ENTRY D5048 20080729 D062D504800000001 SUBENT D5048001 20080729 D062D504800100001 BIB 16 55 D504800100002 TITLE Excitation functions of 3He-particle induced reactions D504800100003 on 101Ru and 102Ru for production of the medically D504800100004 interesting radionuclide 101mRh D504800100005 AUTHOR (Ye.Skakun, S.M.Qaim) D504800100006 INSTITUTE (4UKRKFT) D504800100007 (2GERJUL) D504800100008 REFERENCE (C,2007NICE,2,1379,2007) D504800100009 SAMPLE The foils of the 2-5 mg/cm**2 thickness and 16-mm D504800100010 diameter made from the enriched ruthenium isotopes D504800100011 were used. The enrichment of 101Ru amounted to 97.6% D504800100012 and of 102Ru to 99.0%. Titanium and aluminium foils D504800100013 were interspersed between the ruthenium foils: Ti for D504800100014 monitoring He-3 beam and Al for the beam energy D504800100015 absorption along the stack. Three stacks of 101Ru and D504800100016 three of 102Ru were used. D504800100017 INC-SPECT Maximum incident energy was 34 MeV. D504800100018 ADD-RES (TTY-C).The integral thick target yield of the product D504800100019 radionuclide Rh-101m and long-lived impurities Rh-101g,D504800100020 Rh-102m and Rh-102g were calculated from the measured D504800100021 excitation functions. D504800100022 DETECTOR (HPGE) HP(Ge)-detector was used to measure the product D504800100023 activities in Ru samples and Ti monitor foils. The D504800100024 efficiency calibration was done using the standard D504800100025 radioactive sources 57Co, 133Ba, 137Cs, 152Eu, 226Ra D504800100026 and 241Am. D504800100027 CORRECTION Corrections for the number of residual nuclei leaving D504800100028 the thin ruthenium foils and cross contaminations of D504800100029 reactions. D504800100030 FACILITY (CYCLO,2GERJUL) The compact cyclotron CV28. D504800100031 METHOD (STTA) D504800100032 (ACTIV,GSPEC) The activities of all samples were D504800100033 periodically measured over a period of 2 months, D504800100034 watching the half-lives and choosing the best cooling D504800100035 time and the minimum dead time. D504800100036 ERR-ANALYS (DATA-ERR)The overall uncertainty in each cross sectionD504800100037 was calculated as a root-mean square value of the majorD504800100038 contributing errors associated with the measurements ofD504800100039 the surface density of target nuclei , incident D504800100040 particle beam current, detector efficiency, counting D504800100041 statistics, and decay data. D504800100042 STATUS (TABLE) Data were received by e-mail from Dr.Ye.Skakun D504800100043 HISTORY (20070525C)UKRNDC D504800100044 (20080226A) SD: Refence was corrected. D504800100045 (20080724A) SD. Reference on Conf.Proc. was corrected. D504800100046 MONITOR (22-TI-0(HE3,X)21-SC-43,,SIG) D504800100047 (22-TI-0(HE3,X)21-SC-44-M,,SIG) D504800100048 (22-TI-0(HE3,X)21-SC-46,,SIG) D504800100049 (22-TI-0(HE3,X)21-SC-47,,SIG) D504800100050 (22-TI-0(HE3,X)21-SC-48,,SIG) D504800100051 (22-TI-0(HE3,X)23-V-48,,SIG) D504800100052 (22-TI-0(HE3,X)24-CR-48,,SIG) D504800100053 (22-TI-0(HE3,X)24-CR-49,,SIG) D504800100054 (22-TI-0(HE3,X)24-CR-51,,SIG) D504800100055 MONIT-REF (,F.TARKANYI+,R,IAEA-TECDOC-1211,49,2001) D504800100056 (D4112001,F.DITROI+,J,NIM/B,168,337,2000) D504800100057 ENDBIB 55 0 D504800100058 NOCOMMON 0 0 D504800100059 ENDSUBENT 58 0 D504800199999 SUBENT D5048002 20070614 D056D504800200001 BIB 3 5 D504800200002 REACTION (44-RU-101(HE3,X)45-RH-101-M,CUM,SIG) D504800200003 DECAY-DATA (45-RH-101-M,4.34D,DG,306.9,0.806,DG,545.1,0.0427) D504800200004 (46-PD-101,8.47HR,DG,269.7,0.0643,DG,296.3,0.192,DG, D504800200005 590.4,0.1206) D504800200006 STATUS (APRVD,TABLE) Corresponds to fig.1 (dark circle points)D504800200007 ENDBIB 5 0 D504800200008 NOCOMMON 0 0 D504800200009 DATA 3 18 D504800200010 EN DATA DATA-ERR D504800200011 MEV MB MB D504800200012 12.0 1.42 0.28 D504800200013 15.3 6.2 0.8 D504800200014 15.7 98.3 11.0 D504800200015 17.6 113. 11. D504800200016 19.1 437. 40. D504800200017 20.4 407. 37. D504800200018 23.0 767. 69. D504800200019 23.1 667. 60. D504800200020 25.0 1065. 96. D504800200021 25.5 1000. 91. D504800200022 26.8 1148. 103. D504800200023 27.5 1043. 94. D504800200024 28.6 1131. 102. D504800200025 29.5 1040. 94. D504800200026 31.2 1026. 93. D504800200027 31.4 902. 82. D504800200028 33.6 797. 72. D504800200029 33.7 752. 71. D504800200030 ENDDATA 20 0 D504800200031 ENDSUBENT 30 0 D504800299999 SUBENT D5048003 20070614 D056D504800300001 BIB 3 5 D504800300002 REACTION (44-RU-101(HE3,X)45-RH-101-G,CUM,SIG) D504800300003 DECAY-DATA (45-RH-101-G,3.3YR,DG,127.2,0.680,DG,198.0,0.73,DG, D504800300004 325.2,0.118) D504800300005 (45-RH-101-M,4.34D,DG,306.9,0.806,DG,545.1,0.0427) D504800300006 STATUS (APRVD,TABLE) Corresponds to fig.1 (dark square points)D504800300007 ENDBIB 5 0 D504800300008 NOCOMMON 0 0 D504800300009 DATA 3 16 D504800300010 EN DATA DATA-ERR D504800300011 MEV MB MB D504800300012 12.0 0.65 0.16 D504800300013 15.3 3.6 0.8 D504800300014 15.7 15.9 2.9 D504800300015 17.6 20.1 3.2 D504800300016 19.1 71.2 12.8 D504800300017 20.4 64.4 10.4 D504800300018 23.0 136. 22. D504800300019 23.1 111. 16. D504800300020 25.0 177. 25. D504800300021 25.5 187. 27. D504800300022 26.8 214. 30. D504800300023 27.5 225. 30. D504800300024 28.6 221. 29. D504800300025 29.5 230. 30. D504800300026 31.4 217. 26. D504800300027 33.7 206. 