ENTRY D4138 20190824 D121D413800000001 SUBENT D4138001 20190824 D121D413800100001 BIB 12 41 D413800100002 TITLE Experimental cross section for charged particle D413800100003 production of the therapeutic radionuclide 111Ag and D413800100004 its PET imaging analogue 104m,gAg. D413800100005 AUTHOR (A.Hermanne,S.Takacs,F.Tarkanyi,R.Bolbos) D413800100006 INSTITUTE (2BLGVUB,3HUNDEB) D413800100007 FACILITY (CYCLO,2BLGVUB) CGR 560 cyclotron of the VUB, Belgium D413800100008 REFERENCE (J,NIM/B,217,193,2004) D413800100009 SAMPLE The samples were elemental high purity natural Pd foilsD413800100010 12.14 and 7.99 micrometers from Goodfellow. D413800100011 METHOD (ACTIV,EXTB,STTA,GSPEC) Stacked target technique was D413800100012 used. Two stacks were irradiated with 20.5 and 15.1 MeVD413800100013 deuterons and three stacks with protons at 37.3, 28.5, D413800100014 and 15.9 MeV. The thickness of the foils was determinedD413800100015 by weighing the original metal sheet. High purity Ti, D413800100016 Cu and Ni monitor foils were inserted in to the stacks.D413800100017 Beam current was measured in Faraday cup and checked D413800100018 by monitor reactions. (200nA for 0.5 h). Activity was D413800100019 measured without chemical separation. The beam energy D413800100020 was determined by TOF. The energy degradation was D413800100021 calculated by using the polynomial approximation of D413800100022 Andersen (see REL-REF). Nuclear data were taken from D413800100023 the Lund ENSDF data file. D413800100024 REL-REF (R,,H.H.Andersen+,B,ANDERSEN,3,,1997) - The energy D413800100025 degradation was calculated using tables from this D413800100026 article. D413800100027 DETECTOR (HPGE) HPGe gamma detectors D413800100028 MONITOR (22-TI-0(D,X)23-V-48,,SIG) D413800100029 (22-TI-0(P,X)23-V-48,,SIG) D413800100030 (29-CU-0(P,X)30-ZN-62,,SIG) D413800100031 (29-CU-0(P,X)30-ZN-65,,SIG) D413800100032 (28-NI-0(P,X)28-NI-57,,SIG) D413800100033 MONIT-REF (,F.Tarkanyi+,R,IAEA-TECDOC-1211,49,2001) chapter 4 D413800100034 (,S.Takacs+,J,NIM/B,188,106,2002) D413800100035 (,S.Takacs+,J,NIM/B,174,235,2001) D413800100036 HISTORY (20040317C) TS D413800100037 (20040831A) OS. Reaction coding in Subents 8,9 modifiedD413800100038 and ERR-ANALYS moved to subentries. D413800100039 (20060727A) Ref.in MONIT-REF corrected. D413800100040 (20190824A) SD: REACTION code updated according to new D413800100041 EXFOR rules in Subents 006-007. REL-REF updated. SmallD413800100042 corrections in all Subents. D413800100043 ENDBIB 41 0 D413800100044 NOCOMMON 0 0 D413800100045 ENDSUBENT 44 0 D413800199999 SUBENT D4138002 20190824 D121D413800200001 BIB 5 15 D413800200002 REACTION (46-PD-110(D,N)47-AG-111,,SIG) D413800200003 DECAY-DATA (47-AG-111-G,7.45D,DG,345.4,0.0133, D413800200004 DG,342.1,0.067) D413800200005 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam 0.2 MeV. D413800200006 (ERR-T) Total errors were given. Correction of the beamD413800200007 was made using the monitor reactions. D413800200008 Contributing errors: D413800200009 (ERR-1) uncertainty in number of target nuclei 5% D413800200010 (ERR-2) uncertainty in beam intensity 3% D413800200011 (ERR-3) uncertainty in detector efficiency 5% D413800200012 (ERR-4,1.,5.) uncertainty in peak area and D413800200013 statistical error 1-5% D413800200014 (ERR-5,1.,5.) uncertainty in nuclear data 1-5% D413800200015 STATUS (TABLE) Table 2. from Nucl.Instr.Meth.,B217(2004)193 D413800200016 HISTORY (20190824U) SD: ERR-ANALYS, STATUS updated. D413800200017 ENDBIB 15 0 D413800200018 COMMON 3 3 D413800200019 ERR-1 ERR-2 ERR-3 D413800200020 PER-CENT PER-CENT PER-CENT D413800200021 5. 3. 5. D413800200022 ENDCOMMON 3 0 D413800200023 DATA 4 17 D413800200024 EN EN-ERR DATA ERR-T D413800200025 MEV MEV MB MB D413800200026 20.3 0.2 14.0 14.0 D413800200027 19.3 0.2 155.0 15.0 D413800200028 18.1 0.3 165.0 16.0 D413800200029 17.0 0.3 190.0 19.0 D413800200030 15.8 0.4 196.0 20.0 D413800200031 15.0 0.2 200.0 20.0 D413800200032 14.5 0.4 204.0 19.0 D413800200033 13.8 0.2 222.0 20.0 D413800200034 13.2 0.5 213.0 20.0 D413800200035 12.6 0.3 243.0 18.0 D413800200036 11.8 0.6 280.0 20.0 D413800200037 11.4 0.4 264.0 21.0 D413800200038 10.0 0.5 297.0 23.0 D413800200039 9.5 0.5 305.0 24.0 D413800200040 7.6 0.6 306.0 25.0 D413800200041 6.7 0.7 271.0 24.0 D413800200042 5.8 0.7 194.0 19.0 D413800200043 ENDDATA 19 0 D413800200044 ENDSUBENT 43 0 D413800299999 SUBENT D4138003 20190824 D121D413800300001 BIB 5 17 D413800300002 REACTION (46-PD-110(D,2N)47-AG-110-M,,SIG) D413800300003 DECAY-DATA (47-AG-110-M,249.8D,DG,657.8,0.946, D413800300004 DG,763.9,0.221, D413800300005 DG,884.7,0.722, D413800300006 DG,937.5,0.341) D413800300007 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam 0.2 MeV. D413800300008 (ERR-T) Total errors were given. Correction of the beamD413800300009 was made using the monitor reactions. D413800300010 Contributing errors: D413800300011 (ERR-1) uncertainty in number of target nuclei 5% D413800300012 (ERR-2) uncertainty in beam intensity 3% D413800300013 (ERR-3) uncertainty in detector efficiency 5% D413800300014 (ERR-4,1.,5.) uncertainty in peak area and D413800300015 statistical error 1-5% D413800300016 (ERR-5,1.,5.) uncertainty in nuclear data 1-5% D413800300017 STATUS (TABLE) Table 2. from Nucl.Instr.Meth.,B217(2004)193 D413800300018 HISTORY (20190824U) SD: ERR-ANALYS, STATUS updated. D413800300019 ENDBIB 17 0 D413800300020 COMMON 3 3 D413800300021 ERR-1 ERR-2 ERR-3 D413800300022 PER-CENT PER-CENT PER-CENT D413800300023 5. 