 2314100200020 shots for 33 h. 2314100200021 INC-SPECT Background level of neutrons was negligible. 2314100200022 The obtained neutron flux is shown in Fig.2 of 2314100200023 J,NST,47,(12),1097,2010. 2314100200024 Energy-integrated neutron intensities at sample 2314100200025 position are 4.5E+6 n/s/cm**2 in neutron energy range 2314100200026 1.5-25 meV, 6.6E+5 n/s/cm**2 in 0.9-1.1 keV. 2314100200027 The incident neutron flux shape was measured with 2314100200028 sintered natural boron sample (8.67 mg). 2314100200029 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314100200030 3.64+-0.11 % for 1.33-MeV gamma- rays. 2314100200031 Typical resolution is 9.8 keV (on beam) and 2.4 keV 2314100200032 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314100200033 ERR-ANALYS (ERR-S) Statistical error. 2314100200034 (ERR-1) Uncertainty due to the difference in the energy2314100200035 distribution of capture gamma-rays for each neutron 2314100200036 resonance, which contributes to the detection 2314100200037 efficiency. 2314100200038 (ERR-2) Uncertainty due to dead-time correction. 2314100200039 (ERR-3) Uncertainty due to multiplicity for the capture2314100200040 gamma-rays. 2314100200041 (ERR-SYS) Total systematical uncertainty. 2314100200042 ADD-RES (COMP) Comparison with JENDL-3.3 data. 2314100200043 Ratios for En 85.96 and 96.12 eV are different from the2314100200044 evaluated values. In the former case, two resonances of2314100200045 85.96 (Cm-244C; foreground) and 84.62 eV (Cm-246; 2314100200046 background) overlap in the TOF spectrum; these two 2314100200047 resonance peaks are difficult to separate.In the latter2314100200048 case, 98.85 eV (248Cm; background) overlaps with the 2314100200049 foreground. 2314100200050 STATUS (TABLE) Table 2 of J,NST,47,(12),1097,2010. 2314100200051 HISTORY (20170825U) SD: Syntax correction in BIB. 2314100200052 ENDBIB 50 0 2314100200053 COMMON 5 3 2314100200054 EN-RES-DN ERR-1 ERR-2 ERR-3 ERR-SYS 2314100200055 EV PER-CENT PER-CENT PER-CENT PER-CENT 2314100200056 7.67 5. 3. 1.5 6. 2314100200057 ENDCOMMON 3 0 2314100200058 DATA 3 7 2314100200059 EN-RES-NM DATA ERR-S 2314100200060 EV NO-DIM NO-DIM 2314100200061 7.67 1.0 2314100200062 16.77 0.1191 0.0020 2314100200063 22.85 0.0352 0.0017 2314100200064 34.99 0.1142 0.0034 2314100200065 85.96 0.1047 0.0052 2314100200066 96.12 0.0960 0.0089 2314100200067 132.8 0.0747 0.0084 2314100200068 ENDDATA 9 0 2314100200069 ENDSUBENT 68 0 2314100299999 SUBENT 23141003 20120823 22332314100300001 BIB 7 63 2314100300002 REACTION (96-CM-244(N,G)96-CM-245,,SIG) 2314100300003 SAMPLE Cm-244 sample was 0.6 mg of curium oxide. 2314100300004 Isotopic enrichment was 90.1 mole%, main activity was 2314100300005 1.8 GBq. Sample was sealed in an Al case of 9 mm outer 2314100300006 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314100300007 Sample was put in a bag of fluorinated ethylene 2314100300008 propylene (FEP) films and attached to a sample holder 2314100300009 made of polytetrafluoroethylene and shaped into 2314100300010 50mmx70 mm rectangular frame. 2314100300011 The isotopic abundances were determined by thermal 2314100300012 ionization mass spectrometry - TIMS (mole%) : 2314100300013 Cm-244 - 90.1 +- 1.7 , Cm-245 - 2.71 +- 0.34, 2314100300014 Cm-246 - 7.22 +- 0.34, Cm-247 - not detected, 2314100300015 Cm-248 - not detected. 2314100300016 The isotopic abundances were determined by alpha-ray 2314100300017 spectrometry(normalized to results of 244Cm with TIMS):2314100300018 Cm-244 - 90.1, Cm-245 - not detected, 2314100300019 Cm-246 - 7.0 +- 0.6, Cm-247 - not detected, 2314100300020 Cm-248 - not detected, Pu-240 - 13.6 +- 0.6 . 2314100300021 Cm sample was irradiated 64 h. 2314100300022 Am-243 abundance was obtained by fitting of normalized 2314100300023 yields at first resonance with code SAMMY-7 and was 2314100300024 defined to be (0.63+-0.04) % . 2314100300025 INC-SPECT The energy integrated neutron intensities at the sample2314100300026 position are 5.2E+10 n/s/m2 in the neutron energy 2314100300027 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314100300028 under a proton beam power of 120 kW. 2314100300029 ANALYSIS The contributions from 244Cm were calculated by 2314100300030 subtracting the contributions from the impurities from 2314100300031 the capture yields. 2314100300032 Contributions from impurities of 240Pu, 243Am, 246Cm 2314100300033 (without 244Cm) were calculated with SAMMY using the 2314100300034 parameters of these work and JENDL-4.0. 2314100300035 Neutron-capture cross sections of 244Cm were obtained 2314100300036 by dividing the 244Cm contributions by the isotopic 2314100300037 ratio. 2314100300038 ERR-ANALYS (ERR-T,,,P) Total uncertainty. 2314100300039 (ERR-S,,,U) Statistical Error. 2314100300040 (ERR-1,,,F) Systematic Error in the normalization. 2314100300041 (ERR-2,,,U) Error in the contribution of capture events2314100300042 of the other nuclei. 2314100300043 (ERR-3,,,U) Error in the contribution of fission events2314100300044 (ERR-4,,,U) Error in the corrections of self-shielding 2314100300045 and multiple scattering. 2314100300046 (ERR-5,,,P) Other uncertainties (neutron flux, 2314100300047 contaminations of scattered events, deadtime 2314100300048 correction. 2314100300049 Non-neutron-energy-dependent errors are: 2314100300050 SAMMY fitting error 0.6 %. 2314100300051 Errors in the abundances of 240Pu 4.4 %. 2314100300052 Errors in the evaluated value of JENDL-4.0 of 2314100300053 the first resonance of 240Pu 2.2 %. 2314100300054 Systematic errors in influences of the 2314100300055 scattered neutrons 0.3 0.3 2314100300056 Error in the abundances of 240Pu and error in the 2314100300057 isotopic ratio of 244Cm to 246Cm" are not independent; 2314100300058 both errors include error in the isotopic ratio of 2314100300059 244Cm (comment of author Atsushi Kimura ). 2314100300060 MISC-COL (MISC) ERR-1 in absolute units. 2314100300061 STATUS (TABLE) Data were received from author Atsushi Kimura 2314100300062 23.10.2012 . 2314100300063 Data are on Fig. 22 of J,NST,49,(7),708,2012 . 2314100300064 Preliminary data on Fig. 6a of J,KPS,59,(2),1828,2011. 