ENTRY D4175 20220506 D137D417500000001 SUBENT D4175001 20220506 D137D417500100001 BIB 12 43 D417500100002 TITLE Deuteron-induced reactions on Yb: Measured cross D417500100003 sections and rationale for production pathways of D417500100004 carrier-free, medically relevant radionuclides D417500100005 AUTHOR (A.Hermanne, S.Takacs, M.B.Goldberg, E.Lavie, D417500100006 Yu.N.Shubin, S.Kovalev) D417500100007 INSTITUTE (2BLGVUB,3HUNDEB,3ISLSOR) D417500100008 REFERENCE (J,NIM/B,247,223,2006) D417500100009 FACILITY (CYCLO,2BLGVUB) CGR 560 cyclotron D417500100010 SAMPLE Natural Yb foils 30 microns thick and natural Ti 25 D417500100011 microns foils for beam monitoring from Goodfellow. D417500100012 METHOD (STTA,ACTIV,EXTB) D417500100013 Standard stacked foil irradiation method was used. D417500100014 Two stacks were irradiated with incident deuteron D417500100015 beams of 21 and 15 MeV. D417500100016 (GSPEC) Long measurements of more than 24 h duration, D417500100017 to assay the long-lived radionuclides, were performed D417500100018 8 months after EOB at a distance of 5 cm. D417500100019 (EDEG) Energy degradation in the stacks was estimated D417500100020 by calculation using the stopping power data and D417500100021 polynomial approximation of Andersen and Ziegler. D417500100022 DETECTOR (HPGE) Samples were measured using HPGE detectors, D417500100023 first at large detector-sample distances 50 cm. D417500100024 MONITOR (22-TI-0(D,X)23-V-48,,SIG) D417500100025 MONIT-REF (,F.Tarkanyi+,R,IAEA-TECDOC-1211,2001) D417500100026 ERR-ANALYS (ERR-T) The total resulting uncertainties (8-13%) D417500100027 obtained as square root of the sum of contributing D417500100028 sources in quadrature: D417500100029 (ERR-1) Number of target nuclei, including target D417500100030 non-uniformities (5%) D417500100031 (ERR-2) Incident particle intensity (5%) D417500100032 (ERR-3) Detection efficiency (5%) D417500100033 (ERR-4,1.,5.) Determination of the peak areas, D417500100034 including statistical errors (1-5%) D417500100035 (ERR-5,1.,5.) Abundance of the gamma rays (1-5%) D417500100036 (EN-ERR) The uncertainty in the primary beam energy, D417500100037 estimated to be 0.2 MeV. The overall uncertainty in D417500100038 the mean energy at the last foil in the stack was D417500100039 estimated to be 0.7 MeV, taking into account D417500100040 cumulative effects of the possible variations in D417500100041 incident energy and number of target atoms. D417500100042 HISTORY (20060524C) ts D417500100043 (20140409A) On. ERR-ANALYS updated D417500100044 (20220506A) On+VT. Major revisions in 002 and 003. D417500100045 ENDBIB 43 0 D417500100046 COMMON 3 3 D417500100047 ERR-1 ERR-2 ERR-3 D417500100048 PER-CENT PER-CENT PER-CENT D417500100049 5. 5. 