3. 5. D413800300024 ENDCOMMON 3 0 D413800300025 DATA 4 17 D413800300026 EN EN-ERR DATA ERR-T D413800300027 MEV MEV MB MB D413800300028 20.3 0.2 122.0 12.0 D413800300029 19.3 0.2 153.0 15.0 D413800300030 18.1 0.3 186.0 18.0 D413800300031 17.0 0.3 261.0 20.0 D413800300032 15.8 0.4 308.0 22.0 D413800300033 15.0 0.2 314.0 21.0 D413800300034 14.5 0.4 311.0 21.0 D413800300035 13.8 0.2 339.0 22.0 D413800300036 13.2 0.5 330.0 22.0 D413800300037 12.6 0.3 313.0 21.0 D413800300038 11.8 0.6 343.0 23.0 D413800300039 11.4 0.4 306.0 22.0 D413800300040 10.0 0.5 218.0 22.0 D413800300041 9.5 0.5 127.0 16.0 D413800300042 7.6 0.6 82.0 11.0 D413800300043 6.7 0.7 44.0 6.0 D413800300044 5.8 0.7 16.0 3.0 D413800300045 ENDDATA 19 0 D413800300046 ENDSUBENT 45 0 D413800399999 SUBENT D4138004 20190824 D121D413800400001 BIB 5 20 D413800400002 REACTION (46-PD-0(D,X)47-AG-104-G,M+,SIG) D413800400003 DECAY-DATA (47-AG-104-G,69.2MIN,DG,555.8,0.926, D413800400004 DG,767.7,0.657, D413800400005 DG,858.,0.104, D413800400006 DG,941.7,0.25, D413800400007 DG,1341.7,.073) D413800400008 (47-AG-104-M,33.5MIN,DG,555.8,0.91, D413800400009 DG,1238.0,0.0387) D413800400010 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam 0.2 MeV. D413800400011 (ERR-T) Total errors were given. Correction of the beamD413800400012 was made using the monitor reactions. D413800400013 Contributing errors: D413800400014 (ERR-1) uncertainty in number of target nuclei 5% D413800400015 (ERR-2) uncertainty in beam intensity 3% D413800400016 (ERR-3) uncertainty in detector efficiency 5% D413800400017 (ERR-4,1.,5.) uncertainty in peak area and D413800400018 statistical error 1-5% D413800400019 (ERR-5,1.,5.) uncertainty in nuclear data 1-5% D413800400020 STATUS (TABLE) Table 2. from Nucl.Instr.Meth.,B217(2004)193 D413800400021 HISTORY (20190824U) SD: ERR-ANALYS, STATUS updated. D413800400022 ENDBIB 20 0 D413800400023 COMMON 3 3 D413800400024 ERR-1 ERR-2 ERR-3 D413800400025 PER-CENT PER-CENT PER-CENT D413800400026 5. 3. 5. D413800400027 ENDCOMMON 3 0 D413800400028 DATA 4 16 D413800400029 EN EN-ERR DATA ERR-T D413800400030 MEV MEV MB MB D413800400031 20.3 0.2 128.0 13.0 D413800400032 19.3 0.2 121.0 12.0 D413800400033 18.1 0.3 101.0 13.0 D413800400034 17.0 0.3 88.0 10.0 D413800400035 15.8 0.4 68.0 9.0 D413800400036 15.0 0.2 63.0 9.0 D413800400037 14.5 0.4 56.0 8.0 D413800400038 13.8 0.2 59.0 8.0 D413800400039 13.2 0.5 50.0 7.0 D413800400040 12.6 0.3 45.0 6.0 D413800400041 11.8 0.6 46.0 7.0 D413800400042 11.4 0.4 38.0 6.0 D413800400043 10.0 0.5 25.0 4.0 D413800400044 9.5 0.5 9.0 2.0 D413800400045 7.6 0.6 3.0 1.0 D413800400046 6.7 0.7 0.5 0.3 D413800400047 ENDDATA 18 0 D413800400048 ENDSUBENT 47 0 D413800499999 SUBENT