ENTRY D4322 20190211 D119D432200000001 SUBENT D4322001 20190211 D119D432200100001 BIB 13 58 D432200100002 TITLE Reexamination of cross sections of the D432200100003 100Mo(p,2n)99mTc reaction D432200100004 AUTHOR (S.Takacs,A.Hermanne,F.Ditroi,F.Tarkanyi,M.Aikawa) D432200100005 INSTITUTE (3HUNDEB,2BLGVUB) D432200100006 REFERENCE (J,NIM/B,347,26,2015) D432200100007 #doi:10.1016/j.nimb.2015.01.056 D432200100008 FACILITY (CYCLO,3HUNDEB) D432200100009 (CYCLO,2BLGVUB) D432200100010 SAMPLE Target foils were 10 x 10 mm rectangular Mo foils with D432200100011 natural isotopic composition from Goodfellow, UK D432200100012 measured average thickness 11.98 um, chemical purity: D432200100013 99.9%. Atomic weight: 95.96(2)g. D432200100014 (42-MO-92,NAT=0.14525) D432200100015 (42-MO-94,NAT=0.091514) D432200100016 (42-MO-95,NAT=0.158375) D432200100017 (42-MO-96,NAT=0.16672) D432200100018 (42-MO-97,NAT=0.09599) D432200100019 (42-MO-98,NAT=0.24391) D432200100020 (42-MO-100,NAT=0.09824) D432200100021 DETECTOR (HPGE) D432200100022 METHOD (ACTIV) Activation method was used. Irradiation were D432200100023 done at 16 and 36.4 MeV proton energies. D432200100024 (EXTB) The beam was extracted from the cyclotron and D432200100025 the irradiation was done in a Faraday-type target D432200100026 holder. D432200100027 (STTA) Stacked target irradiation technique was D432200100028 applied. D432200100029 (EDEG) Energy degradation in each layers the stack D432200100030 was calculated by using the semi-empirical polynomial D432200100031 formula of Ziegler and Andersen. D432200100032 (GSPEC) Non-destructive gamma-spectrometry was used. D432200100033 (MOSEP) The beam energy and intensity were monitored D432200100034 by natTi(p,x)V48 reaction. D432200100035 MONITOR (22-TI-0(P,X)23-V-48,,SIG) D432200100036 MONIT-REF (,F.TARKANYI+,R,IAEA-NDS-1211,2001) D432200100037 ERR-ANALYS (EN-ERR)Uncertainty on the energy scale includes D432200100038 cumulative effects of initial beam energy, stopping D432200100039 estimation influenced by target thickness and beam D432200100040 straggling. Throughout the stack it increases from D432200100041 0.25MeV for the first foil to 0.45MeV for 16MeV proton D432200100042 irradiation and 1.56 MeV for the 36MeV irradiation. D432200100043 (ERR-T)The uncertainty on the cross section values D432200100044 are estimated in the standard way as the square root D432200100045 of the quadratic summation of the independently D432200100046 contributing parameters. Uncertainty of time D432200100047 parameters is not included. Overall uncertainty were D432200100048 6-12%. D432200100049 (ERR-1)surface density of target nuclei(1%), D432200100050 (ERR-2)incident charged particle flux (3%), D432200100051 (ERR-3)nuclear decay and branching data(3%) D432200100052 (ERR-4)detector efficiency (3%) D432200100053 (ERR-S,2.0,10.0)statistical and peak fitting (2-10%) D432200100054 ADD-RES (THEO) The experimental data were compared to the D432200100055 results of the theoretical model codes TENDL-2013. D432200100056 (COMP) The measured experimental data were compared to D432200100057 those found in the literature. D432200100058 HISTORY (20150316C) ts D432200100059 (20190211A) So NDS, Major revision in 002 and 004 D432200100060 ENDBIB 58 0 D432200100061 COMMON 4 3 D432200100062 ERR-1 ERR-2 ERR-3 ERR-4 D432200100063 PER-CENT PER-CENT PER-CENT PER-CENT D432200100064 1. 