5. D417500100050 ENDCOMMON 3 0 D417500100051 ENDSUBENT 50 0 D417500199999 SUBENT D4175002 20220506 D137D417500200001 BIB 5 9 D417500200002 REACTION 1(70-YB-176(D,X)71-LU-177-G,CUM,SIG) D417500200003 Measured after the total decay of 177Yb D417500200004 2(70-YB-176(D,X)71-LU-177-G,CUM,TTY,,PHY,DERIV) D417500200005 ANALYSIS 2(INTEF) D417500200006 DECAY-DATA (71-LU-177-G,6.71D,DG,208.,0.11) D417500200007 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B247(2006)223 D417500200008 HISTORY (20140409U) On. REACTION(SF9): EXP deleted D417500200009 (20220506A) On+VT. 177Yb SIG moved to 003. 177gLu TTY D417500200010 moved from 003. D417500200011 ENDBIB 9 0 D417500200012 NOCOMMON 0 0 D417500200013 DATA 5 18 D417500200014 EN EN-ERR DATA 1ERR-T 1DATA 2 D417500200015 MEV MEV MB MB KBQ/MUAHR D417500200016 20.3 0.2 143.7 11. 8124.3 D417500200017 19.2 0.2 136.9 11. 7451.4 D417500200018 18.0 0.2 147.4 12. 6662.8 D417500200019 16.8 0.3 140.3 11. 5883.3 D417500200020 15.6 0.3 165.1 13. 5083.2 D417500200021 14.3 0.2 190.5 15. 4157.3 D417500200022 14.2 0.3 189.6 15. 4083.6 D417500200023 12.9 0.3 199.3 16. 3109.5 D417500200024 12.8 0.4 201.9 16. 3034.2 D417500200025 11.9 0.3 217.4 17. 2364.6 D417500200026 11.3 0.4 211.1 17. 1936.9 D417500200027 10.8 0.4 199.2 16. 1601.6 D417500200028 9.6 0.5 163.8 13. 906.4 D417500200029 9.6 0.5 163.4 13. D417500200030 8.3 0.6 111.3 9. 384.2 D417500200031 6.9 0.6 39.6 5. 104.0 D417500200032 5.3 0.7 8.4 1. 13.5 D417500200033 3.2 0.8 0.01 D417500200034 ENDDATA 20 0 D417500200035 ENDSUBENT 34 0 D417500299999 SUBENT D4175003 20220506 D137D417500300001 BIB 5 15 D417500300002 REACTION 1(70-YB-176(D,P)70-YB-177,,SIG) D417500300003 Measured after the total decay of metastable state D417500300004 2(70-YB-176(D,N)71-LU-177-G,,SIG) D417500300005 DECAY-DATA1(70-YB-177-G,1.9HR,DG,121.6,0.034, D417500300006 DG,150.4,0.20, D417500300007 DG,1080.2,0.055) D417500300008 2(71-LU-177-G,6.71D,DG,208.,0.11) D417500300009 ANALYSIS 2Derived by subtraction of the 177Yb production cross D417500300010 section from the 177gLu cumulative production cross D417500300011 section D417500300012 STATUS (TABLE) Table 2 of Nucl.Instrum.Meth.B247(2006)223 D417500300013 2(DEP,D4175002) 177gLu cumulative prod. cross section D417500300014 HISTORY (20140409U) On. REACTION(SF9): EXP deleted D417500300015 (20220506A) On+VT. 177gLu TTY moved to 002. 177Yb SIG D417500300016 moved from 002. D417500300017 ENDBIB 15 0 D417500300018 NOCOMMON 0 0 D417500300019 DATA 5 18 D417500300020 EN EN-ERR DATA 1ERR-T 1DATA 2 D417500300021 MEV MEV MB MB MB D417500300022 20.3 0.2 101.6 8. 38.5 D417500300023 19.2 0.2 108.3 9. 31.3 D417500300024 18.0 0.2 119.2 10. 22.8 D417500300025 16.8 0.3 132.8 11. 15.7 D417500300026 15.6 0.3 150.9 12. 12.6 D417500300027 14.3 0.2 190.0 15. 9.6 D417500300028 14.2 0.3 167.6 13. 9.3 D417500300029 12.9 0.3 214.1 17. 3.9 D417500300030 12.8 0.4 190.7 15. 