D4138005 20190824 D121D413800500001 BIB 5 20 D413800500002 REACTION (46-PD-0(P,X)47-AG-104-G,M+,SIG) D413800500003 DECAY-DATA (47-AG-104-G,69.2MIN,DG,555.8,0.926, D413800500004 DG,767.7,0.657, D413800500005 DG,858.,0.104, D413800500006 DG,941.7,0.25, D413800500007 DG,1341.7,.073) D413800500008 (47-AG-104-M,33.5MIN,DG,555.8,0.91, D413800500009 DG,1238.0,0.0387) D413800500010 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam 0.2 MeV. D413800500011 (ERR-T) Total errors were given. Correction of the beamD413800500012 was made using the monitor reactions. D413800500013 Contributing errors: D413800500014 (ERR-1) uncertainty in number of target nuclei 5% D413800500015 (ERR-2) uncertainty in beam intensity 3% D413800500016 (ERR-3) uncertainty in detector efficiency 5% D413800500017 (ERR-4,1.,5.) uncertainty in peak area and D413800500018 statistical error 1-5% D413800500019 (ERR-5,1.,5.) uncertainty in nuclear data 1-5% D413800500020 STATUS (TABLE) Table 2. from Nucl.Instr.Meth.,B217(2004)193 D413800500021 HISTORY (20190824U) SD: ERR-ANALYS, STATUS updated. D413800500022 ENDBIB 20 0 D413800500023 COMMON 3 3 D413800500024 ERR-1 ERR-2 ERR-3 D413800500025 PER-CENT PER-CENT PER-CENT D413800500026 5. 3. 5. D413800500027 ENDCOMMON 3 0 D413800500028 DATA 4 36 D413800500029 EN EN-ERR DATA ERR-T D413800500030 MEV MEV MB MB D413800500031 37.0 0.2 134.0 11.0 D413800500032 36.2 0.2 144.0 12.0 D413800500033 35.4 0.3 166.0 13.0 D413800500034 34.5 0.3 154.0 12.0 D413800500035 32.7 0.3 157.0 12.0 D413800500036 31.9 0.4 173.0 14.0 D413800500037 30.9 0.4 179.0 14.0 D413800500038 30.0 0.5 184.0 15.0 D413800500039 29.0 0.5 174.0 14.0 D413800500040 28.2 0.2 152.0 12.0 D413800500041 28.0 0.6 163.0 13.0 D413800500042 27.0 0.7 138.0 11.0 D413800500043 26.6 0.2 149.0 12.0 D413800500044 25.9 0.7 154.0 13.0 D413800500045 25.0 0.3 139.0 11.0 D413800500046 24.8 0.8 129.0 10.0 D413800500047 23.7 0.3 134.0 11.0 D413800500048 23.7 0.8 126.0 10.0 D413800500049 22.5 0.9 148.0 13.0 D413800500050 22.5 0.4 131.0 12.0 D413800500051 21.4 0.9 148.0 13.0 D413800500052 21.1 0.4 140.0 13.0 D413800500053 20.1 1.0 148.0 13.0 D413800500054 19.7 0.5 138.0 12.0 D413800500055 18.6 0.6 130.0 12.0 D413800500056 16.5 0.6 118.0 9.0 D413800500057 15.9 0.7 110.0 9.0 D413800500058 15.8 0.2 117.0 9.0 D413800500059 14.9 0.3 104.0 9.0 D413800500060 14.0 0.3 84.0 8.0 D413800500061 13.0 0.4 46.0 5.0 D413800500062 11.9 0.5 40.0 4.0 D413800500063 10.8 0.5 34.0 3.0 D413800500064 9.5 0.6 23.0 3.0 D413800500065 8.2 0.6 15.0 2.0 D413800500066 6.7 0.7 6.9 1.0 D413800500067 ENDDATA 38 0 D413800500068 ENDSUBENT 67 0 D413800599999 SUBENT D4138006 20190824 D121D413800600001 BIB 5 6 D413800600002 REACTION (46-PD-110(D,N)47-AG-111,,TTY,,PHY,DERIV) D413800600003 