ENTRY D4154 20210929 D132D415400000001 SUBENT D4154001 20210929 D132D415400100001 BIB 13 44 D415400100002 TITLE Cross sections for production of the therapeutic D415400100003 radioisotopes 198Au and 199Au in proton and deuteron D415400100004 induced reactions on 198Pt D415400100005 AUTHOR (F.Tarkanyi,A.Hermanne,S.Takacs,Yu.N.Shubin,A.I.Dityuk)D415400100006 INSTITUTE (2BLGVUB,3HUNDEB,4RUSFEI) D415400100007 REFERENCE (J,RCA,92,223,2004) D415400100008 FACILITY (CYCLO,2BLGVUB) CGR 560 cyclotron of Brussels D415400100009 SAMPLE Targets were high purity natural Pt foils of 26.6 and D415400100010 29.7 microns for protons and 12.05 microns for deuteronD415400100011 from GoodFellow. D415400100012 METHOD (ACTIV,EXTB,STTA,GSPEC) D415400100013 Stacked target technique was used. Initial energies: D415400100014 37.9 and 22.5 MeV for protons and 21.0 and 15.1 MeV forD415400100015 deuterons. D415400100016 Al, Ti, Cu and Ni were used as monitor and energy D415400100017 degrader foils. D415400100018 Beam intensity was 200nA and was also measured in D415400100019 Faraday cup. The bombarding energy was determined by D415400100020 TOF method. Irradiation time was 10-30 min. D415400100021 High resolution gamma spectrometry was applied without D415400100022 chemical separation. Spectra were measured after few D415400100023 hours of EOB. D415400100024 Energy scale and beam intensity along the stacks were D415400100025 corrected according to the applied monitor reactions. D415400100026 REL-REF Guide to Expression of Uncertainty in Measurement. D415400100027 International Organisation for Standardization, D415400100028 Geneva (1993) (ISBN 92-67-10188-9). D415400100029 (R,,H.H.Andersen+,B,ANDERSEN,,,1997) - The energy D415400100030 degradation was calculated using tables from this D415400100031 article. D415400100032 (R,,R.B.Firestone,B,FIRESTONE,,,1996) Decay data were D415400100033 taken from this article. D415400100034 DETECTOR (HPGE) D415400100035 MONITOR (22-TI-0(D,X)23-V-48,,SIG) D415400100036 (26-FE-0(P,X)27-CO-56,,SIG) D415400100037 MONIT-REF (,F.Tarkanyi+,R,IAEA-NDS-1211,2001) chapter 4 D415400100038 CORRECTION Correction of the beam was made using the D415400100039 monitor reactions. D415400100040 HISTORY (20050913C) D415400100041 (20190824A) SD: Corrections in all Subents. D415400100042 ERR-ANALYS updated. ERR-T -> DATA-ERR. Subent 005 was D415400100043 splitted in two. D415400100044 On. ERR-ANALYS moved to 002-004. D415400100045 (20210927A) VS. SF3 corrected in 003 and 006.2 D415400100046 ENDBIB 44 0 D415400100047 NOCOMMON 0 0 D415400100048 ENDSUBENT 47 0 D415400199999 SUBENT D4154002 20190824 D121D415400200001 BIB 5 10 D415400200002 REACTION (78-PT-198(P,N)79-AU-198-G,,SIG) D415400200003 DECAY-DATA (79-AU-198-G,2.695D,DG,411.8,0.96) D415400200004 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam 0.3 MeV. D415400200005 (DATA-ERR) Total errors excluding the uncertainties of D415400200006 the non linear contributions (time, half-life, etc.). D415400200007 STATUS (TABLE) Table 2 of the Radiochim.Acta 92(2004)223 D415400200008 (APRVD) Approved by S.Takacs D415400200009 HISTORY (20190824A) SD: SF9=EXP deleted from REACTION code. D415400200010 ERR-T -> DATA-ERR. STATUS updated. D415400200011 On. ERR-ANALYS moved from 001. D415400200012 ENDBIB 10 0 D415400200013 NOCOMMON 0 0 D415400200014 DATA 4 38 D415400200015 EN EN-ERR