25. D504800300028 ENDDATA 18 0 D504800300029 ENDSUBENT 28 0 D504800399999 SUBENT D5048004 20070614 D056D504800400001 BIB 4 7 D504800400002 REACTION (44-RU-101(HE3,X)45-RH-102-M,,SIG) D504800400003 DECAY-DATA (45-RH-102-M,3.742YR,DG,475.1,0.95,DG,628.1,0.083,DG, D504800400004 631.3,0.56,DG,697.5,0.44,DG,766.8,0.34,DG,1046.6,0.34) D504800400005 COMMENT -By authors. In REACTION X corresponds to PN+D. The D504800400006 half-life was given from (,M.Shibata+,J,ARI,49,1481, D504800400007 1998). D504800400008 STATUS (APRVD,TABLE) Corresponds to fig.1 (open circles) D504800400009 ENDBIB 7 0 D504800400010 NOCOMMON 0 0 D504800400011 DATA 3 18 D504800400012 EN DATA DATA-ERR D504800400013 MEV MB MB D504800400014 12.0 8.4 1.1 D504800400015 15.3 32.4 3.3 D504800400016 15.7 72.4 7.2 D504800400017 17.6 84.9 8.3 D504800400018 19.1 124. 12. D504800400019 20.4 137. 13. D504800400020 23.0 132. 13. D504800400021 23.1 145. 14. D504800400022 25.0 131. 13. D504800400023 25.5 123. 12. D504800400024 26.8 114. 11. D504800400025 27.5 108. 11. D504800400026 28.6 99.1 10.2 D504800400027 29.5 85.7 9.5 D504800400028 31.2 66.3 6.8 D504800400029 31.4 69.3 6.9 D504800400030 33.6 60.2 6.0 D504800400031 33.7 67.5 6.9 D504800400032 ENDDATA 20 0 D504800400033 ENDSUBENT 32 0 D504800499999 SUBENT D5048005 20070614 D056D504800500001 BIB 4 5 D504800500002 REACTION (44-RU-101(HE3,X)45-RH-102-G,,SIG) D504800500003 DECAY-DATA (45-RH-102-G,207.3D,DG,475.1,0.46,DG,628.1,0.045,DG, D504800500004 631.3,0.0010) D504800500005 COMMENT -By authors. In REACTION X corresponds to PN+D. D504800500006 STATUS (APRVD,TABLE) Corresponds to fig.1 (open squares) D504800500007 ENDBIB 5 0 D504800500008 NOCOMMON 0 0 D504800500009 DATA 3 18 D504800500010 EN DATA DATA-ERR D504800500011 MEV MB MB D504800500012 12.0 31.3 3.8 D504800500013 15.3 78.4 9.4 D504800500014 15.7 196. 22. D504800500015 17.6 163. 19. D504800500016 19.1 216. 24. D504800500017 20.4 217. 24. D504800500018 23.0 169. 19. D504800500019 23.1 172. 19. D504800500020 25.0 163. 18. D504800500021 25.5 149. 17. D504800500022 26.8 137. 15. D504800500023 27.5 140. 16. D504800500024 28.6 118. 13. D504800500025 29.5 117. 14. D504800500026 31.2 87.8 9.7 D504800500027 31.4 89.2 10.2 D504800500028 33.6 78.8 8.7 D504800500029 33.7 87.1 10.1 D504800500030 ENDDATA 20 0 D504800500031 ENDSUBENT 30 0 D504800599999 SUBENT D5048006 20070614 D056D504800600001 BIB 3 5 D504800600002 REACTION (44-RU-102(HE3,X)45-RH-101-M,CUM,SIG) D504800600003 DECAY-DATA (45-RH-101-M,4.34D,DG,306.9,0.806,DG,545.1,0.0427) D504800600004 (46-PD-101,8.47HR,DG,269.7,0.0643,DG,296.3,0.192,DG, D504800600005 590.4,0.1206) D504800600006 STATUS (APRVD,TABLE) Corresponds to fig.2 (dark circles) D504800600007 ENDBIB 5 0 D504800600008 NOCOMMON 0 0 D504800600009 DATA 3 9 D504800600010 EN DATA DATA-ERR D504800600011 MEV MB MB D504800600012 19.3 3.43 0.69 D504800600013 22.8 6.23 1.00 D504800600014 25.4 13.1 1.9 D504800600015 25.6 16.1 2.0 D504800600016 27.7 79.5 8.8 D504800600017 28.8 176. 18. D504800600018 29.7 253. 23. D504800600019 31.6 400. 36. D504800600020 33.5 557. 