2314100300065 ENDBIB 63 0 2314100300066 COMMON 1 3 2314100300067 ERR-1 2314100300068 PER-CENT 2314100300069 5.5 2314100300070 ENDCOMMON 3 0 2314100300071 DATA 9 1009 2314100300072 EN DATA ERR-T ERR-S MISC ERR-2 2314100300073 ERR-3 ERR-4 ERR-5 2314100300074 EV B B B B B 2314100300075 B B B 2314100300076 2.0027E+00 1.03E+01 3.02E+01 2.48E+01 5.67E-01 6.55E-012314100300077 1.72E+01 4.89E-03 1.08E-01 2314100300078 2.0064E+00 3.97E+00 3.01E+01 2.49E+01 2.19E-01 6.49E-012314100300079 1.70E+01 6.88E-03 9.53E-02 2314100300080 2.0100E+00 1.26E+01 3.00E+01 2.48E+01 6.95E-01 6.44E-012314100300081 1.68E+01 1.06E-02 1.10E-01 2314100300082 2.0137E+00 8.31E+00 2.98E+01 2.48E+01 4.59E-01 6.38E-012314100300083 1.65E+01 1.10E-02 1.01E-01 2314100300084 2.0174E+00 1.02E+01 2.96E+01 2.47E+01 5.62E-01 6.32E-012314100300085 1.62E+01 1.23E-02 1.03E-01 2314100300086 2.0211E+00 2.72E+01 2.96E+01 2.48E+01 1.50E+00 6.27E-012314100300087 1.60E+01 1.91E-02 1.34E-01 2314100300088 2.0248E+00 1.85E+01 2.92E+01 2.46E+01 1.02E+00 6.22E-012314100300089 1.57E+01 2.32E-02 1.18E-01 2314100300090 2.0285E+00 -1.99E+01 2.92E+01 2.48E+01 1.10E+00 6.16E-012314100300091 1.54E+01 1.14E-02 4.53E-02 2314100300092 2.0322E+00 3.01E+01 2.89E+01 2.47E+01 1.66E+00 6.11E-012314100300093 1.50E+01 3.78E-02 1.39E-01 2314100300094 2.0359E+00 4.80E+01 2.88E+01 2.46E+01 2.65E+00 6.06E-012314100300095 1.47E+01 4.65E-02 1.73E-01 2314100300096 2.0397E+00 6.39E+01 2.87E+01 2.46E+01 3.53E+00 6.01E-012314100300097 1.44E+01 5.31E-02 2.00E-01 2314100300098 2.0434E+00 3.78E+01 2.85E+01 2.47E+01 2.09E+00 5.96E-012314100300099 1.40E+01 3.28E-02 1.47E-01 2314100300100 2.0472E+00 3.00E+01 2.83E+01 2.47E+01 1.66E+00 5.90E-012314100300101 1.37E+01 2.19E-02 1.29E-01 2314100300102 2.0510E+00 8.98E+01 2.84E+01 2.46E+01 4.96E+00 5.85E-012314100300103 1.34E+01 4.03E-02 2.36E-01 2314100300104 2.0548E+00 -2.74E+01 2.80E+01 2.47E+01 1.51E+00 5.80E-012314100300105 1.30E+01 5.80E-03 1.89E-02 2314100300106 2.0585E+00 1.00E+01 2.76E+01 2.45E+01 5.55E-01 5.76E-012314100300107 1.27E+01 3.83E-02 8.50E-02 2314100300108 2.0624E+00 6.39E+01 2.76E+01 2.45E+01 3.53E+00 5.71E-012314100300109 1.23E+01 9.07E-02 1.80E-01 2314100300110 2.0662E+00 -2.49E+01 2.74E+01 2.46E+01 1.38E+00 5.66E-012314100300111 1.20E+01 9.08E-03 1.82E-02 2314100300112 2.0700E+00 4.02E+01 2.73E+01 2.45E+01 2.22E+00 5.61E-012314100300113 1.17E+01 6.72E-02 1.33E-01 2314100300114 2.0738E+00 -9.28E+00 2.70E+01 2.45E+01 5.12E-01 5.56E-012314100300115 1.13E+01 2.54E-02 4.32E-02 2314100300116 2.0777E+00 3.05E+01 2.69E+01 2.44E+01 1.68E+00 5.52E-012314100300117 1.10E+01 7.77E-02 1.13E-01 2314100300118 2.0815E+00 3.02E+01 2.67E+01 2.44E+01 1.67E+00 5.47E-012314100300119 1.07E+01 7.82E-02 1.11E-01 2314100300120 2.0854E+00 4.16E+01 2.66E+01 2.43E+01 2.30E+00 5.42E-012314100300121 1.04E+01 7.77E-02 1.31E-01 2314100300122 2.0893E+00 5.99E+01 2.66E+01 2.44E+01 3.31E+00 5.38E-012314100300123 1.02E+01 8.02E-02 1.63E-01 2314100300124 2.0932E+00 -6.21E+00 2.64E+01 2.44E+01 3.43E-01 5.33E-012314100300125 9.87E+00 2.10E-02 4.21E-02 2314100300126 2.0971E+00 6.37E+00 2.62E+01 2.43E+01 3.52E-01 5.29E-012314100300127 9.60E+00 3.44E-02 6.36E-02 2314100300128 2.1010E+00 3.60E+01 2.62E+01 2.44E+01 1.99E+00 5.24E-012314100300129 9.35E+00 6.32E-02 1.16E-01 2314100300130 2.1049E+00 1.54E+01 2.60E+01 2.43E+01 8.51E-01 5.20E-012314100300131 9.09E+00 3.52E-02 7.71E-02 2314100300132 2.1088E+00 1.44E+01 2.59E+01 2.43E+01 7.94E-01 5.16E-012314100300133 8.85E+00 2.72E-02 7.39E-02 2314100300134 2.1128E+00 1.66E+01 2.57E+01 2.42E+01 9.14E-01 5.11E-012314100300135 8.62E+00 3.20E-02 7.64E-02 2314100300136 2.1167E+00 1.59E+01 2.56E+01 2.42E+01 8.79E-01 5.07E-012314100300137 8.40E+00 3.99E-02 7.38E-02 2314100300138 2.1207E+00 2.07E+01 2.55E+01 2.41E+01 1.14E+00 5.03E-012314100300139 8.19E+00 5.16E-02 8.08E-02 2314100300140 2.1247E+00 1.11E+01 2.55E+01 2.42E+01 6.10E-01 4.99E-012314100300141 7.99E+00 4.10E-02 6.23E-02 2314100300142 2.1287E+00 3.81E+01 2.55E+01 2.42E+01 2.10E+00 4.95E-012314100300143 7.79E+00 7.25E-02 1.09E-01 2314100300144 2.1327E+00 3.71E+01 2.54E+01 2.41E+01 2.05E+00 4.91E-012314100300145 7.61E+00 6.61E-02 1.08E-01 2314100300146 2.1367E+00 7.17E+01 2.55E+01 2.41E+01 3.96E+00 4.86E-012314100300147 7.43E+00 9.15E-02 1.70E-01 2314100300148 2.1407E+00 -1.63E+01 2.51E+01 2.40E+01 9.02E-01 4.83E-012314100300149 7.27E+00 5.76E-03 1.13E-02 2314100300150 2.1447E+00 3.20E+01 2.51E+01 2.40E+01 1.77E+00 4.79E-012314100300151 7.11E+00 6.42E-02 9.99E-02 2314100300152 2.1488E+00 1.75E+01 2.51E+01 2.41E+01 9.68E-01 4.75E-012314100300153 6.96E+00 5.69E-02 7.19E-02 2314100300154 2.1528E+00 9.45E+00 2.50E+01 2.41E+01 5.22E-01 4.71E-012314100300155 6.81E+00 4.26E-02 5.60E-02 2314100300156 2.1569E+00 3.36E+01 2.50E+01 2.41E+01 1.85E+00 4.67E-012314100300157 6.67E+00 6.33E-02 9.84E-02 2314100300158 2.1610E+00 2.58E+01 2.49E+01 2.40E+01 1.43E+00 4.63E-012314100300159 6.55E+00 4.44E-02 8.35E-02 2314100300160 2.1651E+00 3.77E-02 2.49E+01 2.41E+01 2.09E-03 4.59E-012314100300161 6.43E+00 1.63E-02 3.67E-02 2314100300162 2.1692E+00 2.69E+00 2.49E+01 2.41E+01 1.48E-01 4.55E-012314100300163 6.31E+00 1.51E-02 4.12E-02 2314100300164 2.1733E+00 4.02E+00 2.49E+01 2.41E+01 2.22E-01 4.52E-012314100300165 6.20E+00 1.84E-02 4.34E-02 2314100300166 2.1774E+00 5.31E+00 2.47E+01 2.39E+01 2.93E-01 4.48E-012314100300167 6.10E+00 2.40E-02 4.55E-02 2314100300168 2.1816E+00 2.09E+01 2.48E+01 2.40E+01 1.15E+00 4.44E-012314100300169 6.00E+00 4.28E-02 7.39E-02 2314100300170 2.1857E+00 -2.15E+01 2.47E+01 2.40E+01 1.19E+00 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3.60E-022314100301989 1.43E+00 3.12E-01 3.95E-02 2314100301990 1.2040E+02 -1.18E+01 1.78E+01 1.76E+01 6.50E-01 1.54E+002314100301991 1.40E+00 3.84E-02 9.31E-03 2314100301992 1.2212E+02 1.02E+01 2.06E+01 1.79E+01 5.64E-01 1.02E+012314100301993 1.37E+00 2.87E-02 9.50E-02 2314100301994 1.2387E+02 -1.09E+01 1.77E+01 1.76E+01 6.02E-01 2.63E-012314100301995 1.35E+00 3.70E-02 1.51E-02 2314100301996 1.2566E+02 3.03E+01 1.78E+01 1.76E+01 1.67E+00 2.19E-012314100301997 1.32E+00 3.02E-01 8.28E-02 2314100301998 1.2750E+02 -1.93E+01 1.74E+01 1.73E+01 1.06E+00 5.93E-022314100301999 1.30E+00 1.96E-01 3.67E-02 2314100302000 1.2937E+02 3.45E+01 1.73E+01 1.72E+01 1.90E+00 2.75E-012314100302001 1.27E+00 7.56E-01 9.24E-02 2314100302002 1.3128E+02 7.94E+01 1.93E+01 1.78E+01 4.38E+00 6.07E+002314100302003 1.27E+00 6.63E-01 2.35E-01 2314100302004 1.3324E+02 1.48E+02 2.05E+01 1.80E+01 8.18E+00 1.50E-012314100302005 5.46E+00 4.90E-01 3.91E-01 2314100302006 1.3524E+02 4.92E+01 2.21E+01 1.78E+01 2.72E+00 1.28E+012314100302007 1.20E+00 6.61E-01 2.01E-01 2314100302008 1.3729E+02 8.65E+01 1.76E+01 1.65E+01 4.77E+00 2.47E-012314100302009 1.18E+00 3.15E+00 2.15E-01 2314100302010 1.3938E+02 6.79E+01 1.79E+01 1.72E+01 3.75E+00 1.33E-012314100302011 2.73E+00 2.08E+00 1.83E-01 2314100302012 1.4152E+02 4.34E+01 1.55E+01 1.44E+01 2.40E+00 4.02E-022314100302013 1.13E+00 5.33E+00 1.12E-01 2314100302014 1.4371E+02 4.58E+01 1.54E+01 1.34E+01 2.53E+00 1.47E-012314100302015 1.11E+00 7.00E+00 1.18E-01 2314100302016 1.4595E+02 4.99E+01 1.58E+01 1.42E+01 2.75E+00 2.34E-012314100302017 1.09E+00 6.22E+00 1.28E-01 2314100302018 1.4825E+02 4.61E+01 1.62E+01 1.54E+01 2.54E+00 9.48E-022314100302019 1.06E+00 4.22E+00 1.18E-01 2314100302020 1.5060E+02 7.38E+01 1.77E+01 1.68E+01 4.07E+00 1.80E+002314100302021 1.04E+00 3.44E+00 1.94E-01 2314100302022 1.5300E+02 4.18E+01 1.80E+01 1.75E+01 2.31E+00 3.53E+002314100302023 1.03E+00 1.23E+00 1.29E-01 2314100302024 1.5546E+02 2.93E+01 1.79E+01 1.78E+01 1.62E+00 5.88E-022314100302025 9.99E-01 6.13E-01 7.75E-02 2314100302026 1.5799E+02 1.94E+01 1.93E+01 1.84E+01 1.07E+00 5.78E+002314100302027 1.01E+00 1.62E-01 8.93E-02 2314100302028 1.6057E+02 5.86E+01 1.84E+01 1.81E+01 3.24E+00 3.55E-012314100302029 9.57E-01 9.30E-01 1.50E-01 2314100302030 1.6322E+02 1.82E+01 