ENTRY C2156 20150310 C148C215600000001 SUBENT C2156001 20150310 C148C215600100001 BIB 8 26 C215600100002 TITLE Cyclotron production of 99mTc: Experimental C215600100003 measurement of the 100Mo(p,x)99Mo, 99mTc and 99gTc C215600100004 excitation functions from 8 to 18 MeV C215600100005 AUTHOR (K.Gagnon,F.Benard,M.Kovacs,T.J.Ruth,P.Schaffer, C215600100006 J.S.Wilson,S.A.Mcquarrie) C215600100007 REFERENCE (J,NMB,38,907,2011) C215600100008 #doi:10.1016/j.nucmedbio.2011.02.010 C215600100009 INSTITUTE (1CANALA,1CANTMF) C215600100010 (1CANCAN) BC Cancer Agency, Vancouver, BC, Canada. C215600100011 (1CANCAN) Lawson Health Research Institute, London, ON,C215600100012 Canada. C215600100013 FACILITY (CYCLO,1CANALA) The variable energy TR 19/9 Cyclotron. C215600100014 MONITOR Monitor values taken from C215600100015 IAEA Charged-particle cross section database for C215600100016 medical radioisotope production, Monitor reactions. C215600100017 http://www-nds.iaea.org/medical/monitor C215600100018 reactions.html, 2009. C215600100019 (29-CU-0(P,X)30-ZN-62,,SIG) C215600100020 (29-CU-0(P,X)30-ZN-63,,SIG) C215600100021 (29-CU-0(P,X)30-ZN-65,,SIG) C215600100022 DECAY-MON (30-ZN-62,9.26HR,DG,548.35,0.153, C215600100023 DG,596.56,0.26) C215600100024 (30-ZN-63,38.47MIN,DG,669.62,0.082, C215600100025 DG,962.06,0.065) C215600100026 (30-ZN-65,243.66D,DG,1115.539,0.506) C215600100027 HISTORY (20150310C) BP C215600100028 ENDBIB 26 0 C215600100029 NOCOMMON 0 0 C215600100030 ENDSUBENT 29 0 C215600199999 SUBENT C2156002 20150310 C148C215600200001 BIB 8 17 C215600200002 REACTION (42-MO-100(P,X)42-MO-99,(CUM),SIG) C215600200003 DECAY-DATA (42-MO-99,65.94HR,DG,140.511,0.0452, C215600200004 DG,181.068,0.0599,DG,739.500,0.1213) C215600200005 PART-DET (DG) C215600200006 SAMPLE (42-MO-100,ENR=0.9742) C215600200007 DETECTOR (HPGE) Ortec model GEM35P4-S. C215600200008 METHOD (ACTIV,GSPEC) Long irradiation on Mo-100. The C215600200009 production of 99Mo was quantified via gamma-ray C215600200010 spectrometry using a high purity germanium (HPGe) C215600200011 detector. C215600200012 ERR-ANALYS (ERR-T) Total uncertainty C215600200013 (ERR-S,,2.5) Maximum weighted counting error. C215600200014 (ERR-1) HPGe efficiency. C215600200015 (ERR-2) Nuclear decay data. C215600200016 (ERR-3) Relative foil thickness. C215600200017 (ERR-4) Beam current. C215600200018 STATUS (TABLE) Table 3, page 913. C215600200019 ENDBIB 17 0 C215600200020 COMMON 4 3 C215600200021 ERR-1 ERR-2 ERR-3 ERR-4 C215600200022 PER-CENT PER-CENT PER-CENT PER-CENT C215600200023 5.0 1.0 5.0 5.0 C215600200024 ENDCOMMON 3 0 C215600200025 DATA 4 8 C215600200026 EN EN-RSL DATA ERR-T C215600200027 MEV MEV MB MB C215600200028 10.0 0.1 0.264 0.036 C215600200029 11.3 0.1 3.140 0.280 C215600200030 12.5 0.1 9.890 0.870 C215600200031 13.5 0.2 20.300 1.800 C215600200032 14.6 0.2 35.700 3.100 C215600200033 15.6 0.2 52.100 4.600 C215600200034 16.6 0.2 74.100 6.500 C215600200035 17.5 0.2 87.900 7.700 C215600200036 ENDDATA 10 0 C215600200037 ENDSUBENT 36 0 C215600299999 SUBENT C2156003 20150310 C148C215600300001 BIB 8 18 C215600300002 REACTION (42-MO-100(P,X)42-MO-99,(CUM),SIG) C215600300003 