ENTRY D4320 20151007 D101D432000000001 SUBENT D4320001 20151007 D101D432000100001 BIB 13 69 D432000100002 TITLE Production of 111In and 114mIn by proton induced D432000100003 reactions: an update on excitation functions, chemical D432000100004 separation - purification and recovery of target D432000100005 material D432000100006 AUTHOR (A.Hermanne,R.Adam-Rebeles,P.Van den Winkel, D432000100007 F.Tarkanyi,S.Takacs) D432000100008 INSTITUTE (2BLGVUB,3HUNDEB) D432000100009 REFERENCE (J,RCA,102,1111,2014) D432000100010 #doi:10.1515/ract-2013-2233 D432000100011 FACILITY (CYCLO,2BLGVUB) D432000100012 (CYCLO,2BLGLVN) D432000100013 SAMPLE Enriched 112Cd elecroplated onto Cu backing with D432000100014 the following isotopic composition: D432000100015 -48-CD-116, enrichment not given D432000100016 -48-CD-114, enrichment <0.008 D432000100017 -48-CD-113, enrichment <0.008 D432000100018 -48-CD-112, enrichment >0.976 D432000100019 -48-CD-111, enrichment <0.006 D432000100020 -48-CD-110, enrichment <0.002 D432000100021 -48-CD-108, enrichment not given D432000100022 -48-CD-106, enrichment not given D432000100023 Enriched 114Cd elecroplated onto Cu backing. D432000100024 (48-CD-116,ENR=0.0023) D432000100025 (48-CD-114,ENR=0.9901) D432000100026 (48-CD-113,ENR=0.0026) D432000100027 (48-CD-112,ENR=0.0032) D432000100028 (48-CD-111,ENR=0.0010) D432000100029 (48-CD-110,ENR=0.0008) D432000100030 (48-CD-108,ENR=0.00005) D432000100031 (48-CD-106,ENR=0.00005) D432000100032 DETECTOR (HPGE) D432000100033 METHOD (ACTIV,EXTB,EDEG,GSPEC,MOSEP,STTA) Two stacks D432000100034 consisting of 112Cd on Cu-backing targets interleaved D432000100035 with Al degraders, were irradiated with a 36.7 MeV and D432000100036 25 MeV protons. The second stack contained also 114Cd D432000100037 targets. Irradiation was done in a Faraday-cup type D432000100038 target holder with proton beams of 100nA for 40 and 60 D432000100039 minutes. Beam intensity was monitored by using Cu D432000100040 monitor reactions. Activity was measured with no D432000100041 chemical separation. Several series of spectra were D432000100042 recorded to be able to follow the decay. Decay data D432000100043 were taken from NUDAT online data library. D432000100044 MONITOR (29-CU-0(P,X)30-ZN-65,,SIG) D432000100045 (29-CU-0(P,X)30-ZN-62,,SIG) D432000100046 MONIT-REF (,F.TARKANYI+,R,IAEA-NDS-1211,2001) D432000100047 ERR-ANALYS (EN-ERR)Uncertainty on the energy scale includes D432000100048 cumulative effects of initial beam energy, stopping D432000100049 estimation influenced by target thickness and beam D432000100050 straggling. Throughout the stack it increases from D432000100051 0.2MeV for the first foil to 1.4MeV at the last foil D432000100052 for the 36.7MeV irradiation and to 1.1MeV for the D432000100053 25.0MeV experiment. D432000100054 (ERR-T)The uncertainty on the cross section values D432000100055 are estimated in the standard way as the square root D432000100056 of the quadratic summation of the independently D432000100057 contributing parameters. Uncertainty of time D432000100058 parameters is not included. Overall uncertainty were D432000100059 10-13%. D432000100060 (ERR-1)surface density of target nuclei(5%), D432000100061 (ERR-2)incident charged particle flux (7%), D432000100062 (ERR-3)nuclear decay and branching data(3%) D432000100063 (ERR-4)detector efficiency (5%) D432000100064 (ERR-S,2.0,8.0)statistical and peak fitting (2-8%) D432000100065 ADD-RES (THEO) The experimental data were compared to the D432000100066 results of the theoretical model codes TENDL-2012. D432000100067 (COMP) The measured experimental data were compared to D432000100068 those found in the literature. D432000100069 HISTORY (20150311C) ts D432000100070 (20151007A) VS SAMPLE modified D432000100071 ENDBIB 69 0 D432000100072 COMMON 4 3 D432000100073 ERR-1 ERR-2 ERR-3 ERR-4 D432000100074 PER-CENT PER-CENT PER-CENT PER-CENT D432000100075 5. 