1.89E+01 1.84E+01 1.01E+00 3.96E+002314100302031 9.36E-01 3.27E-01 7.40E-02 2314100302032 1.6594E+02 3.83E+01 1.81E+01 1.79E+01 2.12E+00 9.28E-022314100302033 9.16E-01 9.58E-01 9.89E-02 2314100302034 1.6872E+02 4.43E+01 1.85E+01 1.82E+01 2.45E+00 1.96E+002314100302035 8.98E-01 6.30E-01 1.25E-01 2314100302036 1.7158E+02 5.36E+01 1.91E+01 1.88E+01 2.96E+00 1.53E+002314100302037 1.37E+00 4.55E-01 1.49E-01 2314100302038 1.7451E+02 3.73E+01 1.81E+01 1.79E+01 2.06E+00 1.32E-012314100302039 8.58E-01 1.19E+00 9.65E-02 2314100302040 1.7751E+02 2.34E+01 1.81E+01 1.81E+01 1.29E+00 8.16E-022314100302041 8.40E-01 6.76E-01 6.27E-02 2314100302042 1.8059E+02 6.65E+01 1.96E+01 1.90E+01 3.67E+00 6.40E-022314100302043 3.33E+00 7.02E-01 1.83E-01 2314100302044 1.8375E+02 3.39E+01 1.84E+01 1.83E+01 1.87E+00 6.59E-012314100302045 8.18E-01 1.29E+00 9.19E-02 2314100302046 1.8700E+02 4.97E+01 1.87E+01 1.82E+01 2.75E+00 2.90E+002314100302047 7.85E-01 1.42E+00 1.43E-01 2314100302048 1.9033E+02 4.71E+01 1.85E+01 1.83E+01 2.60E+00 1.18E-012314100302049 7.67E-01 1.69E+00 1.20E-01 2314100302050 1.9376E+02 2.26E+01 1.89E+01 1.79E+01 1.25E+00 5.62E+002314100302051 7.57E-01 1.56E+00 9.45E-02 2314100302052 1.9727E+02 1.09E+02 2.07E+01 1.95E+01 6.04E+00 1.61E-012314100302053 3.33E+00 1.27E+00 2.87E-01 2314100302054 2.0089E+02 1.19E+01 1.78E+01 1.78E+01 6.58E-01 2.49E-012314100302055 7.24E-01 6.63E-01 3.60E-02 2314100302056 2.0460E+02 2.60E+01 1.74E+01 1.72E+01 1.44E+00 3.29E-022314100302057 7.17E-01 1.46E+00 6.84E-02 2314100302058 2.0842E+02 8.65E+01 1.94E+01 1.86E+01 4.78E+00 6.81E-022314100302059 1.71E+00 2.18E+00 2.22E-01 2314100302060 2.1234E+02 7.99E+01 1.86E+01 1.67E+01 4.41E+00 7.55E-022314100302061 7.23E-01 6.64E+00 1.99E-01 2314100302062 2.1638E+02 3.87E+01 1.74E+01 1.70E+01 2.14E+00 3.26E-022314100302063 7.13E-01 2.91E+00 9.95E-02 2314100302064 2.2053E+02 8.55E+01 2.02E+01 1.92E+01 4.72E+00 5.15E-022314100302065 3.46E+00 2.12E+00 2.31E-01 2314100302066 2.2480E+02 3.43E+01 1.66E+01 1.59E+01 1.89E+00 7.13E-022314100302067 7.02E-01 4.26E+00 8.92E-02 2314100302068 2.2920E+02 5.93E+01 1.89E+01 1.83E+01 3.28E+00 5.56E-022314100302069 1.14E+00 3.10E+00 1.54E-01 2314100302070 2.3373E+02 1.99E+01 1.76E+01 1.75E+01 1.10E+00 1.42E+002314100302071 8.53E-01 1.60E+00 6.49E-02 2314100302072 2.3840E+02 -2.38E+01 1.75E+01 1.73E+01 1.31E+00 2.25E+002314100302073 6.87E-01 1.28E+00 3.88E-02 2314100302074 2.4320E+02 4.00E+00 1.74E+01 1.74E+01 2.21E-01 6.99E-022314100302075 8.01E-01 5.50E-01 1.71E-02 2314100302076 2.4816E+02 -4.14E+01 1.73E+01 1.66E+01 2.29E+00 2.52E-012314100302077 6.79E-01 4.28E+00 9.43E-02 2314100302078 2.5326E+02 -2.89E+01 1.76E+01 1.74E+01 1.60E+00 2.45E-012314100302079 6.75E-01 2.01E+00 6.41E-02 2314100302080 2.5853E+02 -4.51E+01 1.98E+01 1.96E+01 2.49E+00 1.62E+002314100302081 6.72E-01 1.18E+00 9.58E-02 2314100302082 2.6396E+02 -2.44E+01 2.03E+01 2.03E+01 1.35E+00 2.53E-012314100302083 9.84E-01 3.36E-01 5.05E-02 2314100302084 2.6956E+02 -2.29E+01 2.04E+01 2.03E+01 1.26E+00 4.13E-032314100302085 6.65E-01 4.14E-01 5.12E-02 2314100302086 2.7535E+02 5.12E+00 2.06E+01 2.06E+01 2.83E-01 1.35E-012314100302087 9.25E-01 9.41E-02 3.02E-02 2314100302088 2.8132E+02 -9.10E+00 1.99E+01 1.99E+01 5.02E-01 1.47E-012314100302089 6.57E-01 2.72E-01 2.27E-02 2314100302090 2.8749E+02 -3.47E+01 2.19E+01 2.11E+01 1.92E+00 5.17E+002314100302091 6.63E-01 2.92E-01 5.42E-02 2314100302092 2.9386E+02 -4.31E+01 2.01E+01 1.98E+01 2.38E+00 3.68E-022314100302093 6.49E-01 2.41E+00 1.45E-01 2314100302094 ENDDATA 2022 0 2314100302095 ENDSUBENT 2094 0 2314100399999 SUBENT 23141004 20120823 22332314100400001 BIB 7 67 2314100400002 REACTION (96-CM-246(N,G)96-CM-247,,SIG) 2314100400003 SAMPLE Cm-246 sample was 2.1 mg of curium oxide. 2314100400004 Cm-246 Isotopic enrichment was 59.4 mole% with 27.5 2314100400005 mole% Cm-244, it's main activities were Cm246 12.1 MBq,2314100400006 Cm-244 1.7 GBq. 2314100400007 Sample was sealed in an Al case of 9 mm outer 2314100400008 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314100400009 Sample was put in a bag of fluorinated ethylene 2314100400010 propylene (FEP) films and attached to a sample holder 2314100400011 made of polytetrafluoroethylene and shaped into 2314100400012 50mmx70 mm rectangular frame. 2314100400013 The isotopic abundances were determined by thermal 2314100400014 ionization mass spectrometry - TIMS (mole%) : 2314100400015 Cm-244 - 27.5 +- 0.5 , Cm-245 - 1.06 +- 0.28, 2314100400016 Cm-246 - 59.4 +- 1.3 , Cm-247 - 2.9 +- 0.4, 2314100400017 Cm-248 - 9.10 +- 0.24 . 2314100400018 The isotopic abundances were determined by alpha-ray 2314100400019 spectrometry(normalized to results of 244Cm with TIMS):2314100400020 Cm-244 - 27.5, Cm-245 - not detected, 2314100400021 Cm-246 - 55.6 +- 1.7, Cm-247 - not detected, 2314100400022 Cm-248 - not detected, Pu-240 - 2.97 +- 0.14 . 2314100400023 Cm sample was irradiated 94 h. 2314100400024 Am-243 abundance was obtained by fitting of normalized 2314100400025 yields at first resonance with code SAMMY-7 and was 2314100400026 defined to be (1.06+-0.10) % . 2314100400027 INC-SPECT The energy integrated neutron intensities at the sample2314100400028 position are 5.2E+10 n/s/m2 in the neutron energy 2314100400029 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314100400030 under a proton beam power of 120 kW. 2314100400031 ANALYSIS The contributions from 246Cm were calculated by 2314100400032 subtracting the contributions from the impurities from 2314100400033 the capture yields. 2314100400034 Contributions from impurities of 240Pu, 243Am, 244Cm 2314100400035 were calculated with SAMMY code using the parameters of2314100400036 these work and JENDL-4.0. 2314100400037 Neutron-capture cross sections of 246Cm were obtained 2314100400038 by dividing the 246Cm contributions by the isotopic 2314100400039 ratio. 2314100400040 ERR-ANALYS (ERR-T,,,P) Total uncertainty. 2314100400041 (ERR-S,,,U) Statistical Error. 2314100400042 (ERR-1,,,F) Systematic Error in the normalization. 2314100400043 (ERR-2,,,U) Error in the contribution of capture events2314100400044 of the other nuclei. 2314100400045 (ERR-3,,,U) Error in the contribution of fission events2314100400046 (ERR-4,,,U) Error in the corrections of self-shielding 2314100400047 and multiple scattering. 2314100400048 (ERR-5,,,P) Other uncertainties (neutron flux, 2314100400049 contaminations of scattered events, deadtime 2314100400050 correction. 2314100400051 Non-neutron-energy-dependent errors are: 2314100400052 SAMMY fitting error 0.3%. 2314100400053 Errors in the abundances of 240Pu 4.7%. 2314100400054 Errors in the evaluated value of JENDL-4.0 of 2314100400055 the first resonance of 240Pu 2.2% . 2314100400056 Systematic errors in influences of the 2314100400057 scattered neutrons 0.3%. 2314100400058 Error in the isotopic ratio of 244Cm to 2314100400059 246Cm 2.7%. 2314100400060 Error in the abundances of 240Pu and error in the 2314100400061 isotopic ratio of 244Cm to 246Cm" are not independent; 2314100400062 both errors include error in the isotopic ratio of 2314100400063 244Cm (comment of author Atsushi Kimura ). 