DATA DATA-ERR D415400200016 MEV MEV MB MB D415400200017 6.0 2.1 0.5 0.1 D415400200018 8.0 1.9 14.6 1.8 D415400200019 9.7 1.7 48.8 7.8 D415400200020 11.2 1.5 55.8 9.1 D415400200021 12.6 1.4 46.6 8.6 D415400200022 13.9 1.2 29.5 8.3 D415400200023 15.1 1.1 27.4 10.7 D415400200024 16.3 1.0 30.7 9.9 D415400200025 17.4 0.8 45.3 11.9 D415400200026 18.4 0.7 37.9 13.1 D415400200027 19.4 0.6 29.4 11.2 D415400200028 19.8 2.2 24.8 3.5 D415400200029 20.4 0.5 37.5 15.0 D415400200030 20.8 2.1 25.1 4.1 D415400200031 21.3 0.4 30.7 11.9 D415400200032 21.7 2.0 22.6 3.5 D415400200033 22.2 0.3 30.0 9.8 D415400200034 22.6 1.9 20.5 3.4 D415400200035 23.5 1.8 21.8 3.5 D415400200036 24.4 1.7 23.4 5.5 D415400200037 25.2 1.6 19.8 3.0 D415400200038 26.1 1.5 19.9 3.6 D415400200039 26.9 1.5 19.0 2.9 D415400200040 27.7 1.4 20.0 3.3 D415400200041 28.4 1.3 19.7 3.2 D415400200042 29.2 1.2 18.6 3.1 D415400200043 29.9 1.1 17.5 3.0 D415400200044 30.7 1.0 17.0 2.9 D415400200045 31.4 1.0 16.1 2.2 D415400200046 32.1 0.9 17.7 2.7 D415400200047 32.8 0.8 15.3 2.5 D415400200048 33.5 0.7 16.1 2.7 D415400200049 34.2 0.7 15.3 2.6 D415400200050 34.8 0.6 15.2 3.0 D415400200051 35.5 0.5 14.6 3.3 D415400200052 36.1 0.4 14.8 3.2 D415400200053 36.7 0.4 15.0 2.9 D415400200054 37.4 0.3 14.2 2.9 D415400200055 ENDDATA 40 0 D415400200056 ENDSUBENT 55 0 D415400299999 SUBENT D4154003 20210929 D132D415400300001 BIB 5 12 D415400300002 REACTION (78-PT-198(D,N)79-AU-199,,SIG) D415400300003 DECAY-DATA (79-AU-199,3.139D,DG,158.37,0.4, D415400300004 DG,208.21,0.0872) D415400300005 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam 0.3 MeV. D415400300006 (DATA-ERR) Total errors excluding the uncertainties of D415400300007 the non linear contributions (time, half-life, etc.). D415400300008 STATUS (TABLE) Table 2 of the Radiochim.Acta 92(2004)223 D415400300009 (APRVD) Approved by S.Takacs D415400300010 HISTORY (20190824A) SD: SF9=EXP deleted from REACTION code. D415400300011 ERR-T -> DATA-ERR. STATUS updated. D415400300012 On. ERR-ANALYS moved from 001. D415400300013 (20210927A) VS. SF3 X->N c.f. Memo CP-D/1017. D415400300014 ENDBIB 12 0 D415400300015 NOCOMMON 0 0 D415400300016 DATA 4 24 D415400300017 EN EN-ERR DATA DATA-ERR D415400300018 MEV MEV MB MB D415400300019 5.5 1.3 2.8 0.7 D415400300020 6.9 1.2 25.1 3.9 D415400300021 8.2 1.0 91.1 13.2 D415400300022 9.4 0.9 181.5 25.9 D415400300023 10.4 0.8 163.4 24.6 D415400300024 10.5 1.4 211.5 25.0 D415400300025 11.4 1.3 237.4 27.8 D415400300026 11.5 0.7 216.4 29.2 D415400300027 12.3 1.2 225.5 26.9 D415400300028 12.4 0.6 227.0 33.5 D415400300029 13.1 1.1 214.4 25.2 D415400300030 13.3 0.5 218.5 30.8 D415400300031 14.0 1.0 253.6 31.8 D415400300032 14.2 0.4 207.5 33.5 D415400300033 14.7 0.9 214.6 25.8 D415400300034 15.0 0.3 177.0 22.6 D415400300035 15.5 0.8 197.3 24.7 D415400300036 16.2 0.7 267.3 32.5 D415400300037 17.0 0.7 184.8 23.3 D415400300038 17.7 0.6 192.5 24.4 D415400300039 18.3 0.5 157.4 20.2 D415400300040 19.0 0.4 182.2 23.1 D415400300041 19.6 0.4 157.0 24.1 D415400300042 20.3 0.3 151.7 22.1 D415400300043 ENDDATA 26 0 D415400300044 ENDSUBENT 43 0 D415400399999 SUBENT D4154004 20190824 D121D415400400001 BIB 5 14 D415400400002 REACTION 1(78-PT-198(D,2N)79-AU-198-M,,SIG) D415400400003 2(78-PT-198(D,2N)79-AU-198-G,,SIG) D415400400004 DECAY-DATA1(79-AU-198-M,2.270D,DG,180.3,0.5, D415400400005 DG,204.1,0.408, D415400400006 