7. 3. 5. D432000100076 ENDCOMMON 3 0 D432000100077 ENDSUBENT 76 0 D432000199999 SUBENT D4320002 20150311 D098D432000200001 BIB 3 4 D432000200002 REACTION (48-CD-112(P,2N)49-IN-111,,SIG) D432000200003 DECAY-DATA (49-IN-111-G,67.32HR,DG,171.28,0.907,DG,245.35,0.94) D432000200004 STATUS (TABLE)Decay data are taken from Table1 and D432000200005 Data are taken from Table2 of the publication. D432000200006 ENDBIB 4 0 D432000200007 NOCOMMON 0 0 D432000200008 DATA 4 36 D432000200009 EN EN-ERR DATA ERR-T D432000200010 MEV MEV MB MB D432000200011 10.1 1.2 94. 10. D432000200012 10.9 1.1 380. 42. D432000200013 11.6 1.0 686. 75. D432000200014 13.0 0.9 883. 97. D432000200015 13.6 0.7 520. 57. D432000200016 14.3 0.9 938. 103. D432000200017 15.5 0.8 1051. 116. D432000200018 16.0 0.6 894. 98. D432000200019 16.7 0.8 1029. 113. D432000200020 17.8 0.7 1062. 117. D432000200021 18.2 0.5 1021. 112. D432000200022 18.9 0.7 1123. 124. D432000200023 19.9 0.7 1177. 129. D432000200024 20.1 0.4 1075. 118. D432000200025 20.9 0.6 1118. 123. D432000200026 21.8 0.6 1016. 112. D432000200027 21.9 0.3 1116. 123. D432000200028 22.7 0.6 886. 98. D432000200029 23.6 0.6 752. 83. D432000200030 23.7 0.2 1031. 113. D432000200031 24.5 0.5 672. 74. D432000200032 25.3 0.5 573. 63. D432000200033 26.2 0.5 467. 51. D432000200034 27.0 0.5 370. 41. D432000200035 27.7 0.4 333. 37. D432000200036 28.5 0.4 308. 34. D432000200037 29.3 0.4 271. 30. D432000200038 30.0 0.4 258. 28. D432000200039 30.7 0.4 219. 24. D432000200040 31.4 0.3 201. 22. D432000200041 32.1 0.3 208. 23. D432000200042 32.8 0.3 178. 20. D432000200043 33.4 0.3 176. 19. D432000200044 34.1 0.2 161. 18. D432000200045 34.7 0.2 159. 18. D432000200046 35.4 0.2 174. 19. D432000200047 ENDDATA 38 0 D432000200048 ENDSUBENT 47 0 D432000299999 SUBENT D4320003 20150311 D098D432000300001 BIB 3 4 D432000300002 REACTION (48-CD-112(P,3N)49-IN-110-M,,SIG) D432000300003 DECAY-DATA (49-IN-110-M,1.15HR,DG,657.75,0.98) D432000300004 STATUS (TABLE)Decay data are taken from Table1 and D432000300005 Data are taken from Table2 of the publication. D432000300006 ENDBIB 4 0 D432000300007 NOCOMMON 0 0 D432000300008 DATA 4 22 D432000300009 EN EN-ERR DATA ERR-T D432000300010 MEV MEV MB MB D432000300011 19.9 0.7 15.0 3.6 D432000300012 20.9 0.6 24. 6. D432000300013 21.8 0.6 65. 16. D432000300014 22.7 0.6 155. 37. D432000300015 23.6 0.6 217. 52. D432000300016 23.7 0.2 41. 5. D432000300017 24.5 0.5 276. 66. D432000300018 25.3 0.5 312. 75. D432000300019 26.2 0.5 365. 88. D432000300020 27.0 0.5 319. 77. D432000300021 27.7 0.4 381. 91. D432000300022 28.5 0.4 310. 74. D432000300023 29.3 0.4 399. 96. D432000300024 30.0 0.4 246. 59. D432000300025 30.7 0.4 397. 95. D432000300026 31.4 0.3 234. 56. D432000300027 32.1 0.3 369. 89. D432000300028 32.8 0.3 273. 65. D432000300029 33.4 0.3 325. 78. D432000300030 34.1 0.2 146. 35. D432000300031 34.7 0.2 226. 54. D432000300032 35.4 0.2 155. 