2314100400064 MISC-COL (MISC) ERR-1 in absolute units. 2314100400065 STATUS (TABLE) Data were received from author Atsushi Kimura 2314100400066 23.10.2012 . 2314100400067 Data are on Fig. 23 of J,NST,49,(7),708,2012 . 2314100400068 Preliminary data on Fig. 6b of J,KPS,59,(2),1828,2011. 2314100400069 ENDBIB 67 0 2314100400070 COMMON 1 3 2314100400071 ERR-1 2314100400072 PER-CENT 2314100400073 5.9 2314100400074 ENDCOMMON 3 0 2314100400075 DATA 9 1009 2314100400076 EN DATA ERR-T ERR-S MISC ERR-2 2314100400077 ERR-3 ERR-4 ERR-5 2314100400078 EV B B B B B 2314100400079 B B B 2314100400080 2.0027E+00 -6.62E+00 4.47E+01 1.00E+01 3.92E-01 4.80E-012314100400081 4.36E+01 1.36E-02 1.65E-01 2314100400082 2.0064E+00 -2.20E+01 4.42E+01 1.00E+01 1.30E+00 4.74E-012314100400083 4.30E+01 5.77E-03 5.17E-01 2314100400084 2.0100E+00 -8.38E+00 4.37E+01 1.00E+01 4.97E-01 4.69E-012314100400085 4.25E+01 9.49E-03 2.03E-01 2314100400086 2.0137E+00 -1.05E+01 4.31E+01 1.00E+01 6.21E-01 4.64E-012314100400087 4.19E+01 7.50E-03 2.50E-01 2314100400088 2.0174E+00 -1.33E+01 4.24E+01 9.96E+00 7.90E-01 4.59E-012314100400089 4.12E+01 5.57E-03 3.15E-01 2314100400090 2.0211E+00 -1.49E+01 4.17E+01 1.00E+01 8.85E-01 4.55E-012314100400091 4.05E+01 3.83E-03 3.52E-01 2314100400092 2.0248E+00 -7.85E+00 4.10E+01 9.94E+00 4.65E-01 4.50E-012314100400093 3.97E+01 2.54E-03 1.90E-01 2314100400094 2.0285E+00 -2.09E+01 4.02E+01 9.99E+00 1.24E+00 4.46E-012314100400095 3.89E+01 2.45E-05 4.91E-01 2314100400096 2.0322E+00 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3.26E-012314100402023 2.78E+00 2.04E+00 6.71E-01 2314100402024 1.5060E+02 3.56E+01 7.61E+00 6.51E+00 2.11E+00 5.95E-012314100402025 2.73E+00 1.61E+00 8.42E-01 2314100402026 1.5300E+02 2.11E+01 7.57E+00 6.84E+00 1.25E+00 1.15E+002314100402027 2.69E+00 4.75E-01 5.00E-01 2314100402028 1.5546E+02 2.93E+01 7.89E+00 7.19E+00 1.73E+00 1.69E-012314100402029 2.65E+00 2.52E-01 6.91E-01 2314100402030 1.5799E+02 1.65E+02 1.37E+01 7.60E+00 9.78E+00 1.94E-012314100402031 4.18E+00 5.74E-01 3.90E+00 2314100402032 1.6057E+02 7.73E+01 9.25E+00 6.82E+00 4.59E+00 6.37E-012314100402033 2.57E+00 2.78E+00 1.83E+00 2314100402034 1.6322E+02 2.48E+01 7.55E+00 6.71E+00 1.47E+00 1.29E+002314100402035 2.54E+00 1.18E+00 5.87E-01 2314100402036 1.6594E+02 4.78E+00 6.39E+00 5.82E+00 2.84E-01 3.17E-012314100402037 2.50E+00 7.27E-01 1.14E-01 2314100402038 1.6872E+02 -2.02E+00 6.17E+00 5.60E+00 1.20E-01 7.12E-012314100402039 2.47E+00 2.27E-01 4.76E-02 2314100402040 1.7158E+02 -8.77E+00 8.72E+00 6.24E+00 5.20E-01 5.49E+002314100402041 2.49E+00 6.19E-01 2.07E-01 2314100402042 1.7451E+02 2.69E+01 7.61E+00 5.61E+00 1.59E+00 4.72E-012314100402043 2.42E+00 4.17E+00 6.36E-01 2314100402044 1.7751E+02 4.40E+01 8.30E+00 6.25E+00 2.61E+00 2.99E-012314100402045 2.40E+00 4.00E+00 1.04E+00 2314100402046 1.8059E+02 3.78E+01 1.14E+01 7.11E+00 2.24E+00 7.88E+002314100402047 2.80E+00 1.77E+00 9.00E-01 2314100402048 1.8375E+02 2.62E+01 7.83E+00 6.98E+00 1.55E+00 1.50E+002314100402049 2.37E+00 1.37E+00 6.21E-01 2314100402050 1.8700E+02 2.08E+01 7.93E+00 7.18E+00 1.23E+00 1.90E+002314100402051 2.39E+00 5.19E-01 4.94E-01 2314100402052 1.9033E+02 2.07E+01 7.66E+00 7.14E+00 1.23E+00 2.12E-012314100402053 2.35E+00 6.84E-01 4.88E-01 2314100402054 1.9376E+02 9.53E+01 1.04E+01 7.19E+00 5.65E+00 6.41E-012314100402055 2.38E+00 3.62E+00 2.25E+00 2314100402056 1.9727E+02 2.72E+01 2.80E+01 7.65E+00 1.61E+00 2.67E+012314100402057 2.78E+00 1.16E+00 6.81E-01 2314100402058 2.0089E+02 3.80E+01 7.97E+00 6.99E+00 2.25E+00 2.62E-012314100402059 2.31E+00 1.81E+00 8.98E-01 2314100402060 2.0460E+02 3.27E+01 7.67E+00 6.86E+00 1.94E+00 1.64E-012314100402061 2.19E+00 1.65E+00 7.74E-01 2314100402062 2.0842E+02 2.62E+01 1.44E+01 7.32E+00 1.55E+00 1.21E+012314100402063 2.20E+00 1.30E+00 6.32E-01 2314100402064 2.1234E+02 4.86E+01 9.15E+00 6.53E+00 2.88E+00 2.80E+002314100402065 2.00E+00 4.43E+00 1.15E+00 2314100402066 2.1638E+02 3.59E+01 7.83E+00 6.74E+00 2.13E+00 4.67E-012314100402067 1.92E+00 2.59E+00 8.48E-01 2314100402068 2.2053E+02 -1.05E+01 2.33E+01 7.43E+00 6.22E-01 2.19E+012314100402069 2.42E+00 1.14E+00 2.74E-01 2314100402070 2.2480E+02 2.08E+01 7.11E+00 6.27E+00 1.23E+00 3.44E-012314100402071 1.82E+00 2.47E+00 4.92E-01 2314100402072 2.2920E+02 8.24E+00 1.26E+01 7.21E+00 4.89E-01 1.00E+012314100402073 1.90E+00 1.62E+00 2.12E-01 2314100402074 2.3373E+02 5.23E+01 9.42E+00 7.00E+00 3.10E+00 3.44E+002314100402075 1.96E+00 3.61E+00 1.24E+00 2314100402076 2.3840E+02 4.01E+01 8.94E+00 7.24E+00 2.38E+00 2.93E+002314100402077 2.10E+00 2.84E+00 9.51E-01 2314100402078 2.4320E+02 6.17E+01 9.71E+00 6.99E+00 3.66E+00 1.14E+002314100402079 2.19E+00 4.90E+00 1.46E+00 2314100402080 2.4816E+02 6.58E+01 1.01E+01 7.16E+00 3.90E+00 3.01E-012314100402081 2.39E+00 5.19E+00 1.56E+00 2314100402082 2.5326E+02 7.32E+01 1.02E+01 7.14E+00 4.34E+00 8.05E-022314100402083 2.36E+00 5.03E+00 1.73E+00 2314100402084 2.5853E+02 6.78E+01 1.05E+01 8.00E+00 4.02E+00 4.43E+002314100402085 2.27E+00 1.77E+00 1.61E+00 2314100402086 2.6396E+02 4.14E+01 9.79E+00 7.80E+00 2.45E+00 4.49E+002314100402087 2.08E+00 1.91E+00 9.82E-01 2314100402088 2.6956E+02 3.93E+01 8.44E+00 7.24E+00 2.33E+00 2.82E-012314100402089 1.94E+00 2.95E+00 9.29E-01 2314100402090 2.7535E+02 4.12E+01 1.01E+01 7.88E+00 2.44E+00 5.18E+002314100402091 1.91E+00 1.39E+00 9.87E-01 2314100402092 2.8132E+02 9.33E+00 7.89E+00 7.64E+00 5.53E-01 1.94E-022314100402093 1.81E+00 5.45E-01 2.23E-01 2314100402094 2.8749E+02 -4.06E+00 8.71E+00 8.38E+00 2.41E-01 1.53E+002314100402095 1.81E+00 2.98E-02 9.57E-02 2314100402096 2.9386E+02 -1.14E+01 7.53E+00 7.26E+00 6.76E-01 7.75E-032314100402097 1.66E+00 8.74E-01 2.70E-01 2314100402098 ENDDATA 2022 0 2314100402099 ENDSUBENT 2098 0 2314100499999 SUBENT 23141005 20120823 22332314100500001 BIB 7 46 2314100500002 REACTION 1(96-CM-244(N,0),,EN) 2314100500003 2(96-CM-244(N,G),,WID) 2314100500004 3(96-CM-244(N,EL),,WID) 2314100500005 SAMPLE Cm-244 sample was 0.6 mg of curium oxide. 2314100500006 Isotopic enrichment was 90.1 mole%, main activity was 2314100500007 1.8 GBq. Sample was sealed in an Al case of 9 mm outer 2314100500008 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314100500009 Sample was put in a bag of fluorinated ethylene 2314100500010 propylene (FEP) films and attached to a sample holder 2314100500011 made of polytetrafluoroethylene and shaped into 2314100500012 50mmx70 mm rectangular frame. 2314100500013 The isotopic abundances were determined by thermal 2314100500014 ionization mass spectrometry - TIMS (mole%) : 2314100500015 Cm-244 - 90.1 +- 1.7 , Cm-245 - 2.71 +- 0.34, 2314100500016 Cm-246 - 7.22 +- 0.34, Cm-247 - not detected, 2314100500017 Cm-248 - not detected. 2314100500018 The isotopic abundances were determined by alpha-ray 2314100500019 spectrometry(normalized to results of 244Cm with TIMS):2314100500020 Cm-244 - 90.1, Cm-245 - not detected, 2314100500021 Cm-246 - 7.0 +- 0.6, Cm-247 - not detected, 2314100500022 Cm-248 - not detected, Pu-240 - 13.6 +- 0.6 . 