3. 3. 3. D432200100065 ENDCOMMON 3 0 D432200100066 ENDSUBENT 65 0 D432200199999 SUBENT D4322002 20190211 D119D432200200001 BIB 4 6 D432200200002 REACTION (42-MO-100(P,2N)43-TC-99-M,,SIG) D432200200003 DECAY-DATA (43-TC-99-M,6.0082HR,DG,140.5,0.885) D432200200004 STATUS (TABLE)Data are taken from Table4. D432200200005 Direct production, contribution of decay production andD432200200006 99Mo decay is subtracted. D432200200007 HISTORY (20190211A) REACTION(SF5): IND deleted D432200200008 ENDBIB 6 0 D432200200009 NOCOMMON 0 0 D432200200010 DATA 4 34 D432200200011 EN EN-ERR DATA ERR-T D432200200012 MEV MEV MB MB D432200200013 35.54 0.32 25.4 3.0 D432200200014 34.09 0.35 34.2 4.0 D432200200015 32.60 0.39 28.8 3.4 D432200200016 31.04 0.43 35.7 4.2 D432200200017 29.42 0.47 36.0 4.3 D432200200018 27.73 0.51 34.8 4.1 D432200200019 26.18 0.57 47.5 5.6 D432200200020 24.80 0.62 77.1 9.1 D432200200021 23.37 0.68 89.7 10.6 D432200200022 21.85 0.75 119.4 14.1 D432200200023 20.26 0.83 163.6 19.4 D432200200024 18.56 0.91 212.6 25.2 D432200200025 16.73 1.00 220.1 26.0 D432200200026 15.89 0.25 230.2 15.6 D432200200027 15.68 0.25 237.5 16.2 D432200200028 15.35 0.26 230.0 15.7 D432200200029 15.13 0.27 231.2 15.7 D432200200030 14.78 0.27 232.8 15.9 D432200200031 14.74 1.10 231.6 27.4 D432200200032 14.56 0.28 230.8 15.7 D432200200033 14.21 0.29 230.7 15.7 D432200200034 13.97 0.29 228.8 15.6 D432200200035 13.61 0.30 228.4 15.5 D432200200036 13.37 0.30 227.7 15.5 D432200200037 13.00 0.31 226.6 15.2 D432200200038 12.75 0.32 219.7 14.9 D432200200039 12.51 1.21 214.7 25.4 D432200200040 12.10 0.33 212.2 14.4 D432200200041 11.43 0.35 197.2 13.4 D432200200042 10.72 0.36 169.9 11.5 D432200200043 9.99 0.38 129.6 8.9 D432200200044 9.93 1.33 121.6 14.4 D432200200045 9.21 0.40 72.2 5.1 D432200200046 8.38 0.41 13.3 1.3 D432200200047 ENDDATA 36 0 D432200200048 ENDSUBENT 47 0 D432200299999 SUBENT D4322003 20150316 D099D432200300001 BIB 3 6 D432200300002 REACTION (42-MO-100(P,X)42-MO-99,CUM,SIG) D432200300003 DECAY-DATA (42-MO-99,65.9496HR,DG,140.5,0.0472,DG,181.1,0.0601, D432200300004 DG,739.5,0.1212) D432200300005 STATUS (TABLE)Data are taken from Table4. D432200300006 Cumulative production includes possible decay D432200300007 production from 99Nb. D432200300008 ENDBIB 6 0 D432200300009 NOCOMMON 0 0 D432200300010 DATA 4 28 D432200300011 EN EN-ERR DATA ERR-T D432200300012 MEV MEV MB MB D432200300013 35.54 0.32 185.8 16.5 D432200300014 34.09 0.35 180.6 16.3 D432200300015 32.60 0.39 181.6 16.8 D432200300016 31.04 0.43 183.0 17.8 D432200300017 29.42 0.47 174.9 17.4 D432200300018 27.73 0.51 178.8 16.6 D432200300019 26.18 0.57 169.8 15.5 D432200300020 24.80 0.62 169.1 15.3 D432200300021 23.37 0.68 165.0 16.5 D432200300022 21.85 0.75 148.0 13.6 D432200300023 20.26 0.83 120.3 13.0 D432200300024 18.56 0.91 94.8 9.2 D432200300025 16.73 1.00 68.4 10.2 D432200300026 15.89 0.25 41.9 3.88 D432200300027 15.68 0.25 38.4 3.44 D432200300028 15.35 0.26 33.2 4.34 D432200300029 15.13 0.27 30.3 2.78 D432200300030 14.78 0.27 25.2 2.79 D432200300031 14.74 1.10 30.6 5.4 D432200300032 14.56 0.28 24.1 1.34 D432200300033 14.21 0.29 18.4 2.99 D432200300034 13.97 0.29 17.3 3.11 