ANALYSIS (INTEF) Derived from measured excitation function D413800600004 ERR-ANALYS No information D413800600005 STATUS (TABLE) Table 3 from Nucl.Instr.Meth.,B217(2004)193 D413800600006 HISTORY (20190824A) SD: SF9=CALC -> DERIV in REACTION code. D413800600007 STATUS updated. ANALYSIS added. D413800600008 ENDBIB 6 0 D413800600009 NOCOMMON 0 0 D413800600010 DATA 2 33 D413800600011 EN DATA D413800600012 MEV GBQ/COUL D413800600013 4.5 0.0 D413800600014 5.5 0.1 D413800600015 6.0 0.1 D413800600016 6.5 0.2 D413800600017 7.0 0.3 D413800600018 7.5 0.4 D413800600019 8.0 0.5 D413800600020 8.5 0.7 D413800600021 9.0 0.8 D413800600022 9.5 1.0 D413800600023 10.0 1.1 D413800600024 10.5 1.3 D413800600025 11.0 1.4 D413800600026 11.5 1.6 D413800600027 12.0 1.7 D413800600028 12.5 1.9 D413800600029 13.0 2.0 D413800600030 13.5 2.2 D413800600031 14.0 2.3 D413800600032 14.5 2.4 D413800600033 15.0 2.6 D413800600034 15.5 2.7 D413800600035 16.0 2.8 D413800600036 16.5 3.0 D413800600037 17.0 3.1 D413800600038 17.5 3.3 D413800600039 18.0 3.4 D413800600040 18.5 3.5 D413800600041 19.0 3.6 D413800600042 19.5 3.8 D413800600043 19.6 3.9 D413800600044 20.0 4.0 D413800600045 20.1 4.0 D413800600046 ENDDATA 35 0 D413800600047 ENDSUBENT 46 0 D413800699999 SUBENT D4138007 20190824 D121D413800700001 BIB 5 6 D413800700002 REACTION (46-PD-110(D,2N)47-AG-110-M,,TTY,,PHY,DERIV) D413800700003 ANALYSIS (INTEF) Derived from measured excitation function D413800700004 ERR-ANALYS No information D413800700005 STATUS (TABLE) Table 3 from Nucl.Instr.Meth.,B217(2004)193 D413800700006 HISTORY (20190824A) SD: SF9=CALC -> DERIV in REACTION code. D413800700007 STATUS updated. ANALYSIS added. D413800700008 ENDBIB 6 0 D413800700009 NOCOMMON 0 0 D413800700010 DATA 2 33 D413800700011 EN DATA D413800700012 MEV MBQ/COUL D413800700013 4.5 0.0 D413800700014 5.5 0.1 D413800700015 6.0 0.3 D413800700016 6.5 0.6 D413800700017 7.0 1.1 D413800700018 7.5 1.9 D413800700019 8.0 3.0 D413800700020 8.5 4.4 D413800700021 9.0 6.3 D413800700022 9.5 8.5 D413800700023 10.0 11.0 D413800700024 10.5 15.0 D413800700025 11.0 19.0 D413800700026 11.5 24.0 D413800700027 12.0 29.0 D413800700028 12.5 34.0 D413800700029 13.0 40.0 D413800700030 13.5 47.0 D413800700031 14.0 53.0 D413800700032 14.5 60.0 D413800700033 15.0 66.0 D413800700034 15.5 72.0 D413800700035 16.0 79.0 D413800700036 16.5 85.0 D413800700037 17.0 90.0 D413800700038 17.5 96.0 D413800700039 18.0 100.0 D413800700040 18.5 105.0 D413800700041 19.0 109.0 D413800700042 19.5 113.0 D413800700043 19.6 113.0 D413800700044 20.0 116.0 D413800700045 20.1 117.0 D413800700046 ENDDATA 35 0 D413800700047 ENDSUBENT 46 0 D413800799999 SUBENT D4138008 20190824 D121D413800800001 BIB 5 6 D413800800002 REACTION (46-PD-0(D,X)47-AG-104-G,,TTY,,PHY,DERIV) D413800800003 ANALYSIS (INTEF) Derived from measured excitation function D413800800004 ERR-ANALYS No information D413800800005 STATUS (TABLE) Table 3 from Nucl.Instr.Meth.,B217(2004)193 D413800800006 HISTORY (20190824A) SD: SF9=CALC -> DERIV in REACTION code. D413800800007 STATUS updated. ANALYSIS added. D413800800008 ENDBIB 6 0 D413800800009 NOCOMMON 0 0 D413800800010 DATA 2 33 D413800800011 EN DATA D413800800012 MEV GBQ/COUL D413800800013 4.5 0.0 D413800800014 5.5 0.0 D413800800015 6.0 0.0 D413800800016 6.5 0.0 D413800800017 7.0 0.0 D413800800018 7.5 0.0 D413800800019 8.0 0.1 D413800800020 8.5 0.4 D413800800021 9.0 0.9 D413800800022 9.5 1.7 D413800800023 10.0 2.9 D413800800024 10.5 4.4 D413800800025 11.0 6.3 D413800800026 11.5 8.7 D413800800027 12.0 12.0 D413800800028 12.5 15.0 D413800800029 13.0 19.0 D413800800030 13.5 23.0 D413800800031 14.0 28.0 D413800800032 14.5 34.0 D413800800033 15.0 40.0 D413800800034 15.5 47.0 D413800800035 16.0 54.0 D413800800036 16.5 63.0 D413800800037 17.0 72.0 D413800800038 17.5 82.0 D413800800039 18.0 92.0 D413800800040 18.5 104.0 D413800800041 19.0 116.0 D413800800042 19.5 130.0 D413800800043 19.6 144.0 D413800800044 20.0 160.0 D413800800045 20.1 163.0 D413800800046 ENDDATA 35 0 D413800800047 ENDSUBENT 46 0 D413800899999 SUBENT D4138009 20190824 D121D413800900001 BIB 5 6 D413800900002 REACTION (46-PD-0(P,X)47-AG-104-G,,TTY,,PHY,DERIV) D413800900003 ANALYSIS (INTEF) Derived from measured excitation function D413800900004 ERR-ANALYS No information D413800900005 STATUS (TABLE) Table 3 from Nucl.Instr.Meth.,B217(2004)193 D413800900006 HISTORY (20190824A) SD: SF9=CALC -> DERIV in REACTION code. D413800900007 STATUS updated. ANALYSIS added. D413800900008 ENDBIB 6 0 D413800900009 NOCOMMON 0 0 D413800900010 DATA 2 32 D413800900011 EN DATA D413800900012 MEV GBQ/COUL D413800900013 6.0 0.1 D413800900014 7.0 0.6 D413800900015 8.0 2.9 D413800900016 9.0 6.7 D413800900017 10.0 12.0 D413800900018 11.0 20.0 D413800900019 12.0 31.0 D413800900020 13.0 45.0 D413800900021 14.0 66.0 D413800900022 15.0 94.0 D413800900023 16.0 129.0 D413800900024 17.0 171.0 D413800900025 18.0 218.0 D413800900026 19.0 271.0 D413800900027 20.0 327.0 D413800900028 21.0 387.0 D413800900029 22.0 448.0 D413800900030 23.0 511.0 D413800900031 24.0 577.0 D413800900032 25.0 645.0 D413800900033 26.0 717.0 D413800900034 27.0 795.0 D413800900035 28.0 879.0 D413800900036 29.0 969.0 D413800900037 30.0 1065.0 D413800900038 31.0 1165.0 D413800900039 32.0 1267.0 D413800900040 33.0 1370.0 D413800900041 34.0 1473.0 D413800900042 35.0 1573.0 D413800900043 36.0 1671.0 D413800900044 36.9 1756.0 D413800900045 ENDDATA 34 0 D413800900046 ENDSUBENT 45 0 D413800999999 ENDENTRY 9 0 D413899999999