3.3 D417500300031 11.9 0.3 217.3 17. D417500300032 11.3 0.4 198.2 16. D417500300033 10.8 0.4 211.7 17. D417500300034 9.6 0.5 171.9 14. D417500300035 9.6 0.5 180.9 14. D417500300036 8.3 0.6 117.3 14. D417500300037 6.9 0.6 41.4 5. D417500300038 5.3 0.7 8.7 1.0 D417500300039 3.2 0.8 0.7 0.1 D417500300040 ENDDATA 20 0 D417500300041 ENDSUBENT 40 0 D417500399999 SUBENT D4175004 20140409 D094D417500400001 BIB 4 8 D417500400002 REACTION 1(70-YB-0(D,X)71-LU-170,,SIG) D417500400003 2(70-YB-0(D,X)71-LU-171-G,CUM,SIG) D417500400004 DECAY-DATA1(71-LU-170-G,48.HR,DG,193.2,0.0207, D417500400005 DG,1054.,0.0461) D417500400006 2(71-LU-171-G,8.24D,DG,667.4,0.111, D417500400007 DG,739.8,0.48) D417500400008 STATUS (TABLE) Table 3 of Nucl.Instrum.Meth.B247(2006)223 D417500400009 HISTORY (20140409U) On. REACTION(SF9): EXP deleted D417500400010 ENDBIB 8 0 D417500400011 NOCOMMON 0 0 D417500400012 DATA 6 17 D417500400013 EN EN-ERR DATA 1ERR-T 1DATA 2ERR-T 2D417500400014 MEV MEV MB MB MB MB D417500400015 20.3 0.2 184.7 15. 268.5 21. D417500400016 19.2 0.2 170.0 14. 251.7 20. D417500400017 18.0 0.2 145.6 12. 237.7 19. D417500400018 16.8 0.3 105.1 8. 210.1 17. D417500400019 15.6 0.3 66.7 5. 184.7 15. D417500400020 14.3 0.2 22.4 2. 145.2 12. D417500400021 14.2 0.3 31.9 3. 141.9 11. D417500400022 12.9 0.3 21.4 2. 109.9 9. D417500400023 12.8 0.4 24.9 2. 110.3 9. D417500400024 11.9 0.3 17.2 1. 90.0 7. D417500400025 11.3 0.4 17.5 1. 80.4 6. D417500400026 10.8 0.4 8.3 1. 64.9 5. D417500400027 9.6 0.5 5.7 0.5 40.4 3. D417500400028 9.6 0.5 3.9 0.3 39.8 3. D417500400029 8.3 0.6 1.1 0.1 16.3 1. D417500400030 6.9 0.6 2.8 0.3 D417500400031 5.3 0.7 1.1 0.1 D417500400032 ENDDATA 19 0 D417500400033 ENDSUBENT 32 0 D417500499999 SUBENT D4175005 20140409 D094D417500500001 BIB 4 9 D417500500002 REACTION 1(70-YB-0(D,X)71-LU-172,CUM,SIG) D417500500003 2(70-YB-0(D,X)71-LU-173,,SIG) D417500500004 DECAY-DATA1(71-LU-172-G,6.7D,DG,810.1,0.16, D417500500005 DG,900.8,0.288, D417500500006 DG,1093.7,0.635) D417500500007 2(71-LU-173,1.37YR,DG,171.3,0.018, D417500500008 DG,271.99,0.013) D417500500009 STATUS (TABLE) Table 3 of Nucl.Instrum.Meth.B247(2006)223 D417500500010 HISTORY (20140409U) On. REACTION(SF9): EXP deleted D417500500011 ENDBIB 9 0 D417500500012 NOCOMMON 0 0 D417500500013 DATA 6 17 D417500500014 EN EN-ERR DATA 1ERR-T 1DATA 2ERR-T 2D417500500015 MEV MEV MB MB MB MB D417500500016 20.3 0.2 225.4 18. 381.7 31. D417500500017 19.2 0.2 214.4 17. 363.6 29. D417500500018 18.0 0.2 226.6 18. 350.5 28. D417500500019 16.8 0.3 211.5 17. 313.1 25. D417500500020 15.6 0.3 220.8 18. 282.4 23. D417500500021 14.3 0.2 209.0 17. 250.0 20. D417500500022 14.2 0.3 198.9 16. 223.0 18. D417500500023 12.9 0.3 164.4 13. 159.3 13. D417500500024 12.8 0.4 156.0 12. 154.7 12. D417500500025 11.9 0.3 140.6 11. 113.4 9. D417500500026 11.3 0.4 119.5 10. 96.0 8. D417500500027 10.8 0.4 108.0 9. 84.6 7. D417500500028 9.6 0.5 60.9 5. 55.3 4. D417500500029 9.6 0.5 60.4 5. 55.0 4. D417500500030 8.3 0.6 25.6 2. 