DECAY-DATA (42-MO-99,65.94HR,DG,140.511,0.0452, C215600300004 DG,181.068,0.0599, C215600300005 DG,739.500,0.1213) C215600300006 PART-DET (DG) C215600300007 SAMPLE (42-MO-100,ENR=0.9742) C215600300008 DETECTOR (HPGE) Ortec model GEM35P4-S. C215600300009 METHOD (ACTIV,GSPEC) Short irradiation on Mo-100. The C215600300010 production of 99Mo was quantified via gamma-ray C215600300011 spectrometry using a high purity germanium (HPGe) C215600300012 detector. C215600300013 ERR-ANALYS (ERR-T) Total uncertainty C215600300014 (ERR-S,,2.5) Maximum weighted counting error. C215600300015 (ERR-1) HPGe efficiency. C215600300016 (ERR-2) Nuclear decay data. C215600300017 (ERR-3) Relative foil thickness. C215600300018 (ERR-4) Beam current. C215600300019 STATUS (TABLE) Table 3, page 913. C215600300020 ENDBIB 18 0 C215600300021 COMMON 4 3 C215600300022 ERR-1 ERR-2 ERR-3 ERR-4 C215600300023 PER-CENT PER-CENT PER-CENT PER-CENT C215600300024 5.0 1.0 5.0 5.0 C215600300025 ENDCOMMON 3 0 C215600300026 DATA 4 11 C215600300027 EN EN-RSL DATA ERR-T C215600300028 MEV MEV MB MB C215600300029 10.9 0.6 2.470 0.220 C215600300030 11.9 0.2 5.810 0.510 C215600300031 12.9 0.5 14.100 1.200 C215600300032 14.0 0.2 24.100 2.100 C215600300033 14.0 0.2 26.400 2.300 C215600300034 15.0 0.2 39.300 3.400 C215600300035 16.3 0.2 62.700 5.500 C215600300036 17.0 0.3 76.000 6.600 C215600300037 17.2 0.8 79.700 7.000 C215600300038 17.6 0.8 85.400 7.500 C215600300039 17.8 0.4 98.100 8.600 C215600300040 ENDDATA 13 0 C215600300041 ENDSUBENT 40 0 C215600399999 SUBENT C2156004 20150310 C148C215600400001 BIB 8 18 C215600400002 REACTION (42-MO-100(P,X)42-MO-99,(CUM),SIG) C215600400003 DECAY-DATA (42-MO-99,65.94HR,DG,140.511,0.0452, C215600400004 DG,181.068,0.0599, C215600400005 DG,739.500,0.1213) C215600400006 PART-DET (DG) C215600400007 SAMPLE Natural molybdenum. C215600400008 DETECTOR (HPGE) Ortec model GEM35P4-S. C215600400009 METHOD (ACTIV,GSPEC) Short irradiation on Mo-0. The C215600400010 production of 99Mo was quantified via gamma-ray C215600400011 spectrometry using a high purity germanium (HPGe) C215600400012 detector. C215600400013 ERR-ANALYS (ERR-T) Total uncertainty C215600400014 (ERR-S,,2.5) Maximum weighted counting error. C215600400015 (ERR-1) HPGe efficiency. C215600400016 (ERR-2) Nuclear decay data. C215600400017 (ERR-3) Relative foil thickness. C215600400018 (ERR-4) Beam current. C215600400019 STATUS (TABLE) Table 3, page 913. C215600400020 ENDBIB 18 0 C215600400021 COMMON 4 3 C215600400022 ERR-1 ERR-2 ERR-3 ERR-4 C215600400023 PER-CENT PER-CENT PER-CENT PER-CENT C215600400024 5.0 1.0 5.0 5.0 C215600400025 ENDCOMMON 3 0 C215600400026 DATA 4 6 C215600400027 EN EN-RSL DATA ERR-T C215600400028 MEV MEV MB MB C215600400029 12.7 0.3 10.300 6.200 C215600400030 14.0 0.3 18.700 5.400 C215600400031 15.1 0.4 37.700 6.000 C215600400032 16.3 0.5 55.100 7.600 C215600400033 17.4 0.7 71.800 9.600 C215600400034 17.9 0.8 82.000 10.000 C215600400035 ENDDATA 8 0 C215600400036 ENDSUBENT 35 0 C215600499999 SUBENT C2156005 20150310 C148C215600500001 BIB 8 16 C215600500002 REACTION (42-MO-100(P,2N)43-TC-99-M,,SIG) C215600500003 DECAY-DATA (43-TC-99-M,6.01HR,DG,140.511,0.8908) C215600500004 PART-DET (DG) C215600500005 SAMPLE (42-MO-100,ENR=0.9742) C215600500006 DETECTOR (HPGE) Ortec model GEM35P4-S. C215600500007 METHOD (ACTIV,GSPEC) Long irradiation on Mo-100. The C215600500008 production of Tc-99m was quantified via gamma-ray C215600500009 spectrometry using a high purity germanium (HPGe) C215600500010 detector. C215600500011 ERR-ANALYS (ERR-T) Total uncertainty C215600500012 (ERR-S,,2.5) Maximum weighted counting error. C215600500013 (ERR-1) HPGe efficiency. C215600500014 (ERR-2) Nuclear decay data. C215600500015 (ERR-3) Relative foil thickness. C215600500016 (ERR-4) Beam current. C215600500017 STATUS (TABLE) Table 3, page 913. C215600500018 ENDBIB 16 0 C215600500019 COMMON 4 3 C215600500020 ERR-1 ERR-2 ERR-3 ERR-4 C215600500021 PER-CENT PER-CENT PER-CENT PER-CENT C215600500022 5.0 1.0 5.0 5.0 C215600500023 ENDCOMMON 3 0 C215600500024 DATA 4 9 C215600500025 EN EN-RSL DATA ERR-T C215600500026 MEV MEV MB MB C215600500027 8.5 0.1 37.0 3.0 C215600500028 10.0 0.1 173.0 15.0 C215600500029 11.3 0.1 252.0 22.0 C215600500030 12.5 0.1 282.0 25.0 C215600500031 13.5 0.2 276.0 24.0 C215600500032 14.6 0.2 288.0 25.0 C215600500033 15.6 0.2 293.0 26.0 C215600500034 16.6 0.2 307.0 27.0 C215600500035 17.5 0.2 293.0 26.0 C215600500036 ENDDATA 11 0 C215600500037 ENDSUBENT 36 0 C215600599999 SUBENT C2156006 20150310 C148C215600600001 BIB 8 16 C215600600002 REACTION (42-MO-100(P,2N)43-TC-99-M,,SIG) C215600600003 DECAY-DATA (43-TC-99-M,6.01HR,DG,140.511,0.8908) C215600600004 PART-DET (DG) C215600600005 SAMPLE (42-MO-100,ENR=0.9742) C215600600006 DETECTOR (HPGE) Ortec model GEM35P4-S. C215600600007 METHOD (ACTIV,GSPEC) Short irradiation on Mo-100. The C215600600008 production of 99Mo was quantified via gamma-ray C215600600009 spectrometry using a high purity germanium (HPGe) C215600600010 detector. C215600600011 ERR-ANALYS (ERR-T) Total uncertainty C215600600012 (ERR-S,,2.5) Maximum weighted counting error. C215600600013 (ERR-1) HPGe efficiency. C215600600014 (ERR-2) Nuclear decay data. C215600600015 (ERR-3) Relative foil thickness. C215600600016 (ERR-4) Beam current. C215600600017 STATUS (TABLE) Table 3, page 913. C215600600018 ENDBIB 16 0 C215600600019 COMMON 4 3 C215600600020 ERR-1 ERR-2 ERR-3 ERR-4 C215600600021 PER-CENT PER-CENT PER-CENT PER-CENT C215600600022 5.0 1.0 5.0 5.0 C215600600023 ENDCOMMON 3 0 C215600600024 DATA 4 11 C215600600025 EN EN-RSL DATA ERR-T C215600600026 MEV MEV MB MB C215600600027 10.9 0.6 254.0 22.0 C215600600028 11.9 0.2 270.0 24.0 C215600600029 12.9 0.5 299.0 26.0 C215600600030 14.0 0.2 283.0 25.0 C215600600031 14.0 0.2 312.0 27.0 C215600600032 15.0 0.2 294.0 26.0 C215600600033 16.3 0.2 310.0 27.0 C215600600034 17.0 0.3 281.0 24.0 C215600600035 17.2 0.8 266.0 23.0 C215600600036 17.6 0.8 249.0 22.0 C215600600037 17.8 0.4 315.0 27.0 C215600600038 ENDDATA 13 0 C215600600039 ENDSUBENT 38 0 C215600699999 SUBENT C2156007 20150310 C148C215600700001 BIB 8 16 C215600700002 REACTION (42-MO-100(P,2N)43-TC-99-M,,SIG) C215600700003 DECAY-DATA (43-TC-99-M,6.01HR,DG,140.511,0.8908) C215600700004 PART-DET (DG) C215600700005 SAMPLE