ENTRY D4209 20220111 D136D420900000001 SUBENT D4209001 20220111 D136D420900100001 BIB 15 64 D420900100002 TITLE Excitation functions for production of medically D420900100003 relevant radioisotopes in deuteron irradiations of D420900100004 Pr and Tm targets D420900100005 AUTHOR (A.Hermanne,F.Tarkanyi,S.Takacs,F.Ditroi,M.Baba, D420900100006 T.Ohtsuki,I.Spahn,A.V.Ignatyuk) Ohtshuki -> Ohtsuki D420900100007 REFERENCE (J,NIM/B,267,727,2009) D420900100008 INSTITUTE (2BLGVUB,3HUNDEB,2JPNTOH,4RUSFEI) D420900100009 FACILITY (CYCLO,2BLGVUB) D420900100010 (CYCLO,2JPNTOH) D420900100011 SAMPLE Oxides of Tm and Pr were prepared by sedimentation D420900100012 technique on Al or Ni backings. D420900100013 DETECTOR (HPGE) D420900100014 METHOD (ACTIV,BCINT,EDEG,EXTB,GSPEC,MOSEP,STTA) D420900100015 Irradiations were performed at the external beams of D420900100016 the Tohoku University (Sendai) and Vrije Universiteit D420900100017 Brussels (VUB) cyclotrons. D420900100018 The Tm2O3: D420900100019 25-35 microns in Tm equivalent for Sendai experiments; D420900100020 15-60 microns thick for VUB experiments, purity 99.9%. D420900100021 The Pr6O11: D420900100022 250-60 lm thick in Pr equivalent, purity 99.5%. D420900100023 Al (100 microns) and Ti (12.5 microns) monitor foils D420900100024 were used. The stacks were mounted in a Faraday cup D420900100025 like target holder equipped with a suppressor of D420900100026 secondary electrons. The energy of the incident D420900100027 deuteron beams was up to 40 MeV at Sendai and 20 MeV D420900100028 at VUB, respectively. The beam current: of 90-200 nA. D420900100029 Independent and cumulative cross sections were D420900100030 determined. D420900100031 MONITOR (22-TI-0(D,X)23-V-48,,SIG) D420900100032 (13-AL-27(D,X)11-NA-22,,SIG) D420900100033 (13-AL-27(D,X)11-NA-24,,SIG) D420900100034 Downshifts of 0.5-2 MeV in nominal incident energy and D420900100035 corrections in particle flux of a few percent result D420900100036 were necessary to apply. D420900100037 MONIT-REF (,F.Tarkanyi+,R,IAEA-NDS-1211,2001) updated web versionD420900100038 ERR-ANALYS (EN-ERR)The monitoring method allows estimating the D420900100039 uncertainty on the primary beam energy at +-0.2 MeV. D420900100040 The uncertainty on the average energy in each foil is, D420900100041 however, continuously rising through the stack and D420900100042 attains +-1 MeV for the last foil due to cumulative D420900100043 possible variations on target thickness and energy D420900100044 degradation. D420900100045 (ERR-T)The included experimental uncertainties are: D420900100046 * number of target nuclei including non-uniformity D420900100047 of the deposits, D420900100048 * incident particle flux, D420900100049 * peak area including statistical errors on counts, D420900100050 * detector efficiency, D420900100051 * gamma ray abundance and branching rate data. D420900100052 A