D432200300035 13.61 0.30 12.6 1.17 D432200300036 13.37 0.30 11.6 1.29 D432200300037 13.00 0.31 5.8 0.69 D432200300038 12.75 0.32 7.9 2.69 D432200300039 12.51 1.21 7.4 5.6 D432200300040 11.43 0.35 5.4 0.73 D432200300041 ENDDATA 30 0 D432200300042 ENDSUBENT 41 0 D432200399999 SUBENT D4322004 20190211 D119D432200400001 BIB 4 10 D432200400002 REACTION (42-MO-100(P,2N)43-TC-99-M,,SIG) D432200400003 DECAY-DATA (43-TC-99-M,6.0082HR,DG,140.5,0.885) D432200400004 STATUS (TABLE)Data are taken from Table5. D432200400005 Re-evaluated data of Takacs et al. J. Radioanal. D432200400006 Nucl. Chem. 257 (2003) 195-201 with up to date decay D432200400007 parameters. D432200400008 Direct production, contribution of decay production andD432200400009 99Mo decay is subtracted. D432200400010 Supersedes data of D4115002 D432200400011 HISTORY (20190211A) REACTION(SF5): IND deleted D432200400012 ENDBIB 10 0 D432200400013 NOCOMMON 0 0 D432200400014 DATA 4 23 D432200400015 EN EN-ERR DATA ERR-T D432200400016 MEV MEV MB MB D432200400017 37.9 0.3 6.8 0.6 D432200400018 36.5 0.3 9.0 0.8 D432200400019 35.3 0.4 22.6 2.0 D432200400020 33.9 0.4 20.1 1.8 D432200400021 32.5 0.4 28.2 2.5 D432200400022 31.0 0.4 27.7 2.5 D432200400023 29.4 0.5 29.0 2.6 D432200400024 27.8 0.5 29.2 2.6 D432200400025 26.1 0.6 41.8 3.8 D432200400026 24.9 0.3 31.8 8.1 D432200400027 24.3 0.6 56.6 5.1 D432200400028 23.6 0.33 49.2 10.8 D432200400029 22.8 0.7 85.9 7.7 D432200400030 22.2 0.36 88.3 18.7 D432200400031 21.4 0.7 134.5 12.1 D432200400032 20.7 0.4 140.5 24.1 D432200400033 19.8 0.8 176.9 15.9 D432200400034 19.2 0.44 196.0 29.4 D432200400035 17.5 0.48 231.2 33.4 D432200400036 15.7 0.53 232.6 33.4 D432200400037 13.8 0.58 233.1 32.5 D432200400038 11.6 0.64 203.2 39.2 D432200400039 9.0 0.71 33.0 11.5 D432200400040 ENDDATA 25 0 D432200400041 ENDSUBENT 40 0 D432200499999 SUBENT D4322005 20150316 D099D432200500001 BIB 3 10 D432200500002 REACTION (42-MO-100(P,X)42-MO-99,CUM,SIG) D432200500003 DECAY-DATA (42-MO-99,65.9496HR,DG,140.5,0.0472,DG,181.1,0.0601, D432200500004 DG,739.5,0.1212) D432200500005 STATUS (TABLE)Data are taken from Table5. D432200500006 Re-evaluated data of Takacs et al. J. Radioanal. D432200500007 Nucl. Chem. 257 (2003) 195-201 with up to date decay D432200500008 parameters. D432200500009 Cumulative production includes possible decay D432200500010 production from 99Nb. D432200500011 Supersedes data of D4115002 D432200500012 ENDBIB 10 0 D432200500013 NOCOMMON 0 0 D432200500014 DATA 4 23 D432200500015 EN EN-ERR DATA ERR-T D432200500016 MEV MEV MB MB D432200500017 37.9 0.30 178.5 19.8 D432200500018 36.5 0.32 179.1 19.8 D432200500019 35.3 0.35 182.5 20.2 D432200500020 33.9 0.38 184.6 20.5 D432200500021 32.5 0.41 182.1 20.2 D432200500022 31.0 0.44 175.1 19.4 D432200500023 29.4 0.48 179.4 19.9 D432200500024 27.8 0.51 175.9 19.5 D432200500025 26.1 0.56 173.4 19.2 D432200500026 24.9 0.30 173.0 19.4 D432200500027 24.3 0.60 167.9 18.6 D432200500028 23.6 0.33 164.5 18.5 D432200500029 22.8 0.65 154.8 17.2 D432200500030 22.2 0.36 152.9 17.2 D432200500031 21.4 0.70 130.3 14.4 D432200500032 20.7 0.40 130.6 14.7 D432200500033 19.8 0.76 119.6 13.2 D432200500034 19.2 0.44 104.7 11.8 D432200500035 17.5 0.48 75.8 8.5 D432200500036 15.7 0.53 45.4 5.1 D432200500037 13.8 0.58 17.7 2.0 