2314100500023 Cm sample was irradiated 64 h. 2314100500024 Am-243 abundance was obtained by fitting of normalized 2314100500025 yields at first resonance with code SAMMY-7 and was 2314100500026 defined to be (0.63+-0.04) % . 2314100500027 INC-SPECT The energy integrated neutron intensities at the sample2314100500028 position are 5.2E+10 n/s/m2 in the neutron energy 2314100500029 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314100500030 under a proton beam power of 120 kW. 2314100500031 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314100500032 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314100500033 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314100500034 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314100500035 Distance from sample 125 mm. 2314100500036 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314100500037 yields by SAMMY-7 code fitting. Multi-level 2314100500038 Breit-Wigner formalism was used in this R-matrix 2314100500039 Bayesian code (see REL-REF of N.M.Larson) . 2314100500040 The free gas model with a target temperature of 293 K 2314100500041 was applied to the Doppler broadening. 2314100500042 REL-REF (N,,N.M.Larson,R,ORNL-TM-9179/R7,2006) 2314100500043 Updated Users Guide for SAMMY: 2314100500044 Multilevel R-Matrix Fits to Neutron Data Using Bayes 2314100500045 Equations, ORNL/TM-9179/R7, Oak Ridge National Lab., 2314100500046 Oak Ridge, TN, 2006. 2314100500047 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314100500048 ENDBIB 46 0 2314100500049 NOCOMMON 0 0 2314100500050 DATA 6 3 2314100500051 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314100500052 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314100500053 7.659 0.012 38.1 2.9 8.90 0.25 2314100500054 16.790 0.029 38. 4. 1.74 0.06 2314100500055 22.85 0.04 40. 4. 0.90 0.04 2314100500056 ENDDATA 5 0 2314100500057 ENDSUBENT 56 0 2314100599999 SUBENT 23141006 20120823 22332314100600001 BIB 6 41 2314100600002 REACTION 1(96-CM-246(N,0),,EN) 2314100600003 2(96-CM-246(N,G),,WID) 2314100600004 3(96-CM-246(N,EL),,WID) 2314100600005 SAMPLE Cm-244 sample was 0.6 mg of curium oxide. 2314100600006 Isotopic enrichment was 90.1 mole%, main activity was 2314100600007 1.8 GBq. Sample was sealed in an Al case of 9 mm outer 2314100600008 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314100600009 Sample was put in a bag of fluorinated ethylene 2314100600010 propylene (FEP) films and attached to a sample holder 2314100600011 made of polytetrafluoroethylene and shaped into 2314100600012 50mmx70 mm rectangular frame. 2314100600013 The isotopic abundances were determined by thermal 2314100600014 ionization mass spectrometry - TIMS (mole%) : 2314100600015 Cm-244 - 90.1 +- 1.7 , Cm-245 - 2.71 +- 0.34, 2314100600016 Cm-246 - 7.22 +- 0.34, Cm-247 - not detected, 2314100600017 Cm-248 - not detected. 2314100600018 The isotopic abundances were determined by alpha-ray 2314100600019 spectrometry(normalized to results of 244Cm with TIMS):2314100600020 Cm-244 - 90.1, Cm-245 - not detected, 2314100600021 Cm-246 - 7.0 +- 0.6, Cm-247 - not detected, 2314100600022 Cm-248 - not detected, Pu-240 - 13.6 +- 0.6 . 2314100600023 Cm sample was irradiated 64 h. 2314100600024 Am-243 abundance was obtained by fitting of normalized 2314100600025 yields at first resonance with code SAMMY-7 and was 2314100600026 defined to be (0.63+-0.04) % . 2314100600027 INC-SPECT The energy integrated neutron intensities at the sample2314100600028 position are 5.2E+10 n/s/m2 in the neutron energy 2314100600029 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314100600030 under a proton beam power of 120 kW. 2314100600031 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314100600032 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314100600033 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314100600034 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314100600035 Distance from sample 125 mm. 2314100600036 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314100600037 yields by SAMMY-7 code fitting. Multi-level 2314100600038 Breit-Wigner formalism was used in this R-matrix 2314100600039 Bayesian code (see REL-REF of N.M.Larson) . 2314100600040 The free gas model with a target temperature of 293 K 2314100600041 was applied to the Doppler broadening. 2314100600042 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314100600043 ENDBIB 41 0 2314100600044 NOCOMMON 0 0 2314100600045 DATA 6 1 2314100600046 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314100600047 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314100600048 4.317 0.007 26.7 2.6 0.266 0.013 2314100600049 ENDDATA 3 0 2314100600050 ENDSUBENT 49 0 2314100699999 SUBENT 23141007 20120823 22332314100700001 BIB 6 41 2314100700002 REACTION 1(94-PU-240(N,0),,EN) 2314100700003 2(94-PU-240(N,G),,WID) 2314100700004 3(94-PU-240(N,EL),,WID) 2314100700005 SAMPLE Cm-244 sample was 0.6 mg of curium oxide. 2314100700006 Isotopic enrichment was 90.1 mole%, main activity was 2314100700007 1.8 GBq. Sample was sealed in an Al case of 9 mm outer 2314100700008 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314100700009 Sample was put in a bag of fluorinated ethylene 2314100700010 propylene (FEP) films and attached to a sample holder 2314100700011 made of polytetrafluoroethylene and shaped into 2314100700012 50mmx70 mm rectangular frame. 2314100700013 The isotopic abundances were determined by thermal 2314100700014 ionization mass spectrometry - TIMS (mole%) : 2314100700015 Cm-244 - 90.1 +- 1.7 , Cm-245 - 2.71 +- 0.34, 2314100700016 Cm-246 - 7.22 +- 0.34, Cm-247 - not detected, 2314100700017 Cm-248 - not detected. 2314100700018 The isotopic abundances were determined by alpha-ray 2314100700019 spectrometry(normalized to results of 244Cm with TIMS):2314100700020 Cm-244 - 90.1, Cm-245 - not detected, 2314100700021 Cm-246 - 7.0 +- 0.6, Cm-247 - not detected, 2314100700022 Cm-248 - not detected, Pu-240 - 13.6 +- 0.6 . 2314100700023 Cm sample was irradiated 64 h. 2314100700024 Am-243 abundance was obtained by fitting of normalized 2314100700025 yields at first resonance with code SAMMY-7 and was 2314100700026 defined to be (0.63+-0.04) % . 2314100700027 INC-SPECT The energy integrated neutron intensities at the sample2314100700028 position are 5.2E+10 n/s/m2 in the neutron energy 2314100700029 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314100700030 under a proton beam power of 120 kW. 2314100700031 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314100700032 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314100700033 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314100700034 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314100700035 Distance from sample 125 mm. 2314100700036 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314100700037 yields by SAMMY-7 code fitting. Multi-level 2314100700038 Breit-Wigner formalism was used in this R-matrix 2314100700039 Bayesian code (see REL-REF of N.M.Larson) . 