total uncertainty of 10-15% is obtained as positive D420900100053 square root of the quadratic sum of the individual D420900100054 sources. Possible additional uncertainties due to non D420900100055 linear effects of half-lives and waiting time were not D420900100056 accounted for. D420900100057 DECAY-DATA Decay and spectrometric characteristics of the D420900100058 investigated radionuclides were taken from Nudat2. D420900100059 ADD-RES (TTY-C) Thick target production yields were calculated D420900100060 from the fitted experimental croos sections. D420900100061 STATUS (APRVD) S.Takacs, 2009. D420900100062 HISTORY (20090325C) TS D420900100063 (20151007A) VS Data in 010, 012 and 013 compiled in D420900100064 D4180.002,003 and 004 deleted. D420900100065 (20220111A) TS Major revision in 003. D420900100066 ENDBIB 64 0 D420900100067 NOCOMMON 0 0 D420900100068 ENDSUBENT 67 0 D420900199999 SUBENT D4209002 20090325 D066D420900200001 BIB 3 5 D420900200002 REACTION (59-PR-141(D,2N)60-ND-141,,SIG) D420900200003 DECAY-DATA (60-ND-141-G,2.49HR,DG,1126.9,0.008) D420900200004 Decay data were taken from table 1. of the reference D420900200005 originating from Nudat2 database. D420900200006 STATUS (TABLE)Numerical data were taken from table 2. D420900200007 ENDBIB 5 0 D420900200008 NOCOMMON 0 0 D420900200009 DATA 4 7 D420900200010 EN EN-ERR DATA ERR-T D420900200011 MEV MEV MB MB D420900200012 20.6 0.2 716.4 71.6 D420900200013 18.6 0.3 1024.7 102.5 D420900200014 16.8 0.3 1100.1 110.0 D420900200015 14.8 0.4 1374.9 137.5 D420900200016 12.7 0.5 990.1 99.0 D420900200017 10.3 0.6 619.2 61.9 D420900200018 7.4 0.8 52.7 5.3 D420900200019 ENDDATA 9 0 D420900200020 ENDSUBENT 19 0 D420900299999 SUBENT D4209003 20220111 D136D420900300001 BIB 4 8 D420900300002 REACTION (59-PR-141(D,3N)60-ND-140,,SIG) D420900300003 DECAY-DATA (60-ND-140,80.9HR) Measured through the decay of 140Pr D420900300004 (59-PR-140,,AR,511.,1.12) D420900300005 Decay data were taken from table 1. of the reference D420900300006 originating from Nudat2 database. D420900300007 STATUS (TABLE)Numerical data were taken from table 2. D420900300008 HISTORY (20220111A) TS Decay data in subentry 3 was corrected. D420900300009 ...B+/EC,,0.6) -> ...AR,511.,1.12) D420900300010 ENDBIB 8 0 D420900300011 NOCOMMON 0 0 D420900300012 DATA 4 10 D420900300013 EN EN-ERR DATA ERR-T D420900300014 MEV MEV MB MB D420900300015 39.9 0.2 414.1 75.9 D420900300016 36.8 0.3 584.9 106.5 D420900300017 33.0 0.4 734.9 124.8 D420900300018 28.7 0.5 987.5 142.2 D420900300019 23.8 0.6 887.8 135.0 D420900300020 20.6 0.2 496.6 50. D420900300021 18.6 0.3 294.3 30. D420900300022 16.8 0.3 89.4 9.0 D420900300023 14.8 0.4 10.8 1.1 D420900300024 12.7 0.5 0.3 0.1 D420900300025 ENDDATA 12 0 D420900300026 ENDSUBENT 25 0 D420900399999 SUBENT D4209004 20090325 D066D420900400001 BIB 3 5 D420900400002 REACTION (59-PR-141(D,4N)60-ND-139-M,,SIG) D420900400003 