D432200500038 11.6 0.64 3.6 0.6 D432200500039 9.0 0.71 2.0 2.6 D432200500040 ENDDATA 25 0 D432200500041 ENDSUBENT 40 0 D432200599999 SUBENT D4322006 20150316 D099D432200600001 BIB 3 4 D432200600002 REACTION (42-MO-0(P,X)43-TC-95-M,,SIG) D432200600003 DECAY-DATA (43-TC-95-M,61.D,DG,204.0,0.632) D432200600004 STATUS (TABLE)Data are received from authors. D432200600005 EC=96.12% D432200600006 ENDBIB 4 0 D432200600007 NOCOMMON 0 0 D432200600008 DATA 4 46 D432200600009 EN EN-ERR DATA ERR-T D432200600010 MEV MEV MB MB D432200600011 35.54 0.32 30.1 1.9 D432200600012 34.09 0.35 27.9 1.8 D432200600013 32.60 0.39 26.4 1.7 D432200600014 31.04 0.43 25.5 1.6 D432200600015 29.42 0.47 27.2 1.7 D432200600016 27.73 0.51 31.6 2.0 D432200600017 26.18 0.57 36.0 2.3 D432200600018 24.80 0.62 41.6 2.7 D432200600019 23.37 0.68 45.9 2.9 D432200600020 21.85 0.75 46.7 3.0 D432200600021 20.26 0.83 47.4 3.0 D432200600022 18.56 0.91 49.2 3.2 D432200600023 16.73 1.00 52.3 3.4 D432200600024 15.89 0.25 51.0 4.5 D432200600025 15.68 0.25 50.8 4.5 D432200600026 15.35 0.26 50.9 4.5 D432200600027 15.13 0.27 50.8 4.5 D432200600028 14.78 0.27 50.0 4.4 D432200600029 14.74 1.10 51.0 3.3 D432200600030 14.56 0.28 49.2 4.3 D432200600031 14.21 0.29 47.9 4.2 D432200600032 13.97 0.29 47.8 4.2 D432200600033 13.61 0.30 44.3 3.9 D432200600034 13.37 0.30 43.4 3.8 D432200600035 13.00 0.31 40.7 3.6 D432200600036 12.75 0.32 38.6 3.4 D432200600037 12.51 1.21 40.2 2.6 D432200600038 12.36 0.33 35.4 3.1 D432200600039 12.10 0.33 33.7 3.0 D432200600040 11.69 0.34 33.6 3.0 D432200600041 11.43 0.35 33.7 3.0 D432200600042 11.00 0.36 33.2 2.9 D432200600043 10.72 0.36 32.4 2.9 D432200600044 10.28 0.37 31.3 2.8 D432200600045 9.99 0.38 29.8 2.6 D432200600046 9.93 1.33 30.3 1.9 D432200600047 9.52 0.39 27.5 2.4 D432200600048 9.21 0.40 26.3 2.3 D432200600049 8.71 0.41 23.2 2.1 D432200600050 8.38 0.41 21.4 1.9 D432200600051 7.85 0.43 17.8 1.6 D432200600052 7.49 0.43 15.9 1.4 D432200600053 6.91 0.45 12.1 1.1 D432200600054 6.71 1.47 11.5 0.7 D432200600055 6.52 0.45 9.8 0.9 D432200600056 5.27 1.56 5.2 0.3 D432200600057 ENDDATA 48 0 D432200600058 ENDSUBENT 57 0 D432200699999 SUBENT D4322007 20150316 D099D432200700001 BIB 3 4 D432200700002 REACTION (42-MO-0(P,X)43-TC-96-G,M+,SIG) D432200700003 DECAY-DATA (43-TC-96-G,4.28D,DG,314.28,0.0243,DG,812.540,0.82) D432200700004 STATUS (TABLE)Data are received from authors. D432200700005 Includes 96mTc (IT:98%) D432200700006 ENDBIB 4 0 D432200700007 NOCOMMON 0 0 D432200700008 DATA 4 18 D432200700009 EN EN-ERR DATA ERR-T D432200700010 MEV MEV MB MB D432200700011 35.54 0.32 115.4 10.2 D432200700012 34.09 0.35 137.0 12.1 D432200700013 32.60 0.39 163.1 14.4 D432200700014 31.04 0.43 178.4 15.8 D432200700015 29.42 0.47 184.1 16.3 D432200700016 27.73 0.51 184.7 16.3 D432200700017 26.18 0.57 169.0 14.9 D432200700018 24.80 0.62 154.6 13.7 D432200700019 23.37 0.68 129.1 11.4 D432200700020 21.85 0.75 104.2 9.2 D432200700021 20.26 0.83 90.3 8.0 D432200700022 18.56 0.91 92.5 8.2 D432200700023 16.73 1.00 94.2 8.4 D432200700024 14.74 1.10 106.9 9.5 D432200700025 12.51 1.21 130.5 11.6 D432200700026 9.93 1.33 92.2 8.2 D432200700027 6.71 1.47 32.9 2.9 D432200700028 5.27 1.56 13.9 1.2 D432200700029 ENDDATA 20 0 D432200700030 ENDSUBENT 29 0 D432200799999 ENDENTRY 7 0 D432299999999