2314100700040 The free gas model with a target temperature of 293 K 2314100700041 was applied to the Doppler broadening. 2314100700042 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314100700043 ENDBIB 41 0 2314100700044 NOCOMMON 0 0 2314100700045 DATA 6 2 2314100700046 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314100700047 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314100700048 1.0551 0.0015 30.6 0.6 2.446 0.018 2314100700049 20.45 0.05 28. 5. 2.8 0.4 2314100700050 ENDDATA 4 0 2314100700051 ENDSUBENT 50 0 2314100799999 SUBENT 23141008 20120823 22332314100800001 BIB 6 41 2314100800002 REACTION 1(95-AM-243(N,0),,EN) 2314100800003 2(95-AM-243(N,G),,WID) 2314100800004 3(95-AM-243(N,EL),,WID) 2314100800005 SAMPLE Cm-244 sample was 0.6 mg of curium oxide. 2314100800006 Isotopic enrichment was 90.1 mole%, main activity was 2314100800007 1.8 GBq. Sample was sealed in an Al case of 9 mm outer 2314100800008 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314100800009 Sample was put in a bag of fluorinated ethylene 2314100800010 propylene (FEP) films and attached to a sample holder 2314100800011 made of polytetrafluoroethylene and shaped into 2314100800012 50mmx70 mm rectangular frame. 2314100800013 The isotopic abundances were determined by thermal 2314100800014 ionization mass spectrometry - TIMS (mole%) : 2314100800015 Cm-244 - 90.1 +- 1.7 , Cm-245 - 2.71 +- 0.34, 2314100800016 Cm-246 - 7.22 +- 0.34, Cm-247 - not detected, 2314100800017 Cm-248 - not detected. 2314100800018 The isotopic abundances were determined by alpha-ray 2314100800019 spectrometry(normalized to results of 244Cm with TIMS):2314100800020 Cm-244 - 90.1, Cm-245 - not detected, 2314100800021 Cm-246 - 7.0 +- 0.6, Cm-247 - not detected, 2314100800022 Cm-248 - not detected, Pu-240 - 13.6 +- 0.6 . 2314100800023 Cm sample was irradiated 64 h. 2314100800024 Am-243 abundance was obtained by fitting of normalized 2314100800025 yields at first resonance with code SAMMY-7 and was 2314100800026 defined to be (0.63+-0.04) % . 2314100800027 INC-SPECT The energy integrated neutron intensities at the sample2314100800028 position are 5.2E+10 n/s/m2 in the neutron energy 2314100800029 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314100800030 under a proton beam power of 120 kW. 2314100800031 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314100800032 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314100800033 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314100800034 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314100800035 Distance from sample 125 mm. 2314100800036 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314100800037 yields by SAMMY-7 code fitting. Multi-level 2314100800038 Breit-Wigner formalism was used in this R-matrix 2314100800039 Bayesian code (see REL-REF of N.M.Larson) . 2314100800040 The free gas model with a target temperature of 293 K 2314100800041 was applied to the Doppler broadening. 2314100800042 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314100800043 ENDBIB 41 0 2314100800044 NOCOMMON 0 0 2314100800045 DATA 6 1 2314100800046 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314100800047 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314100800048 1.350 0.004 51. 4. 1.02 0.06 2314100800049 ENDDATA 3 0 2314100800050 ENDSUBENT 49 0 2314100899999 SUBENT 23141009 20120823 22332314100900001 BIB 6 43 2314100900002 REACTION 1(96-CM-244(N,0),,EN) 2314100900003 2(96-CM-244(N,G),,WID) 2314100900004 3(96-CM-244(N,EL),,WID) 2314100900005 SAMPLE Cm-246 sample was 2.1 mg of curium oxide. 2314100900006 Cm-246 Isotopic enrichment was 59.4 mole% with 27.5 2314100900007 mole% Cm-244, it's main activities were Cm246 12.1 MBq,2314100900008 Cm-244 1.7 GBq. 2314100900009 Sample was sealed in an Al case of 9 mm outer 2314100900010 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314100900011 Sample was put in a bag of fluorinated ethylene 2314100900012 propylene (FEP) films and attached to a sample holder 2314100900013 made of polytetrafluoroethylene and shaped into 2314100900014 50mmx70 mm rectangular frame. 2314100900015 The isotopic abundances were determined by thermal 2314100900016 ionization mass spectrometry - TIMS (mole%) : 2314100900017 Cm-244 - 27.5 +- 0.5 , Cm-245 - 1.06 +- 0.28, 2314100900018 Cm-246 - 59.4 +- 1.3 , Cm-247 - 2.9 +- 0.4, 2314100900019 Cm-248 - 9.10 +- 0.24 . 2314100900020 The isotopic abundances were determined by alpha-ray 2314100900021 spectrometry(normalized to results of 244Cm with TIMS):2314100900022 Cm-244 - 27.5, Cm-245 - not detected, 2314100900023 Cm-246 - 55.6 +- 1.7, Cm-247 - not detected, 2314100900024 Cm-248 - not detected, Pu-240 - 2.97 +- 0.14 . 2314100900025 Cm sample was irradiated 94 h. 2314100900026 Am-243 abundance was obtained by fitting of normalized 2314100900027 yields at first resonance with code SAMMY-7 and was 2314100900028 defined to be (1.06+-0.10) % . 2314100900029 INC-SPECT The energy integrated neutron intensities at the sample2314100900030 position are 5.2E+10 n/s/m2 in the neutron energy 2314100900031 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314100900032 under a proton beam power of 120 kW. 2314100900033 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314100900034 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314100900035 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314100900036 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314100900037 Distance from sample 125 mm. 2314100900038 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314100900039 yields by SAMMY-7 code fitting. Multi-level 2314100900040 Breit-Wigner formalism was used in this R-matrix 2314100900041 Bayesian code (see REL-REF of N.M.Larson) . 2314100900042 The free gas model with a target temperature of 293 K 2314100900043 was applied to the Doppler broadening. 2314100900044 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314100900045 ENDBIB 43 0 2314100900046 NOCOMMON 0 0 2314100900047 DATA 6 3 2314100900048 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314100900049 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314100900050 7.662 0.012 38. 5. 8.6 0.4 2314100900051 16.79 0.03 38. 7. 1.70 0.12 2314100900052 22.86 0.04 41. 8. 0.93 0.09 2314100900053 ENDDATA 5 0 2314100900054 ENDSUBENT 53 0 2314100999999 SUBENT 23141010 20120823 22332314101000001 BIB 6 43 2314101000002 REACTION 1(96-CM-246(N,0),,EN) 2314101000003 2(96-CM-246(N,G),,WID) 2314101000004 3(96-CM-246(N,EL),,WID) 2314101000005 SAMPLE Cm-246 sample was 2.1 mg of curium oxide. 2314101000006 Cm-246 Isotopic enrichment was 59.4 mole% with 27.5 2314101000007 mole% Cm-244, it's main activities were Cm246 12.1 MBq,2314101000008 Cm-244 1.7 GBq. 2314101000009 Sample was sealed in an Al case of 9 mm outer 2314101000010 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314101000011 Sample was put in a bag of fluorinated ethylene 2314101000012 propylene (FEP) films and attached to a sample holder 2314101000013 made of polytetrafluoroethylene and shaped into 2314101000014 50mmx70 mm rectangular frame. 