DECAY-DATA (60-ND-139-M,5.5HR,DG,738.2,0.35) D420900400004 Decay data were taken from table 1. of the reference D420900400005 originating from Nudat2 database. D420900400006 STATUS (TABLE)Numerical data were taken from table 2. D420900400007 ENDBIB 5 0 D420900400008 NOCOMMON 0 0 D420900400009 DATA 4 4 D420900400010 EN EN-ERR DATA ERR-T D420900400011 MEV MEV MB MB D420900400012 39.9 0.2 768.9 87.3 D420900400013 36.8 0.3 644.7 73.5 D420900400014 33.0 0.4 286.3 32.2 D420900400015 28.7 0.5 26.1 5.6 D420900400016 ENDDATA 6 0 D420900400017 ENDSUBENT 16 0 D420900499999 SUBENT D4209005 20090325 D066D420900500001 BIB 3 5 D420900500002 REACTION (59-PR-141(D,P)59-PR-142,,SIG) D420900500003 DECAY-DATA (59-PR-142-G,19.12HR,DG,1575.6,0.037) D420900500004 Decay data were taken from table 1. of the reference D420900500005 originating from Nudat2 database. D420900500006 STATUS (TABLE)Numerical data were taken from table 2. D420900500007 ENDBIB 5 0 D420900500008 NOCOMMON 0 0 D420900500009 DATA 4 12 D420900500010 EN EN-ERR DATA ERR-T D420900500011 MEV MEV MB MB D420900500012 39.9 0.2 48.2 9.0 D420900500013 36.8 0.3 49.3 9.7 D420900500014 33.0 0.4 55.3 11.6 D420900500015 28.7 0.5 70.0 11.7 D420900500016 23.8 0.6 102.1 15.4 D420900500017 20.6 0.2 82.0 8.2 D420900500018 18.6 0.3 100.0 10.0 D420900500019 16.8 0.3 125.8 12.6 D420900500020 14.8 0.4 170.3 17.0 D420900500021 12.7 0.5 178.0 17.8 D420900500022 10.3 0.6 254.6 25.5 D420900500023 7.4 0.8 92.4 9.2 D420900500024 ENDDATA 14 0 D420900500025 ENDSUBENT 24 0 D420900599999 SUBENT D4209006 20090325 D066D420900600001 BIB 3 5 D420900600002 REACTION (59-PR-141(D,X)58-CE-139,CUM,SIG) D420900600003 DECAY-DATA (58-CE-139-G,137.6D,DG,165.7,0.8) D420900600004 Decay data were taken from table 1. of the reference D420900600005 originating from Nudat2 database. D420900600006 STATUS (TABLE)Numerical data were taken from table 2. D420900600007 ENDBIB 5 0 D420900600008 NOCOMMON 0 0 D420900600009 DATA 4 11 D420900600010 EN EN-ERR DATA ERR-T D420900600011 MEV MEV MB MB D420900600012 39.9 0.2 1047.5 121.1 D420900600013 36.8 0.3 888.5 102.8 D420900600014 33.0 0.4 426.8 52.0 D420900600015 28.7 0.5 67.2 15.2 D420900600016 20.6 0.2 4.2 0.4 D420900600017 18.6 0.3 4.3 0.4 D420900600018 16.8 0.3 4.1 0.4 D420900600019 14.8 0.4 4.4 0.4 D420900600020 12.7 0.5 2.8 0.3 D420900600021 10.3 0.6 1.5 0.1 D420900600022 7.4 0.8 0.0 0.0 D420900600023 ENDDATA 13 0 D420900600024 ENDSUBENT 23 0 D420900699999 SUBENT D4209007 20090325 D066D420900700001 BIB 3 5 D420900700002 REACTION (59-PR-141(D,X)58-CE-137-M,,SIG) D420900700003 DECAY-DATA (58-CE-137-M,34.4HR,DG,254.3,0.11) D420900700004 Decay data were taken from table 1. of the reference D420900700005 originating from Nudat2 database. D420900700006 STATUS (TABLE)Numerical data were taken from table 2. D420900700007 ENDBIB 5 0 D420900700008 NOCOMMON 0 0 D420900700009 DATA 4 3 D420900700010 EN EN-ERR DATA