Natural molybdenum. C215600700006 DETECTOR (HPGE) Ortec model GEM35P4-S. C215600700007 METHOD (ACTIV,GSPEC) Short irradiation on Mo-0. The C215600700008 production of 99Mo was quantified via gamma-ray C215600700009 spectrometry using a high purity germanium (HPGe) C215600700010 detector. C215600700011 ERR-ANALYS (ERR-T) Total uncertainty C215600700012 (ERR-S,,2.5) Maximum weighted counting error. C215600700013 (ERR-1) HPGe efficiency. C215600700014 (ERR-2) Nuclear decay data. C215600700015 (ERR-3) Relative foil thickness. C215600700016 (ERR-4) Beam current. C215600700017 STATUS (TABLE) Table 3, page 913. C215600700018 ENDBIB 16 0 C215600700019 COMMON 4 3 C215600700020 ERR-1 ERR-2 ERR-3 ERR-4 C215600700021 PER-CENT PER-CENT PER-CENT PER-CENT C215600700022 5.0 1.0 5.0 5.0 C215600700023 ENDCOMMON 3 0 C215600700024 DATA 4 11 C215600700025 EN EN-RSL DATA ERR-T C215600700026 MEV MEV MB MB C215600700027 8.0 0.2 11.3 1.2 C215600700028 8.9 0.4 94.1 8.3 C215600700029 10.0 0.2 176.0 15.0 C215600700030 10.5 0.6 236.0 21.0 C215600700031 12.0 0.3 271.0 24.0 C215600700032 12.7 0.3 262.0 23.0 C215600700033 14.0 0.3 293.0 26.0 C215600700034 15.1 0.4 305.0 27.0 C215600700035 16.3 0.5 286.0 25.0 C215600700036 17.4 0.7 273.0 24.0 C215600700037 17.9 0.8 250.0 22.0 C215600700038 ENDDATA 13 0 C215600700039 ENDSUBENT 38 0 C215600799999 SUBENT C2156008 20150310 C148C215600800001 BIB 7 20 C215600800002 REACTION (42-MO-100(P,2N)43-TC-99-G,,SIG) C215600800003 PART-DET (DG,B-) C215600800004 SAMPLE (42-MO-100,ENR=0.9742) C215600800005 DETECTOR (HPGE,SCIN) Ortec model GEM35P4-S. C215600800006 METHOD (ACTIV,GSPEC,CHSEP) Long irradiation on Mo-100. The C215600800007 direct 99gTc excitation function was thus determined C215600800008 using liquid scintillation counting and inductively C215600800009 coupled plasma mass spectrometry (ICP-MS)in C215600800010 combination with gamma- ray spectrometry to correct C215600800011 for the indirect 99gTc contributions following decay C215600800012 of 99mTc and 99Mo. C215600800013 ERR-ANALYS (ERR-T) Total uncertainty C215600800014 (ERR-S,,2.5) Maximum weighted counting error. C215600800015 (ERR-1) Nuclear decay data error. C215600800016 (ERR-2,1.,5.) Extraction efficiency error. C215600800017 (ERR-3) ICP-MS calibration error. C215600800018 (ERR-4,,1.) Three ICP-MS replicate readings. C215600800019 (ERR-5) Relative foil thickness. C215600800020 (ERR-6) Beam current. C215600800021 STATUS (TABLE) Table 3, page 913. C215600800022 ENDBIB 20 0 C215600800023 COMMON 4 3 C215600800024 ERR-1 ERR-3 ERR-5 ERR-6 C215600800025 PER-CENT PER-CENT PER-CENT PER-CENT C215600800026 1.0 8.0 5.0 5.0 C215600800027 ENDCOMMON 3 0 C215600800028 DATA 4 9 C215600800029 EN EN-RSL DATA ERR-T C215600800030 MEV MEV MB MB C215600800031 8.5 0.1 92.0 14.0 C215600800032 10.0 0.1 317.0 46.0 C215600800033 11.3 0.1 536.0 79.0 C215600800034 12.5 0.1 681.0 92.0 C215600800035 13.5 0.2 630.0 90.0 C215600800036 14.6 0.2 689.0 97.0 C215600800037 15.6 0.2 749.0 107.0 C215600800038 16.6 0.2 807.0 112.0 C215600800039 17.5 0.2 812.0 112.0 C215600800040 ENDDATA 11 0 C215600800041 ENDSUBENT 40 0 C215600899999 ENDENTRY 8 0 C215699999999