2314101000015 The isotopic abundances were determined by thermal 2314101000016 ionization mass spectrometry - TIMS (mole%) : 2314101000017 Cm-244 - 27.5 +- 0.5 , Cm-245 - 1.06 +- 0.28, 2314101000018 Cm-246 - 59.4 +- 1.3 , Cm-247 - 2.9 +- 0.4, 2314101000019 Cm-248 - 9.10 +- 0.24 . 2314101000020 The isotopic abundances were determined by alpha-ray 2314101000021 spectrometry(normalized to results of 244Cm with TIMS):2314101000022 Cm-244 - 27.5, Cm-245 - not detected, 2314101000023 Cm-246 - 55.6 +- 1.7, Cm-247 - not detected, 2314101000024 Cm-248 - not detected, Pu-240 - 2.97 +- 0.14 . 2314101000025 Cm sample was irradiated 94 h. 2314101000026 Am-243 abundance was obtained by fitting of normalized 2314101000027 yields at first resonance with code SAMMY-7 and was 2314101000028 defined to be (1.06+-0.10) % . 2314101000029 INC-SPECT The energy integrated neutron intensities at the sample2314101000030 position are 5.2E+10 n/s/m2 in the neutron energy 2314101000031 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314101000032 under a proton beam power of 120 kW. 2314101000033 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314101000034 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314101000035 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314101000036 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314101000037 Distance from sample 125 mm. 2314101000038 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314101000039 yields by SAMMY-7 code fitting. Multi-level 2314101000040 Breit-Wigner formalism was used in this R-matrix 2314101000041 Bayesian code (see REL-REF of N.M.Larson) . 2314101000042 The free gas model with a target temperature of 293 K 2314101000043 was applied to the Doppler broadening. 2314101000044 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314101000045 ENDBIB 43 0 2314101000046 NOCOMMON 0 0 2314101000047 DATA 6 2 2314101000048 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314101000049 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314101000050 4.311 0.007 29.5 3.1 0.300 0.009 2314101000051 15.31 0.03 33. 6. 0.50 0.04 2314101000052 ENDDATA 4 0 2314101000053 ENDSUBENT 52 0 2314101099999 SUBENT 23141011 20120823 22332314101100001 BIB 6 43 2314101100002 REACTION 1(96-CM-248(N,0),,EN) 2314101100003 2(96-CM-248(N,G),,WID) 2314101100004 3(96-CM-248(N,EL),,WID) 2314101100005 SAMPLE Cm-246 sample was 2.1 mg of curium oxide. 2314101100006 Cm-246 Isotopic enrichment was 59.4 mole% with 27.5 2314101100007 mole% Cm-244, it's main activities were Cm246 12.1 MBq,2314101100008 Cm-244 1.7 GBq. 2314101100009 Sample was sealed in an Al case of 9 mm outer 2314101100010 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314101100011 Sample was put in a bag of fluorinated ethylene 2314101100012 propylene (FEP) films and attached to a sample holder 2314101100013 made of polytetrafluoroethylene and shaped into 2314101100014 50mmx70 mm rectangular frame. 2314101100015 The isotopic abundances were determined by thermal 2314101100016 ionization mass spectrometry - TIMS (mole%) : 2314101100017 Cm-244 - 27.5 +- 0.5 , Cm-245 - 1.06 +- 0.28, 2314101100018 Cm-246 - 59.4 +- 1.3 , Cm-247 - 2.9 +- 0.4, 2314101100019 Cm-248 - 9.10 +- 0.24 . 2314101100020 The isotopic abundances were determined by alpha-ray 2314101100021 spectrometry(normalized to results of 244Cm with TIMS):2314101100022 Cm-244 - 27.5, Cm-245 - not detected, 2314101100023 Cm-246 - 55.6 +- 1.7, Cm-247 - not detected, 2314101100024 Cm-248 - not detected, Pu-240 - 2.97 +- 0.14 . 2314101100025 Cm sample was irradiated 94 h. 2314101100026 Am-243 abundance was obtained by fitting of normalized 2314101100027 yields at first resonance with code SAMMY-7 and was 2314101100028 defined to be (1.06+-0.10) % . 2314101100029 INC-SPECT The energy integrated neutron intensities at the sample2314101100030 position are 5.2E+10 n/s/m2 in the neutron energy 2314101100031 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314101100032 under a proton beam power of 120 kW. 2314101100033 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314101100034 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314101100035 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314101100036 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314101100037 Distance from sample 125 mm. 2314101100038 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314101100039 yields by SAMMY-7 code fitting. Multi-level 2314101100040 Breit-Wigner formalism was used in this R-matrix 2314101100041 Bayesian code (see REL-REF of N.M.Larson) . 2314101100042 The free gas model with a target temperature of 293 K 2314101100043 was applied to the Doppler broadening. 2314101100044 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314101100045 ENDBIB 43 0 2314101100046 NOCOMMON 0 0 2314101100047 DATA 6 2 2314101100048 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314101100049 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314101100050 7.242 0.012 25. 4. 1.78 0.10 2314101100051 26.90 0.05 33. 6. 17.8 2.2 2314101100052 ENDDATA 4 0 2314101100053 ENDSUBENT 52 0 2314101199999 SUBENT 23141012 20120823 22332314101200001 BIB 6 43 2314101200002 REACTION 1(94-PU-240(N,0),,EN) 2314101200003 2(94-PU-240(N,G),,WID) 2314101200004 3(94-PU-240(N,EL),,WID) 2314101200005 SAMPLE Cm-246 sample was 2.1 mg of curium oxide. 2314101200006 Cm-246 Isotopic enrichment was 59.4 mole% with 27.5 2314101200007 mole% Cm-244, it's main activities were Cm246 12.1 MBq,2314101200008 Cm-244 1.7 GBq. 2314101200009 Sample was sealed in an Al case of 9 mm outer 2314101200010 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314101200011 Sample was put in a bag of fluorinated ethylene 2314101200012 propylene (FEP) films and attached to a sample holder 2314101200013 made of polytetrafluoroethylene and shaped into 2314101200014 50mmx70 mm rectangular frame. 2314101200015 The isotopic abundances were determined by thermal 2314101200016 ionization mass spectrometry - TIMS (mole%) : 2314101200017 Cm-244 - 27.5 +- 0.5 , Cm-245 - 1.06 +- 0.28, 2314101200018 Cm-246 - 59.4 +- 1.3 , Cm-247 - 2.9 +- 0.4, 2314101200019 Cm-248 - 9.10 +- 0.24 . 2314101200020 The isotopic abundances were determined by alpha-ray 2314101200021 spectrometry(normalized to results of 244Cm with TIMS):2314101200022 Cm-244 - 27.5, Cm-245 - not detected, 2314101200023 Cm-246 - 55.6 +- 1.7, Cm-247 - not detected, 2314101200024 Cm-248 - not detected, Pu-240 - 2.97 +- 0.14 . 2314101200025 Cm sample was irradiated 94 h. 2314101200026 Am-243 abundance was obtained by fitting of normalized 2314101200027 yields at first resonance with code SAMMY-7 and was 2314101200028 defined to be (1.06+-0.10) % . 