ERR-T D420900700011 MEV MEV MB MB D420900700012 39.9 0.2 52.7 7.7 D420900700013 36.8 0.3 51.0 7.4 D420900700014 33.0 0.4 20.2 2.3 D420900700015 ENDDATA 5 0 D420900700016 ENDSUBENT 15 0 D420900799999 SUBENT D4209008 20090325 D066D420900800001 BIB 3 5 D420900800002 REACTION (59-PR-141(D,X)58-CE-135,,SIG) D420900800003 DECAY-DATA (58-CE-135,17.7HR,DG,572.3,0.104) D420900800004 Decay data were taken from table 1. of the reference D420900800005 originating from Nudat2 database. D420900800006 STATUS (TABLE)Numerical data were taken from table 2. D420900800007 ENDBIB 5 0 D420900800008 NOCOMMON 0 0 D420900800009 DATA 4 2 D420900800010 EN EN-ERR DATA ERR-T D420900800011 MEV MEV MB MB D420900800012 36.8 0.3 17.8 5.5 D420900800013 33.0 0.4 2.9 0.6 D420900800014 ENDDATA 4 0 D420900800015 ENDSUBENT 14 0 D420900899999 SUBENT D4209009 20090325 D066D420900900001 BIB 3 5 D420900900002 REACTION (59-PR-141(D,X)57-LA-140,,SIG) D420900900003 DECAY-DATA (57-LA-140,40.27HR,DG,1596.2,0.954) D420900900004 Decay data were taken from table 1. of the reference D420900900005 originating from Nudat2 database. D420900900006 STATUS (TABLE)Numerical data were taken from table 2. D420900900007 ENDBIB 5 0 D420900900008 NOCOMMON 0 0 D420900900009 DATA 4 5 D420900900010 EN EN-ERR DATA ERR-T D420900900011 MEV MEV MB MB D420900900012 39.9 0.2 1.6 0.3 D420900900013 36.8 0.3 2.3 0.4 D420900900014 33.0 0.4 2.9 0.5 D420900900015 28.7 0.5 3.8 0.6 D420900900016 23.8 0.6 3.5 0.5 D420900900017 ENDDATA 7 0 D420900900018 ENDSUBENT 17 0 D420900999999 SUBENT D4209010 20151007 D101D420901000001 BIB 4 7 D420901000002 REACTION (69-TM-169(D,2N)70-YB-169,,SIG) D420901000003 DECAY-DATA (70-YB-169-G,32.0D,DG,197.4,0.358) D420901000004 Decay data were taken from table 1. of the reference D420901000005 originating from Nudat2 database. D420901000006 STATUS (TABLE)Numerical data were taken from table 2. D420901000007 HISTORY (20151007A) VS data at 20.5 MeV and below (except at D420901000008 19.7 MeV) were deleted due to dupl. with D4180.002 D420901000009 ENDBIB 7 0 D420901000010 NOCOMMON 0 0 D420901000011 DATA 4 10 D420901000012 EN EN-ERR DATA ERR-T D420901000013 MEV MEV MB MB D420901000014 38.6 0.3 76.0 20.0 D420901000015 37.2 0.3 57.0 17.0 D420901000016 35.5 0.4 97.0 22.0 D420901000017 34.0 0.4 76.0 15.0 D420901000018 31.5 0.5 86.0 16.0 D420901000019 29.8 0.5 101.0 18.0 D420901000020 27.0 0.6 120.0 21.0 D420901000021 25.1 0.7 134.0 23.0 D420901000022 21.9 0.8 169.0 28.0 D420901000023 19.7 0.9 277.0 35.0 D420901000024 ENDDATA 12 0 D420901000025 ENDSUBENT 24 0 D420901099999 SUBENT D4209011 20090325 D066D420901100001 BIB 3 5 D420901100002 REACTION (69-TM-169(D,5N)70-YB-166,,SIG) D420901100003 DECAY-DATA (70-YB-166,56.7HR,DG,82.3,0.152) D420901100004 Decay data were taken from table 1. of the reference D420901100005 originating from Nudat2 database. D420901100006 STATUS (TABLE)Numerical data were taken from