37. D432000300033 ENDDATA 24 0 D432000300034 ENDSUBENT 33 0 D432000399999 SUBENT D4320004 20150311 D098D432000400001 BIB 3 5 D432000400002 REACTION (48-CD-112(P,3N)49-IN-110-G,,SIG) D432000400003 DECAY-DATA (49-IN-110-G,4.9HR,DG,641.68,0.26,DG,884.67,0.93, D432000400004 DG,937.48,0.68,DG,657.75,0.98) D432000400005 STATUS (TABLE)Decay data are taken from Table1 and D432000400006 Data are taken from Table2 of the publication. D432000400007 ENDBIB 5 0 D432000400008 NOCOMMON 0 0 D432000400009 DATA 4 21 D432000400010 EN EN-ERR DATA ERR-T D432000400011 MEV MEV MB MB D432000400012 19.9 0.7 2.5 0.3 D432000400013 20.9 0.6 15.2 2.0 D432000400014 21.8 0.6 47. 5. D432000400015 22.7 0.6 87. 10. D432000400016 23.6 0.6 141. 15. D432000400017 24.5 0.5 191. 21. D432000400018 25.3 0.5 258. 28. D432000400019 26.2 0.5 283. 31. D432000400020 27.0 0.5 296. 33. D432000400021 27.7 0.4 331. 36. D432000400022 28.5 0.4 367. 40. D432000400023 29.3 0.4 362. 40. D432000400024 30.0 0.4 404. 44. D432000400025 30.7 0.4 389. 43. D432000400026 31.4 0.3 395. 43. D432000400027 32.1 0.3 407. 45. D432000400028 32.8 0.3 374. 41. D432000400029 33.4 0.3 379. 42. D432000400030 34.1 0.2 368. 40. D432000400031 34.7 0.2 330. 36. D432000400032 35.4 0.2 340. 37. D432000400033 ENDDATA 23 0 D432000400034 ENDSUBENT 33 0 D432000499999 SUBENT D4320005 20150311 D098D432000500001 BIB 3 4 D432000500002 REACTION (48-CD-112(P,4N)49-IN-109,,SIG) D432000500003 DECAY-DATA (49-IN-109-G,4.17HR,DG,203.5,0.735,DG,623.5,0.055) D432000500004 STATUS (TABLE)Decay data are taken from Table1 and D432000500005 Data are taken from Table2 of the publication. D432000500006 ENDBIB 4 0 D432000500007 NOCOMMON 0 0 D432000500008 DATA 4 12 D432000500009 EN EN-ERR DATA ERR-T D432000500010 MEV MEV MB MB D432000500011 27.7 0.4 2.0 0.3 D432000500012 28.5 0.4 1.9 0.3 D432000500013 29.3 0.4 1.9 0.2 D432000500014 30.0 0.4 7.1 0.9 D432000500015 30.7 0.4 10. 1. D432000500016 31.4 0.3 20. 2. D432000500017 32.1 0.3 41. 5. D432000500018 32.8 0.3 61. 7. D432000500019 33.4 0.3 95. 10. D432000500020 34.1 0.2 124. 14. D432000500021 34.7 0.2 161. 18. D432000500022 35.4 0.2 203. 22. D432000500023 ENDDATA 14 0 D432000500024 ENDSUBENT 23 0 D432000599999 SUBENT D4320006 20150311 D098D432000600001 BIB 3 4 D432000600002 REACTION (48-CD-114(P,2N)49-IN-113-M,,SIG) D432000600003 DECAY-DATA (49-IN-113-M,1.66HR,DG,391.7,0.649) D432000600004 STATUS (TABLE)Decay data are taken from Table1 and D432000600005 Data are taken from Table4 of the publication. D432000600006 ENDBIB 4 0 D432000600007 NOCOMMON 0 0 D432000600008 DATA 4 8 D432000600009 EN EN-ERR DATA ERR-T D432000600010 MEV MEV MB MB D432000600011 9.3 0.8 3.0 0.4 D432000600012 12.3 0.7 271. 30. D432000600013 14.9 0.6 330. 36. D432000600014 17.1 0.5 344. 38. D432000600015 19.2 0.4 310. 34. D432000600016 21.1 0.3 279. 31. D432000600017 22.8 0.3 207. 23. D432000600018 24.5 0.2 136. 15. D432000600019 ENDDATA 10 0 D432000600020 ENDSUBENT 19 0 D432000699999 SUBENT D4320007 20150311 D098D432000700001 BIB 3 4 D432000700002 REACTION (48-CD-114(P,N)49-IN-114-M,,SIG) D432000700003 DECAY-DATA (49-IN-114-M,49.5D,DG,190.27,0.155,DG,558.43,0.032) D432000700004 STATUS (TABLE)Decay data are taken from Table1 and D432000700005 Data are taken from Table4 of the publication. D432000700006 ENDBIB 4 0 D432000700007 NOCOMMON 0 0 D432000700008 DATA 4 9 D432000700009 EN EN-ERR DATA ERR-T D432000700010 MEV MEV MB MB D432000700011 24.5 0.2 38. 4. D432000700012 22.8 0.3 40. 4. D432000700013 21.1 0.3 45. 5. D432000700014 19.2 0.4 44. 5. D432000700015 17.1 0.5 70. 8. D432000700016 14.9 0.6 107. 12. D432000700017 12.3 0.7 261. 29. D432000700018 9.3 0.8 343. 38. D432000700019 5.2 1.0 31. 3. D432000700020 ENDDATA 11 0 D432000700021 ENDSUBENT 20 0 D432000799999 ENDENTRY 7 0 D432099999999