25.0 2. D417500500031 6.9 0.6 3.4 0.3 5.5 0.4 D417500500032 5.3 0.7 0.2 0.02 0.2 0.02 D417500500033 ENDDATA 19 0 D417500500034 ENDSUBENT 33 0 D417500599999 SUBENT D4175006 20140409 D094D417500600001 BIB 4 4 D417500600002 REACTION (70-YB-0(D,X)71-LU-174-G,,SIG) D417500600003 DECAY-DATA (71-LU-174-G,3.31YR,DG,1241.,0.065) D417500600004 STATUS (TABLE) Table 3 of Nucl.Instrum.Meth.B247(2006)223 D417500600005 HISTORY (20140409U) On. REACTION(SF9): EXP deleted D417500600006 ENDBIB 4 0 D417500600007 NOCOMMON 0 0 D417500600008 DATA 4 15 D417500600009 EN EN-ERR DATA ERR-T D417500600010 MEV MEV MB MB D417500600011 20.3 0.2 54.9 4. D417500600012 19.2 0.2 54.6 4. D417500600013 18.0 0.2 64.7 5. D417500600014 16.8 0.3 82.9 7. D417500600015 15.6 0.3 113.4 9. D417500600016 14.3 0.2 151.4 12. D417500600017 14.2 0.3 135.8 11. D417500600018 12.9 0.3 167.5 13. D417500600019 12.8 0.4 157.5 13. D417500600020 11.9 0.3 156.6 13. D417500600021 11.3 0.4 149.5 12. D417500600022 10.8 0.4 120.9 10. D417500600023 9.6 0.5 82.1 7. D417500600024 9.6 0.5 76.4 6. D417500600025 8.3 0.6 36.5 3. D417500600026 ENDDATA 17 0 D417500600027 ENDSUBENT 26 0 D417500699999 SUBENT D4175007 20140409 D094D417500700001 BIB 5 16 D417500700002 REACTION 1(70-YB-0(D,X)70-YB-175,,SIG) D417500700003 2(70-YB-0(D,X)70-YB-169,,SIG) D417500700004 DECAY-DATA1(70-YB-175,4.19D,DG,282.5,0.0613, D417500700005 DG,396.3,0.132) D417500700006 2(70-YB-169-G,32.02D,DG,197.9,0.349, D417500700007 DG,307.7,0.108) D417500700008 COMMENT Alex Hermanne (2014-04-04): D417500700009 There are misprints in the gamma intensities of 175Yb D417500700010 tabulated in the article: D417500700011 for 282.5 keV 6.13% in place of 3.05% D417500700012 for 396.3 keV 13.2% in place of 6.5% D417500700013 STATUS (TABLE) Table 4 of Nucl.Instrum.Meth.B247(2006)223 D417500700014 (APRVD) Approved by Alex Hermanne (2014-04-09) D417500700015 HISTORY (20140409A) On. DECAY-DATA of 175Yb corrected; D417500700016 one data point added at 3.2 MeV; D417500700017 ERR-T(169Yb) at 9.6 MeV:0.1 mb->0.05 mbD417500700018 ENDBIB 16 0 D417500700019 NOCOMMON 0 0 D417500700020 DATA 6 18 D417500700021 EN EN-ERR DATA 1ERR-T 1DATA 2ERR-T 2D417500700022 MEV MEV MB MB MB MB D417500700023 20.3 0.2 48.5 4. 24.4 2. D417500700024 19.2 0.2 47.7 4. 19.4 2. D417500700025 18.0 0.2 44.1 4. 14.2 1. D417500700026 16.8 0.3 50.8 4. 6.4 1. D417500700027 15.6 0.3 59.1 5. 2.6 0.3 D417500700028 14.3 0.2 63.7 5. D417500700029 14.2 0.3 64.0 5. 1.8 0.2 D417500700030 12.9 0.3 70.9 6. D417500700031 12.8 0.4 67.3 5. 1.2 0.1 D417500700032 11.9 0.3 69.7 6. D417500700033 11.3 0.4 72.5 6. 0.1 0.01 D417500700034 10.8 0.4 67.5 5. D417500700035 9.6 0.5 54.5 4. 0.4 0.05 D417500700036 9.6 0.5 56.5 5. D417500700037 8.3 0.6 35.9 4. D417500700038 6.9 0.6 12.3 1. D417500700039 5.3 0.7 2.9 0.3 D417500700040 3.2 0.8 0.6 0.1 D417500700041 ENDDATA 20 0 D417500700042 ENDSUBENT 41 0 D417500799999 ENDENTRY 7 0 D417599999999