table 2. D420901100007 ENDBIB 5 0 D420901100008 NOCOMMON 0 0 D420901100009 DATA 4 4 D420901100010 EN EN-ERR DATA ERR-T D420901100011 MEV MEV MB MB D420901100012 38.6 0.3 413.0 47.0 D420901100013 37.2 0.3 286.0 33.0 D420901100014 35.5 0.4 108.0 14.0 D420901100015 34.0 0.4 51.0 6.0 D420901100016 ENDDATA 6 0 D420901100017 ENDSUBENT 16 0 D420901199999 SUBENT D4209012 20151007 D101D420901200001 BIB 4 7 D420901200002 REACTION (69-TM-169(D,X)69-TM-168,,SIG) D420901200003 DECAY-DATA (69-TM-168,93.1D,DG,815.9,0.503) D420901200004 Decay data were taken from table 1. of the reference D420901200005 originating from Nudat2 database. D420901200006 STATUS (TABLE)Numerical data were taken from table 2. D420901200007 HISTORY (20151007A) VS data at 20.5 MeV and below were D420901200008 deleted due to dupl. with D4180.003 D420901200009 ENDBIB 7 0 D420901200010 NOCOMMON 0 0 D420901200011 DATA 4 6 D420901200012 EN EN-ERR DATA ERR-T D420901200013 MEV MEV MB MB D420901200014 38.6 0.3 250.0 50.0 D420901200015 37.2 0.3 298.0 53.0 D420901200016 35.5 0.4 237.0 51.0 D420901200017 34.0 0.4 269.0 45.0 D420901200018 31.5 0.5 231.0 44.0 D420901200019 29.8 0.5 166.0 39.0 D420901200020 ENDDATA 8 0 D420901200021 ENDSUBENT 20 0 D420901299999 SUBENT D4209013 20151007 D101D420901300001 BIB 4 7 D420901300002 REACTION (69-TM-169(D,X)69-TM-167,CUM,SIG) D420901300003 DECAY-DATA (69-TM-167,9.25D,DG,207.8,0.42) D420901300004 Decay data were taken from table 1. of the reference D420901300005 originating from Nudat2 database. D420901300006 STATUS (TABLE)Numerical data were taken from table 2. D420901300007 HISTORY (20151007A) VS data at 20.5 MeV and below were D420901300008 deleted due to dupl. with D4180.004 D420901300009 ENDBIB 7 0 D420901300010 NOCOMMON 0 0 D420901300011 DATA 4 8 D420901300012 EN EN-ERR DATA ERR-T D420901300013 MEV MEV MB MB D420901300014 38.6 0.3 863.0 97.0 D420901300015 37.2 0.3 908.0 102.0 D420901300016 35.5 0.4 924.0 104.0 D420901300017 34.0 0.4 1033.0 116.0 D420901300018 31.5 0.5 881.0 99.0 D420901300019 29.8 0.5 705.0 79.0 D420901300020 27.0 0.6 415.0 47.0 D420901300021 25.1 0.7 158.0 18.0 D420901300022 ENDDATA 10 0 D420901300023 ENDSUBENT 22 0 D420901399999 SUBENT D4209014 20090325 D066D420901400001 BIB 3 5 D420901400002 REACTION (69-TM-169(D,X)69-TM-166,CUM,SIG) D420901400003 DECAY-DATA (69-TM-166,7.7HR,DG,785.9,0.099) D420901400004 Decay data were taken from table 1. of the reference D420901400005 originating from Nudat2 database. D420901400006 STATUS (TABLE)Numerical data were taken from table 2. D420901400007 ENDBIB 5 0 D420901400008 NOCOMMON 0 0 D420901400009 DATA 4 4 D420901400010 EN EN-ERR DATA ERR-T D420901400011 MEV MEV MB MB D420901400012 38.6 0.3 475.0 56.0 D420901400013 37.2 0.3 302.0 36.0 D420901400014 35.5 0.4 116.0 17.0 D420901400015 34.0 0.4 52.0 8.0 D420901400016 ENDDATA 6 0 D420901400017 ENDSUBENT 16 0 D420901499999 ENDENTRY 14 0 D420999999999