2314101200029 INC-SPECT The energy integrated neutron intensities at the sample2314101200030 position are 5.2E+10 n/s/m2 in the neutron energy 2314101200031 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314101200032 under a proton beam power of 120 kW. 2314101200033 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314101200034 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314101200035 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314101200036 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314101200037 Distance from sample 125 mm. 2314101200038 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314101200039 yields by SAMMY-7 code fitting. Multi-level 2314101200040 Breit-Wigner formalism was used in this R-matrix 2314101200041 Bayesian code (see REL-REF of N.M.Larson) . 2314101200042 The free gas model with a target temperature of 293 K 2314101200043 was applied to the Doppler broadening. 2314101200044 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314101200045 ENDBIB 43 0 2314101200046 NOCOMMON 0 0 2314101200047 DATA 6 2 2314101200048 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314101200049 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314101200050 1.0550 0.0015 30.6 0.6 2.445 0.018 2314101200051 20.45 0.04 27. 5. 2.9 0.4 2314101200052 ENDDATA 4 0 2314101200053 ENDSUBENT 52 0 2314101299999 SUBENT 23141013 20120823 22332314101300001 BIB 6 43 2314101300002 REACTION 1(95-AM-243(N,0),,EN) 2314101300003 2(95-AM-243(N,G),,WID) 2314101300004 3(95-AM-243(N,EL),,WID) 2314101300005 SAMPLE Cm-246 sample was 2.1 mg of curium oxide. 2314101300006 Cm-246 Isotopic enrichment was 59.4 mole% with 27.5 2314101300007 mole% Cm-244, it's main activities were Cm246 12.1 MBq,2314101300008 Cm-244 1.7 GBq. 2314101300009 Sample was sealed in an Al case of 9 mm outer 2314101300010 diameter, weighing 280 mg, 0.5-mm-thick walls. 2314101300011 Sample was put in a bag of fluorinated ethylene 2314101300012 propylene (FEP) films and attached to a sample holder 2314101300013 made of polytetrafluoroethylene and shaped into 2314101300014 50mmx70 mm rectangular frame. 2314101300015 The isotopic abundances were determined by thermal 2314101300016 ionization mass spectrometry - TIMS (mole%) : 2314101300017 Cm-244 - 27.5 +- 0.5 , Cm-245 - 1.06 +- 0.28, 2314101300018 Cm-246 - 59.4 +- 1.3 , Cm-247 - 2.9 +- 0.4, 2314101300019 Cm-248 - 9.10 +- 0.24 . 2314101300020 The isotopic abundances were determined by alpha-ray 2314101300021 spectrometry(normalized to results of 244Cm with TIMS):2314101300022 Cm-244 - 27.5, Cm-245 - not detected, 2314101300023 Cm-246 - 55.6 +- 1.7, Cm-247 - not detected, 2314101300024 Cm-248 - not detected, Pu-240 - 2.97 +- 0.14 . 2314101300025 Cm sample was irradiated 94 h. 2314101300026 Am-243 abundance was obtained by fitting of normalized 2314101300027 yields at first resonance with code SAMMY-7 and was 2314101300028 defined to be (1.06+-0.10) % . 2314101300029 INC-SPECT The energy integrated neutron intensities at the sample2314101300030 position are 5.2E+10 n/s/m2 in the neutron energy 2314101300031 range 1.5-25 meV and 7.2E+09 n/s/m2 in 0.9-1.1 keV 2314101300032 under a proton beam power of 120 kW. 2314101300033 DETECTOR The peak efficiency of 4PI Ge spectrometer is 2314101300034 2.28+-0.11 % for 1.33-MeV gamma- rays. 2314101300035 Typical resolution is 5.5 keV (on beam) and 2.4 keV 2314101300036 (off beam) in FWHM for 1.33-MeV gamma-rays. 2314101300037 Distance from sample 125 mm. 2314101300038 ANALYSIS (MLA) Resonance parameters were extracted from capture 2314101300039 yields by SAMMY-7 code fitting. Multi-level 2314101300040 Breit-Wigner formalism was used in this R-matrix 2314101300041 Bayesian code (see REL-REF of N.M.Larson) . 2314101300042 The free gas model with a target temperature of 293 K 2314101300043 was applied to the Doppler broadening. 2314101300044 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314101300045 ENDBIB 43 0 2314101300046 NOCOMMON 0 0 2314101300047 DATA 6 1 2314101300048 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314101300049 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314101300050 1.350 0.003 45. 8. 1.07 0.10 2314101300051 ENDDATA 3 0 2314101300052 ENDSUBENT 51 0 2314101399999 SUBENT 23141014 20120823 22332314101400001 BIB 3 7 2314101400002 REACTION 1(96-CM-244(N,0),,EN) 2314101400003 2(96-CM-244(N,G),,WID) 2314101400004 3(96-CM-244(N,EL),,WID) 2314101400005 ANALYSIS Average of two samples. 2314101400006 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314101400007 (DEP,23141005) See 2314101400008 (DEP,23141009) ANALYSIS 2314101400009 ENDBIB 7 0 2314101400010 NOCOMMON 0 0 2314101400011 DATA 6 3 2314101400012 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314101400013 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314101400014 7.661 0.011 37.8 2.9 8.77 0.22 2314101400015 16.79 0.03 38. 4. 1.72 0.07 2314101400016 22.86 0.04 40. 4. 0.91 0.05 2314101400017 ENDDATA 5 0 2314101400018 ENDSUBENT 17 0 2314101499999 SUBENT 23141015 20120823 22332314101500001 BIB 3 7 2314101500002 REACTION 1(96-CM-246(N,0),,EN) 2314101500003 2(96-CM-246(N,G),,WID) 2314101500004 3(96-CM-246(N,EL),,WID) 2314101500005 ANALYSIS Average of two samples. 2314101500006 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314101500007 (DEP,23141006) See 2314101500008 (DEP,23141010) ANALYSIS 2314101500009 ENDBIB 7 0 2314101500010 NOCOMMON 0 0 2314101500011 DATA 6 2 2314101500012 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314101500013 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314101500014 4.314 0.006 28.1 2.0 0.283 0.008 2314101500015 15.310 0.027 33. 6. 0.50 0.04 2314101500016 ENDDATA 4 0 2314101500017 ENDSUBENT 16 0 2314101599999 SUBENT 23141016 20120823 22332314101600001 BIB 3 7 2314101600002 REACTION 1(94-PU-240(N,0),,EN) 2314101600003 2(94-PU-240(N,G),,WID) 2314101600004 3(94-PU-240(N,EL),,WID) 2314101600005 ANALYSIS Average of two samples. 2314101600006 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314101600007 (DEP,23141007) See 2314101600008 (DEP,23141012) ANALYSIS 2314101600009 ENDBIB 7 0 2314101600010 NOCOMMON 0 0 2314101600011 DATA 6 2 2314101600012 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314101600013 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314101600014 1.0551 0.0013 30.6 0.4 2.446 0.013 2314101600015 20.45 0.04 28. 4. 2.88 0.29 2314101600016 ENDDATA 4 0 2314101600017 ENDSUBENT 16 0 2314101699999 SUBENT 23141017 20120823 22332314101700001 BIB 3 7 2314101700002 REACTION 1(95-AM-243(N,0),,EN) 2314101700003 2(95-AM-243(N,G),,WID) 2314101700004 3(95-AM-243(N,EL),,WID) 2314101700005 ANALYSIS Average of two samples. 2314101700006 STATUS (TABLE) Table 3 of J,NST,49,(7),708,2012 2314101700007 (DEP,23141008) See 2314101700008 (DEP,23141013) ANALYSIS 2314101700009 ENDBIB 7 0 2314101700010 NOCOMMON 0 0 2314101700011 DATA 6 1 2314101700012 DATA 1DATA-ERR 1DATA 2DATA-ERR 2DATA 3DATA-ERR 32314101700013 EV EV MILLI-EV MILLI-EV MILLI-EV MILLI-EV 2314101700014 1.350 0.003 47. 5. 1.05 0.06 2314101700015 ENDDATA 3 0 2314101700016 ENDSUBENT 15 0 2314101799999 ENDENTRY 17 0 2314199999999