DG,214.9,0.70) D415400400007 2(79-AU-198-G,2.695D,DG,411.8,0.96) D415400400008 ERR-ANALYS (EN-ERR) The uncertainty of the primary beam 0.3 MeV. D415400400009 (DATA-ERR) Total errors excluding the uncertainties of D415400400010 the non linear contributions (time, half-life, etc.). D415400400011 STATUS (TABLE) Table 2 of the Radiochim.Acta 92(2004)223 D415400400012 (APRVD) Approved by S.Takacs D415400400013 HISTORY (20190824A) SD: SF9=EXP deleted from both REACTION D415400400014 codes. ERR-T -> DARA-ERR. STATUS updated. D415400400015 On. ERR-ANALYS moved from 001. D415400400016 ENDBIB 14 0 D415400400017 NOCOMMON 0 0 D415400400018 DATA 6 24 D415400400019 EN EN-ERR DATA 1DATA-ERR 1DATA 2DATA-ERR 2D415400400020 MEV MEV MB MB MB MB D415400400021 5.5 1.3 0.073 0.027 D415400400022 6.9 1.2 4.0 0.5 D415400400023 8.2 1.0 0.023 0.0063 34.5 3.9 D415400400024 9.4 0.9 2.8 2.1 122.4 13.8 D415400400025 10.4 0.8 2.8 1.6 248.6 28.0 D415400400026 10.5 1.4 297.6 33.9 D415400400027 11.4 1.3 7.1 2.6 383.1 43.4 D415400400028 11.5 0.7 4.9 2.3 355.0 40.1 D415400400029 12.3 1.2 9.7 3.0 379.8 43.1 D415400400030 12.4 0.6 14.0 10.7 410.1 46.3 D415400400031 13.1 1.1 10.1 2.6 361.0 40.6 D415400400032 13.3 0.5 9.8 5.2 385.2 43.5 D415400400033 14.0 1.0 20.4 4.6 357.0 40.7 D415400400034 14.2 0.4 14.0 3.8 337.1 38.1 D415400400035 14.7 0.9 18.2 4.1 308.7 35.0 D415400400036 15.0 0.3 17.2 2.6 365.2 29.8 D415400400037 15.5 0.8 17.6 4.0 253.0 28.4 D415400400038 16.2 0.7 16.9 4.0 218.9 25.2 D415400400039 17.0 0.7 13.7 4.7 168.8 19.5 D415400400040 17.7 0.6 16.1 6.3 147.9 17.3 D415400400041 18.3 0.5 9.9 3.8 131.9 15.3 D415400400042 19.0 0.4 14.8 6.6 129.9 15.2 D415400400043 19.6 0.4 15.4 13.9 102.0 12.1 D415400400044 20.3 0.3 13.3 10.6 117.7 14.8 D415400400045 ENDDATA 26 0 D415400400046 ENDSUBENT 45 0 D415400499999 SUBENT D4154005 20190824 D121D415400500001 BIB 4 7 D415400500002 REACTION (78-PT-198(P,N)79-AU-198-G,,TTY,,PHY,DERIV) D415400500003 ANALYSIS (INTEF) Derived from measured excitation function D415400500004 STATUS (TABLE) Table 2 of the Radiochim.Acta 92(2004)223 D415400500005 (APRVD) Approved by S.Takacs D415400500006 (DEP,D4154002) excitation function D415400500007 HISTORY (20190824A) SD: SF9=CALC->DERIV in REACTION code.SubentD415400500008 was splitted in two. ANALYSIS added. STATUS updated. D415400500009 ENDBIB 7 0 D415400500010 NOCOMMON 0 0 D415400500011 DATA 2 1 D415400500012 EN DATA D415400500013 MEV GBQ/COUL D415400500014 16. 1.2 D415400500015 ENDDATA 3 0 D415400500016 ENDSUBENT 15 0 D415400599999 SUBENT D4154006 20210929 D132D415400600001 BIB 4 9 D415400600002 REACTION 1(78-PT-198(D,2N)79-AU-198-G,,TTY,,PHY,DERIV) D415400600003 2(78-PT-198(D,N)79-AU-199,,TTY,,PHY,DERIV) D415400600004 ANALYSIS (INTEF) Derived from measured excitation function D415400600005 STATUS (TABLE) Table 2 of the Radiochim.Acta 92(2004)223 D415400600006 (APRVD) Approved by S.Takacs D415400600007 1(DEP,D4154004) excitation function D415400600008 2(DEP,D4154003) excitation function D415400600009 HISTORY (20190824T) SD: Part of Subent 005. D415400600010 (20210927A) VS. SF3: X->N in 006.2 c.f. Memo CP-D/1017.D415400600011 ENDBIB 9 0 D415400600012 NOCOMMON 0 0 D415400600013 DATA 3 1 D415400600014 EN DATA 1DATA 2 D415400600015 MEV GBQ/COUL GBQ/COUL D415400600016 15. 4.4 2.8 D415400600017 ENDDATA 3 0 D415400600018 ENDSUBENT 17 0 D415400699999 ENDENTRY 6 0 D415499999999