50. D504800600021 ENDDATA 11 0 D504800600022 ENDSUBENT 21 0 D504800699999 SUBENT D5048007 20070614 D056D504800700001 BIB 3 5 D504800700002 REACTION (44-RU-102(HE3,X)45-RH-101-G,CUM,SIG) D504800700003 DECAY-DATA (45-RH-101-G,3.3YR,DG,127.2,0.680,DG,198.0,0.73,DG, D504800700004 325.2,0.118) D504800700005 (45-RH-101-M,4.34D,DG,306.9,0.806,DG,545.1,0.0427) D504800700006 STATUS (APRVD,TABLE) Corresponds to fig.2 (dark squares) D504800700007 ENDBIB 5 0 D504800700008 NOCOMMON 0 0 D504800700009 DATA 3 9 D504800700010 EN DATA DATA-ERR D504800700011 MEV MB MB D504800700012 19.3 1.69 0.41 D504800700013 22.8 3.35 0.61 D504800700014 25.4 3.88 0.63 D504800700015 25.6 4.01 0.64 D504800700016 27.7 11.6 1.8 D504800700017 28.8 19.2 2.7 D504800700018 29.7 31.0 3.7 D504800700019 31.6 56.5 6.8 D504800700020 33.5 1.5 9.8 D504800700021 ENDDATA 11 0 D504800700022 ENDSUBENT 21 0 D504800799999 SUBENT D5048008 20070614 D056D504800800001 BIB 4 7 D504800800002 REACTION (44-RU-102(HE3,X)45-RH-102-M,,SIG) D504800800003 DECAY-DATA (45-RH-102-M,3.742YR,DG,475.1,0.95,DG,628.1,0.083,DG, D504800800004 631.3,0.56,DG,697.5,0.44,DG,766.8,0.34,DG,1046.6,0.34) D504800800005 COMMENT -By authors. In REACTION X corresponds to P2N+DN+T.TheD504800800006 half-life was given from (,M.Shibata+,J,ARI,49,1481, D504800800007 1998). D504800800008 STATUS (APRVD,TABLE) Corresponds to fig.2 (open circles) D504800800009 ENDBIB 7 0 D504800800010 NOCOMMON 0 0 D504800800011 DATA 3 14 D504800800012 EN DATA DATA-ERR D504800800013 MEV MB MB D504800800014 19.3 18.8 2.1 D504800800015 19.9 23.8 3.6 D504800800016 22.8 91.5 8.9 D504800800017 23.1 82.7 9.4 D504800800018 23.3 115. 12. D504800800019 25.4 152. 15. D504800800020 25.6 145. 14. D504800800021 27.7 211. 20. D504800800022 28.8 269. 26. D504800800023 29.7 265. 26. D504800800024 31.2 251. 24. D504800800025 31.6 272. 26. D504800800026 33.5 268. 26. D504800800027 33.6 260. 25. D504800800028 ENDDATA 16 0 D504800800029 ENDSUBENT 28 0 D504800899999 SUBENT D5048009 20070614 D056D504800900001 BIB 4 5 D504800900002 REACTION (44-RU-102(HE3,X)45-RH-102-G,,SIG) D504800900003 DECAY-DATA (45-RH-102-G,207.3D,DG,475.1,0.46,DG,628.1,0.045,DG, D504800900004 631.3,0.0010) D504800900005 COMMENT -By authors. In REACTION X corresponds to P2N+DN+T. D504800900006 STATUS (APRVD,TABLE) Corresponds to fig.2 (open squares) D504800900007 ENDBIB 5 0 D504800900008 NOCOMMON 0 0 D504800900009 DATA 3 15 D504800900010 EN DATA DATA-ERR D504800900011 MEV MB MB D504800900012 17.5 17.0 2.2 D504800900013 19.3 64.5 7.5 D504800900014 19.9 40.8 4.9 D504800900015 22.8 137. 15. D504800900016 23.1 99.8 11.3 D504800900017 23.3 155. 17. D504800900018 25.4 196. 21. D504800900019 25.6 166. 19. D504800900020 27.7 193. 21. D504800900021 28.8 247. 27. D504800900022 29.7 243. 27. D504800900023 31.2 208. 23. D504800900024 31.6 225. 25. D504800900025 33.5 196. 22. D504800900026 33.6 205. 22. D504800900027 ENDDATA 17 0 D504800900028 ENDSUBENT 27 0 D504800999999 ENDENTRY 9 0 D504899999999